全文获取类型
收费全文 | 11333篇 |
免费 | 21篇 |
国内免费 | 29篇 |
专业分类
安全科学 | 80篇 |
废物处理 | 879篇 |
环保管理 | 1373篇 |
综合类 | 1207篇 |
基础理论 | 3371篇 |
污染及防治 | 2300篇 |
评价与监测 | 1165篇 |
社会与环境 | 997篇 |
灾害及防治 | 11篇 |
出版年
2024年 | 2篇 |
2023年 | 30篇 |
2022年 | 66篇 |
2021年 | 77篇 |
2020年 | 37篇 |
2019年 | 34篇 |
2018年 | 1507篇 |
2017年 | 1417篇 |
2016年 | 1261篇 |
2015年 | 183篇 |
2014年 | 107篇 |
2013年 | 195篇 |
2012年 | 577篇 |
2011年 | 1452篇 |
2010年 | 780篇 |
2009年 | 670篇 |
2008年 | 980篇 |
2007年 | 1304篇 |
2006年 | 107篇 |
2005年 | 106篇 |
2004年 | 94篇 |
2003年 | 99篇 |
2002年 | 129篇 |
2001年 | 27篇 |
2000年 | 15篇 |
1999年 | 13篇 |
1998年 | 16篇 |
1997年 | 4篇 |
1996年 | 5篇 |
1995年 | 5篇 |
1994年 | 5篇 |
1993年 | 2篇 |
1992年 | 2篇 |
1991年 | 4篇 |
1990年 | 4篇 |
1988年 | 5篇 |
1987年 | 2篇 |
1986年 | 3篇 |
1985年 | 3篇 |
1984年 | 13篇 |
1983年 | 10篇 |
1979年 | 2篇 |
1966年 | 2篇 |
1962年 | 2篇 |
1961年 | 2篇 |
1960年 | 2篇 |
1959年 | 2篇 |
1953年 | 2篇 |
1935年 | 2篇 |
1928年 | 2篇 |
排序方式: 共有10000条查询结果,搜索用时 15 毫秒
111.
Vanessa Moschino Luisa Da Ros 《Environmental science and pollution research international》2016,23(13):12770-12776
Biomarkers are internationally recognized as useful tools in marine coastal biomonitoring, in particular, as early-warning signals at the level of individual organisms to assess biological effects of pollutants and other stressors. In the present study, Mytilus galloprovincialis has been employed as a sentinel organism to assess biological pollution effects in the Mar Piccolo of Taranto (Southern Italy), a coastal lagoon divided into two small inlets, connected to the open sea through one natural and one artificial narrow openings. Mussels were collected in June 2013 at three sites located within each of the two inlets of the Mar Piccolo. Biological effects were investigated through a suite of biomarkers suitable to reflect effects and/or exposure to contaminants at biochemical and cellular levels. Biochemical biomarkers included glutathione-S-transferase (GST) and acetylcholinesterase (AChE) enzyme activities; as histochemical biomarkers, lysosomal membrane stability, lipofuscin and neutral lipid accumulation, and lysosomal structural changes were considered. As a whole, results highlighted differences among the three study sites, particularly for GST, AChE, and lipofuscins, which are consistent with the variations of the chemical pollutants in sediments. The applied biomarkers showed that a stress syndrome likely to be ascribed to environmental pollutants is occurring in mussels living in the Mar Piccolo of Taranto, in particular, the ones inhabiting the first inlet. 相似文献
112.
Irene M. C. Lo Kok Sin Woon 《Environmental science and pollution research international》2016,23(8):7081-7091
About 3600 tonnes food waste are discarded in the landfills in Hong Kong daily. It is expected that the three strategic landfills in Hong Kong will be exhausted by 2020. In consideration of the food waste management environment and community needs in Hong Kong, as well as with reference to the food waste management systems in cities such as Linköping in Sweden and Oslo in Norway, a framework of food waste separation, collection, and recycling for food waste valorization is proposed in this paper. Food waste can be packed in an optic bag (i.e., a bag in green color), while the residual municipal solid waste (MSW) can be packed in a common plastic bag. All the wastes are then sent to the refuse transfer stations, in which food waste is separated from the residual MSW using an optic sensor. On the one hand, the sorted food waste can be converted into valuable materials (e.g., compost, swine feed, fish feed). On the other hand, the sorted food waste can be sent to the proposed Organic Waste Treatment Facilities and sewage treatment works for producing biogas. The biogas can be recovered to produce electricity and city gas (i.e., heating fuel for cooking purpose). Due to the challenges faced by the value-added products in Hong Kong, the biogas is recommended to be upgraded as a biogas fuel for vehicle use. Hopefully, the proposed framework will provide a simple and effective approach to food waste separation at source and promote sustainable use of waste to resource in Hong Kong. 相似文献
113.
Yi-Tang Chang Jiunn-Fwu Lee Keng-Hua Liu Yi-Fen Liao Vivian Yang 《Environmental science and pollution research international》2016,23(5):4024-4035
Nonionic surfactant-modified clay is a useful absorbent material that effectively removes hydrophobic organic compounds from soil/groundwater. We developed a novel material by applying an immobilized fungal laccase onto nonionic surfactant-modified clay. Low-water-solubility polycyclic aromatic hydrocarbons (PAHs) (naphthalene/phenanthrene) were degraded in the presence of this bioactive material. PAH degradation by free laccase was higher than degradation by immobilized laccase when the surfactant concentration was allowed to form micelles. PAH degradation by immobilized laccase on TX-100-modified clay was higher than on Brij35-modified clay. Strong laccase degradation of PAH can be maintained by adding surfactant monomers or micelles. The physical adsorption of nonionic surfactants onto clay plays an important role in PAH degradation by laccase, which can be explained by the structure and molecular interactions of the surfactant with the clay and enzyme. A system where laccase is immobilized onto TX-100-monomer-modified clay is a good candidate bioactive material for in situ PAHs bioremediation. 相似文献
114.
Zhigao Sun Xiaojie Mou 《Environmental science and pollution research international》2016,23(6):5189-5202
From April 2008 to November 2009, a field decomposition experiment was conducted to investigate the effects of sediment burial on macro (C, N) and microelement (Pb, Cr, Cu, Zn, Ni, and Mn) variations in decomposing litter of Phragmites australis in the coastal marsh of the Yellow River estuary. Three one-off sediment burial treatments [no sediment burial (0 mm year?1, S0), current sediment burial (100 mm year?1, S10), and strong sediment burial (200 mm year?1, S20)] were laid in different decomposition sites. Results showed that sediment burials showed significant influence on the decomposition rate of P. australis, in the order of S10 (0.001990 day?1)?≈?S20 (0.001710 day?1)?>?S0 (0.000768 day?1) (p?<?0.05). The macro and microelement in decomposing litters of the three burial depths exhibited different temporal variations except for Cu, Zn, and Ni. No significant differences in C, N, Pb, Cr, Zn, and Mn concentrations were observed among the three burial treatments except for Cu and Ni (p?>?0.05). With increasing burial depth, N, Cr, Cu, Ni, and Mn concentrations generally increased, while C, Pb, and Zn concentrations varied insignificantly. Sediment burial was favorable for C and N release from P. australis, and, with increasing burial depth, the C release from litter significantly increased, and the N in litter shifted from accumulation to release. With a few exceptions, Pb, Cr, Zn, and Mn stocks in P. australis in the three treatments evidenced the export of metals from litter to environment, and, with increasing burial depth, the export amounts increased greatly. Stocks of Cu and Ni in P. australis in the S10 and S20 treatments were generally positive, evidencing incorporation of the two metals in most sampling times. Except for Ni, the variations of C, N, Pb, Cr, Cu, Zn, and Mn stocks in P. australis in the S10 and S20 treatments were approximated, indicating that the strong burial episodes (S20) occurred in P. australis marsh in the future would have little influence on the stocks of these elements. With increasing burial depths, the P. australis was particularly efficient in binding Cu and Ni and releasing C, N, Pb, Cr, Zn, and Mn, implying that the potential eco-toxic risk of Pb, Cr, Zn, and Mn exposure might be very serious. This study emphasized the effects of different burials on nutrient and metal cycling and mass balance in the P. australis marsh of the Yellow River estuary. 相似文献
115.
116.
Stuart G. Wakeham Elizabeth A. Canuel 《Environmental science and pollution research international》2016,23(11):10426-10442
Biogenic perylene and higher plant pentacyclic triterpenoid-derived alkylated and partially aromatized tetra- and pentacyclic derivatives of chrysene (3,4,7-trimethyl- and 3,3,7-trimethyl-1,2,3,4-tetrahydrochrysene, THC) and picene (1,2,9-trimethyl- and 2,2,9-trimethyl-1,2,3,4-tetrahydropicene, THP) were two- to four-fold more abundant than pyrogenic PAH in two sediment cores from the San Joaquin River in Northern California (USA). In a core from Venice Cut (VC), located in the river, PAH concentrations varied little downcore and the whole-core PAH concentration (biogenics?+?pyrogenics) was 250.6?±?73.7 ng g?1 dw; biogenic PAH constituted 67?±?4 % of total PAH. THC were 26?±?9 % of total biogenic PAH, THP were 36?±?7 %, and perylene was 38?±?7 %. PAH distributions in a core from Franks Tract (FT), a former wetland that was converted to an agricultural tract in the late 1800s and flooded in 1938, were more variable. Surface sediments were dominated by pyrogenic PAH so that biogenic PAH were only ~30 % of total PAH. Deeper in the core, biogenic PAH constituted 60–93 % of total PAH; THC, THP and perylene were 31?±?28 %, 24?±?32 %, and 45?±?36 % of biogenic PAH. At 100–103 cm depth, THP constituted 80 % of biogenic PAH and at 120–123 cm perylene was 95 % of biogenic PAH. Current concepts related to precursors and transformation processes responsible for the diagenetic generation of perylene and triterpenoid-derived PAH are discussed. Distributions of biogenic PAH in VC and FT sediments suggest that they may not form diagenetically within these sediments but rather might be delivered pre-formed from the river’s watershed. 相似文献
117.
Martina Horáčková Klára Řehounková Karel Prach 《Environmental science and pollution research international》2016,23(14):13617-13625
Seed characteristics play an important role in the colonization and subsequent persistence of species during succession in disturbed sites and thus may contribute to being able to predict restoration success. In the present study, we investigated how various seed characteristics participated in 11 spontaneous successional series running in different mining sites (spoil heaps, extracted sand and sand-gravel pits, extracted peatlands, and stone quarries) in the Czech Republic, Central Europe. Using 1864 samples from 1- to 100-years-old successional stages, we tested whether species optimum along the succession gradient could be predicted using 10 basic species traits connected with diaspores and dispersal. Seed longevity, diaspore mass, endozoochory, and autochory appeared to be the best predictors. The results indicate that seed characteristics can predict to a certain degree spontaneous vegetation succession, i.e., passive restoration, in the mining sites. A screening of species available in the given landscape (regional and local species pools) may help to identify those species which would potentially colonize the disturbed sites. Extensive databases of species traits, nowadays available for the Central European flora, enable such screening. 相似文献
118.
Impact of temperature on the dynamics of organic matter and on the soil-to-plant transfer of Cd,Zn and Pb in a contaminated agricultural soil 总被引:1,自引:0,他引:1
Jean-Yves Cornu L. Denaix J. Lacoste V. Sappin-Didier C. Nguyen A. Schneider 《Environmental science and pollution research international》2016,23(4):2997-3007
Predicting the soil-to-plant transfer of metals in the context of global warming has become a major issue for food safety. It requires a better understanding of how the temperature alters the bioavailability of metals in cultivated soils. This study focuses on one agricultural soil contaminated by Cd, Zn and Pb. DGT measurements were performed at 10, 20 and 30 °C to assess how the bioavailability of metals was affected by a rise in soil temperature. A lettuce crop was cultivated in the same conditions to determine if the soil-to-plant transfer of metals increased with a rise in soil temperature. A gradual decline in Cd and Zn bioavailability was observed from 10 to 30 °C, which was attributed to more intense complexation of metals in the pore water at higher temperatures. Together with its aromaticity, the affinity of dissolved organic matter (DOM) for metals was indeed suspected to increase with soil temperature. One main output of the present work is a model which satisfactorily explains the thermal-induced changes in the characteristics of DOM reported in Cornu et al. (Geoderma 162:65–70, 2011) by assuming that the mineralization of initial aliphatic compounds followed a first-order reaction, increased with soil temperature according to the Arrhenius law, and due to a priming effect, led to the appearance of aromatic molecules. The soil-to-plant transfer of Cd and Zn was promoted at higher soil temperatures despite a parallel decrease in Cd and Zn bioavailability. This suggests that plant processes affect the soil-to-plant transfer of Cd and Zn the most when the soil temperature rises. 相似文献
119.
Bhargav M. M. S. R. S. Ratna Kishore V. Anbuudayasankar S. P. Balaji K. 《Environmental science and pollution research international》2016,23(10):9381-9390
Demand for green energy production is arising all over the world. A lot of emphasis is laid in making the buildings green. Even a small amount of energy savings made contribute to saving the environment. In this study, an idea is proposed and studied to extract power from the high head water in the pipelines of a building. A building of height 15 m is considered for this study. Water flowing in the pipe has sufficient energy to run a micro hydro turbine. The feasibility of producing electrical energy from the energy of pipe water is found. The motivation is to find the feasibility of generating power using a low-cost turbine. The experimental setup consists of micro turbine of 135 mm diameter coupled to a 12-V DC generator; LEDs and resistors are employed to validate the results. The theoretical calculations were presented using the fundamental equations of fluid mechanics. The theoretical results are validated using experimental and numerical results using CFD simulation. In addition, exergy analysis has been carried out to quantify the irreversibilities during the process in the system. 相似文献
120.
Yeonjung Lee Bomi Lee Jin Hur Jun-Oh Min Sun-Yong Ha Kongtae Ra Kyung-Tae Kim Kyung-Hoon Shin 《Environmental science and pollution research international》2016,23(9):8358-8366
In order to understand the biodegradability of algal-derived organic matter, biodegradation experiments were conducted with 13C and 15N-labeled natural phytoplankton and periphytic algal populations in experimental conditions for 60 days. Qualitative changes in the dissolved organic matter were also determined using parallel factor analysis and the stable carbon isotopic composition of the hydrophobic dissolved organic matter through the experimental period. Although algal-derived organic matter is considered to be easily biodegradable, the initial amounts of total organic carbon newly produced by phytoplankton and periphytic algae remained approximately 16 and 44 % after 60 days, respectively, and about 22 and 43 % of newly produced particulate nitrogen remained. Further, the dissolved organic carbon derived from both algal populations increased significantly after 60 days. Although the dissolved organic matter gradually became refractory, the contributions of the algal-derived organic matter to the dissolved organic matter and hydrophobic dissolved organic matter increased. Our laboratory experimental results suggest that algal-derived organic matter produced by phytoplankton and periphytic algae could contribute significantly to the non-biodegradable organic matter through microbial transformations. 相似文献