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121.
Chloe Indermuhle Maria J. Martín de Vidales Cristina Sáez José Robles Pablo Cañizares Juan F. García-Reyes Antonio Molina-Díaz Christos Comninellis Manuel A. Rodrigo 《Chemosphere》2013
The use of Conductive-Diamond Electrochemical Oxidation (CDEO) and Sonoelectrochemical Oxidation (CDSEO) has been evaluated for the removal of caffeine of wastewater. Effects of initial concentration, current density and supporting electrolyte on the process efficiency are assessed. Results show that caffeine is very efficiently removed with CDEO and that depletion of caffeine has two stages depending on its concentration. At low concentrations, opposite to what it is expected in a mass-transfer controlled process, the efficiency increases with current density very significantly, suggesting a very important role of mediated oxidation processes on the removal of caffeine. In addition, the removal of caffeine is faster than TOC, indicating the formation of reaction intermediates. The number and relative abundance of them depend on the operating conditions and supporting electrolyte used. In chloride media, removal of caffeine is faster and more efficiently, although the occurrence of more intermediates takes place. CDSEO does not increase the efficiency of caffeine removal, but it affects to the formation of intermediates. A detailed characterization of intermediates by liquid chromatography time-of-flight mass spectrometry seems to indicate that the degradation of caffeine by CDEO follows an oxidation pathway similar to mechanism proposed by other advanced oxidation processes. 相似文献
122.
Gredilla Ainara Fdez-Ortiz de Vallejuelo Silvia Gomez-Nubla Leticia Carrero Jose Antonio de Leão Felipe B. Madariaga Juan Manuel Silva Luis F. O. 《Environmental science and pollution research international》2017,24(31):24333-24345
Environmental Science and Pollution Research - In city playgrounds, there is a potential risk of harming children’s health by contamination coming from anthropogenic activities. With the aim... 相似文献
123.
Construction and demolition waste as recycled aggregate for environmentally friendly concrete paving
Contreras Llanes Manuel Romero Pérez Maximina Gázquez González Manuel Jesús Bolívar Raya Juan Pedro 《Environmental science and pollution research international》2022,29(7):9826-9840
Environmental Science and Pollution Research - Recycled aggregates (RA) from construction and demolition waste (CDW) instead of natural aggregates (NA) were analysed in the manufacture of new... 相似文献
124.
Ângelo Barroso Cristina Chaves Francisco Vitorino Martins Manuel Castelo Branco 《Environment, Development and Sustainability》2016,18(5):1399-1414
The main purpose of this paper is to discuss whether it is possible to achieve human development without or with less economic growth. For this to happen, it is important that developed countries can maintain high levels of human development while reducing the scale of production and consumption so that developing countries can achieve greater economic growth. Using panel data from 118 countries aggregated in ten blocks of countries, we assess the influence of “growth” on “development”, as proxied by a transformed variable “Social Human Development Index” (SHDI), controlling for the influence of geo-economic factors. In particular, we analyse whether developed countries present a weaker statistical relation between GDP and the social dimension of HDI than their less developed counterparts. Results reveal that the GDP elasticity of SHDI is higher in blocks of countries where the concentration of developing countries occurs than in blocks dominated by the presence of developed countries. Thus, it is possible to envisage that a slowdown in economic activity in developed countries may occur without great sacrifice of human development, at least when it is measured by health and education components. We interpret the findings as meaning that at an aggregate level there are conditions for development to occur without or with less growth. 相似文献
125.
Boris Tartakovsky Yehuda Kleiner Michelle-France Manuel 《Environmental science and pollution research international》2018,25(33):32844-32850
This study describes a novel wastewater treatment technology suitable for small remote northern communities. The technology is based on an enhanced biodegradation of organic carbon through a combination of anaerobic methanogenic and microbial electrochemical (bioelectrochemical) degradation processes leading to biomethane production. The microbial electrochemical degradation is achieved in a membraneless flow-through bioanode–biocathode setup operating at an applied voltage below the water electrolysis threshold. Laboratory wastewater treatment tests conducted through a broad range of mesophilic and psychrophilic temperatures (5–23 °C) using synthetic wastewater showed a biochemical oxygen demand (BOD5) removal efficiency of 90–97% and an effluent BOD5 concentration as low as 7 mg L?1. An electricity consumption of 0.6 kWh kg?1 of chemical oxygen demand (COD) removed was observed. Low energy consumption coupled with enhanced methane production led to a net positive energy balance in the bioelectrochemical treatment system. 相似文献
126.
This paper analyses the relationship between nitrous oxide (N2O) emissions, economic growth, agricultural land used and exports in Germany. We use time‐series data between 1970 and 2012 and the Autoregressive Distributed Lag (ARDL) methodology to test for cointegration in the long run. Results show that there is a quadratic long run relationship between N2O emissions and economic growth, confirming the existence of an Environmental Kuznets Curve (EKC) for Germany. Agricultural land area affects N2O emissions positively, whereas exports affect emissions negatively. The turning point is $27,880, which is within the sample and implies that Germany is in the decreasing part of the curve of environmental degradation. The paper shows that, contrary to testing the EKC in less developed countries, mitigation of N2O emissions does not negatively affect growth in Germany. As such, it is feasible to undertake any conservative policy in order to reduce emissions without major consequences on economic sectors. 相似文献
127.
128.
Cristal Fernández-Gómez José Antonio López-López Victor Matamoros Sergi Díez Manuel García-Vargas Carlos Moreno 《Environmental monitoring and assessment》2013,185(4):3209-3218
In the lower Guadalquivir river basin, a system stressed by a wide variety of anthropogenic activities, eight pesticides (four triazines, two chloroacetanilide herbicides, one organochlorine, and one organophosphorus insecticide); and four emerging pollutants (two personal care products, one organophosphorous flame retardant, and one xanthine alkaloid) were analyzed in river water during a 2-year monitoring program, and after rain episodes. Samples were extracted using the solid phase extraction (SPE) technique prior to determination of compounds using gas chromatograph coupled to a mass spectrometer detector. Except for caffeine, recoveries were mostly above 80 %, while limits of detection and quantification were in the low nanograms per liter level (except for dimethoate). Terbuthylazine, simazine (triazine herbicides), and dimethoate (organophosphorus insecticide), present in agrochemicals, were predominant in the river water, although concentrations were below the quality standards established by the EU Water-Framework-Directive. A general trend to increase concentration was observed after rain events, in particular for pesticides, possibly as a consequence of surface runoff. 相似文献
129.
Benjamin Okang’ Odumo Gregoria Carbonell Hudson Kalambuka Angeyo Jayanti Purshottam Patel Manuel Torrijos José Antonio Rodríguez Martín 《Environmental science and pollution research international》2014,21(21):12426-12435
This work considered the environmental impact of artisanal mining gold activity in the Migori–Transmara area (Kenya). From artisanal gold mining, mercury is released to the environment, thus contributing to degradation of soil and water bodies. High mercury contents have been quantified in soil (140 μg kg?1), sediment (430 μg kg?1) and tailings (8,900 μg kg?1), as expected. The results reveal that the mechanism for transporting mercury to the terrestrial ecosystem is associated with wet and dry depositions. Lichens and mosses, used as bioindicators of pollution, are related to the proximity to mining areas. The further the distance from mining areas, the lower the mercury levels. This study also provides risk maps to evaluate potential negative repercussions. We conclude that the Migori–Transmara region can be considered a strongly polluted area with high mercury contents. The technology used to extract gold throughout amalgamation processes causes a high degree of mercury pollution around this gold mining area. Thus, alternative gold extraction methods should be considered to reduce mercury levels that can be released to the environment. 相似文献
130.
Occurrence of halogenated disinfection by-products (DBPs) (trihalomethanes –THMs– and haloacetic acids –HAAs–) in the waters
of two utilities in Quebec City (Canada) was investigated using two approaches: experimental chlorination studies and full-scale
sampling within distribution systems. Experimental studies were designed to reproduce treatment plant and distribution system
conditions (chlorine dose, water temperature, pH and water residence time). Differences in halogenated DBPs in the two distribution
systems under study were significant and comparable to those observed in experimental laboratory studies. For the waters of
both utilities, chlorination studies better reproduced the occurrence of halogenated DBPs in points of the distribution system
located near the treatment plant (low residence time of water) than in other points. Multivariate regression models for THMs,
HAAs and their species were developed using the data from experimental studies in order to predict halogenated DBP levels
measured in the distribution system. Models were all statistically significant, but showed low ability to predict full-scale
halogenated DBPs, particularly in points located at distribution system extremities. Specifically, experimental chlorination-based
models are not able to simulate the decrease of HAA levels. Results of this research suggest that the use of experimental
data to predict halogenated DBP levels in full-scale distribution systems – for operational, regulatory and epidemiological
purposes – must be done with caution. 相似文献