全文获取类型
收费全文 | 13374篇 |
免费 | 148篇 |
国内免费 | 111篇 |
专业分类
安全科学 | 375篇 |
废物处理 | 344篇 |
环保管理 | 1992篇 |
综合类 | 3377篇 |
基础理论 | 3149篇 |
环境理论 | 7篇 |
污染及防治 | 3356篇 |
评价与监测 | 590篇 |
社会与环境 | 372篇 |
灾害及防治 | 71篇 |
出版年
2018年 | 130篇 |
2017年 | 130篇 |
2016年 | 192篇 |
2015年 | 159篇 |
2014年 | 200篇 |
2013年 | 970篇 |
2012年 | 316篇 |
2011年 | 446篇 |
2010年 | 316篇 |
2009年 | 417篇 |
2008年 | 455篇 |
2007年 | 489篇 |
2006年 | 447篇 |
2005年 | 329篇 |
2004年 | 348篇 |
2003年 | 383篇 |
2002年 | 328篇 |
2001年 | 470篇 |
2000年 | 326篇 |
1999年 | 226篇 |
1998年 | 156篇 |
1997年 | 150篇 |
1996年 | 179篇 |
1995年 | 178篇 |
1994年 | 203篇 |
1993年 | 182篇 |
1992年 | 186篇 |
1991年 | 183篇 |
1990年 | 209篇 |
1989年 | 197篇 |
1988年 | 168篇 |
1987年 | 165篇 |
1986年 | 149篇 |
1985年 | 167篇 |
1984年 | 152篇 |
1983年 | 161篇 |
1982年 | 164篇 |
1981年 | 165篇 |
1980年 | 150篇 |
1979年 | 145篇 |
1978年 | 144篇 |
1977年 | 130篇 |
1976年 | 138篇 |
1975年 | 114篇 |
1974年 | 146篇 |
1973年 | 126篇 |
1972年 | 126篇 |
1971年 | 108篇 |
1970年 | 107篇 |
1967年 | 120篇 |
排序方式: 共有10000条查询结果,搜索用时 15 毫秒
991.
We describe a patient with a significantly elevated serum alphafetoprotein (AFP) concentration at 17 weeks of gestation, who showed only a marginally increased amniotic fluid AFP and lacked the second rapidly migrating band of acetylcholinesterase electrophoresis. Ultrasound examination revealed an encephalocele and ventriculomegaly. Autopsy showed that the encephalocele was not covered by skin. 相似文献
992.
White CM Strazisar BR Granite EJ Hoffman JS Pennline HW;Air & Waste Management Association 《Journal of the Air & Waste Management Association (1995)》2003,53(6):645-715
The topic of global warming as a result of increased atmospheric CO2 concentration is arguably the most important environmental issue that the world faces today. It is a global problem that will need to be solved on a global level. The link between anthropogenic emissions of CO2 with increased atmospheric CO2 levels and, in turn, with increased global temperatures has been well established and accepted by the world. International organizations such as the United Nations Framework Convention on Climate Change (UNFCCC) and the Intergovernmental Panel on Climate Change (IPCC) have been formed to address this issue. Three options are being explored to stabilize atmospheric levels of greenhouse gases (GHGs) and global temperatures without severely and negatively impacting standard of living: (1) increasing energy efficiency, (2) switching to less carbon-intensive sources of energy, and (3) carbon sequestration. To be successful, all three options must be used in concert. The third option is the subject of this review. Specifically, this review will cover the capture and geologic sequestration of CO2 generated from large point sources, namely fossil-fuel-fired power gasification plants. Sequestration of CO2 in geological formations is necessary to meet the President's Global Climate Change Initiative target of an 18% reduction in GHG intensity by 2012. Further, the best strategy to stabilize the atmospheric concentration of CO2 results from a multifaceted approach where sequestration of CO2 into geological formations is combined with increased efficiency in electric power generation and utilization, increased conservation, increased use of lower carbon-intensity fuels, and increased use of nuclear energy and renewables. This review covers the separation and capture of CO2 from both flue gas and fuel gas using wet scrubbing technologies, dry regenerable sorbents, membranes, cryogenics, pressure and temperature swing adsorption, and other advanced concepts. Existing commercial CO2 capture facilities at electric power-generating stations based on the use of monoethanolamine are described, as is the Rectisol process used by Dakota Gasification to separate and capture CO2 from a coal gasifier. Two technologies for storage of the captured CO2 are reviewed--sequestration in deep unmineable coalbeds with concomitant recovery of CH4 and sequestration in deep saline aquifers. Key issues for both of these techniques include estimating the potential storage capacity, the storage integrity, and the physical and chemical processes that are initiated by injecting CO2 underground. Recent studies using computer modeling as well as laboratory and field experimentation are presented here. In addition, several projects have been initiated in which CO2 is injected into a deep coal seam or saline aquifer. The current status of several such projects is discussed. Included is a commercial-scale project in which a million tons of CO2 are injected annually into an aquifer under the North Sea in Norway. The review makes the case that this can all be accomplished safely with off-the-shelf technologies. However, substantial research and development must be performed to reduce the cost, decrease the risks, and increase the safety of sequestration technologies. This review also includes discussion of possible problems related to deep injection of CO2. There are safety concerns that need to be addressed because of the possibilities of leakage to the surface and induced seismic activity. These issues are presented along with a case study of a similar incident in the past. It is clear that monitoring and verification of storage will be a crucial part of all geological sequestration practices so that such problems may be avoided. Available techniques include direct measurement of CO2 and CH4 surface soil fluxes, the use of chemical tracers, and underground 4-D seismic monitoring. Ten new hypotheses were formulated to describe what happens when CO2 is pumped into a coal seam. These hypotheses provide significant insight into the fundamental chemical, physical, and thermodynamic phenomena that occur during coal seam sequestration of CO2. 相似文献
993.
IntroductionChengdu KunmingRailwayLineislocatedonthemountainregionofsouthwesternChina .Therearealotofdebrisflowgulliesspreadingbesidethisrailwayline .Onsummer,thedebrisflowoftenburstsandthreatensthesafetyoftherailwaytransportation.In 1981,alarge scaledebris… 相似文献
994.
Schmidt TS Clements WH Wanty RB Verplanck PL Church SE San Juan CA Fey DL Rockwell BW DeWitt EH Klein TL 《Ecological applications》2012,22(3):870-879
Geologic processes strongly influence water and sediment quality in aquatic ecosystems but rarely are geologic principles incorporated into routine biomonitoring studies. We test if elevated concentrations of metals in water and sediment are restricted to streams downstream of mines or areas that may discharge mine wastes. We surveyed 198 catchments classified as "historically mined" or "unmined," and based on mineral-deposit criteria, to determine whether water and sediment quality were influenced by naturally occurring mineralized rock, by historical mining, or by a combination of both. By accounting for different geologic sources of metals to the environment, we were able to distinguish aquatic ecosystems limited by metals derived from natural processes from those due to mining. Elevated concentrations of metals in water and sediment were not restricted to mined catchments; depauperate aquatic communities were found in unmined catchments. The type and intensity of hydrothermal alteration and the mineral deposit type were important determinants of water and sediment quality as well as the aquatic community in both mined and unmined catchments. This study distinguished the effects of different rock types and geologic sources of metals on ecosystems by incorporating basic geologic processes into reference and baseline site selection, resulting in a refined assessment. Our results indicate that biomonitoring studies should account for natural sources of metals in some geologic environments as contributors to the effect of mines on aquatic ecosystems, recognizing that in mining-impacted drainages there may have been high pre-mining background metal concentrations. 相似文献
995.
Biological plugs are an innovative, low-intervention, in-situ bioremediation methodology for both saturated and unsaturated contaminated soils. They are modular in-ground immobilized microbe bioreactors designed to rapidly increase the oxidation of organic contaminants by placing an adapted consortia of microorganisms in close proximity to the contaminants of concern. The approach is versatile, in that contaminants can be remediated in-situ without the removal of existing structures as well as being able to efficiently and economically treat contaminants over a large area. Amine- and glycol-contaminated soils at gas sweetening plants, represent a significant problem in magnitude, prevalence, and risk along pipelines stretching through Canada's western provinces. A field pilot study was conducted at an isolated former gas sweetening plant in northwestern Alberta. Monoethyamine (MEA) and several glycols were successfully remediated in situ in a 138-day time frame. Soil toxicity was significantly reduced. The engineering challenges and associated economics of remediating such isolated sites are also presented. 相似文献
996.
In 1605 a destructive earthquake affected the northern region of Hainan Island and adjacent parts of the Chinese mainland. Based on a detailed analysis of contemporary chronicles, the authors present a revision of the effects of the earthquake, and show that a sequence of strong shocks throughout 1605 caused cumulative damage and relatively heavy loss of life in Qiongshan. The subsidence of large areas of coast round Puqian Bay and Dongzhai Port is shown to be due to a combination of liquefaction caused by the shock, the occurrence of a typhoon associated with flooding and exacerbated by a high surge tide, as well as a long-term process of active tectonic movement in the area; the subsidence was not caused by downthrow of the earth's crust during the shock. Topographical changes in the area, traced from historical maps, suggest that subsidence is continuing, but a survey of the long-term seismicity of Hainan Island indicates that it is not an area of exceptional seismic risk. 相似文献
997.
Research on community characteristics of riparian herbs is an important scientific basis of riparian vegetation rehabilitation. This study aimed to investigate the species diversity and quantitative characteristics of riparian herbs in Liaohe River Conservation Area and its tributaries. Herbaceous communities were investigated by sample line method. Group average clustering analysis and detrended correspondence analysis (DCA) were used to find the major environmental factors affecting the distribution pattern of riparian herbaceous communities. The result showed altogether 154 herbaceous species, belonging to 40 families and 96 genera. The riparian herbaceous species diversity was found to be correlated to river slope, sinuosity and stream order, being lower in rivers of mountain area than in rivers of plain area, and higher in tributaries than in Liaohe River Conservation Area. Clustering analysis classified the herbaceous communities into 23 types, being dominated by hygrophytes including communities of Echinochloa crusgalli, Oenanthe javanica, Polygonum hydropiper, Murdannia keisak, Artemisia selengensis, Scirpus triqueter, Heleocharis soloniensis, Pycreus sanguinolentus, Cyperus fuscus, Phragmites australis, Polygonum amphibium, Carex diandra + Artemisia selengensis and Carex diandra + Rorippa islandica. Correlation analysis between DCA ordination axes and environmental factors showed that the altitude, river slope, sinuosity and stream level were the major environmental factors affecting the distribution pattern of herbaceous communities in the riparian zone of Liaohe River Conservation Area and its tributaries. The results of CCA showed that the contribution ratio of stream level was the highest, followed by altitude and slope, with sinuosity the last. The results suggested that riparian herbaceous characteristics are affected by the comprehensive force of altitude, river slope, sinuosity and stream order, and that Calamagrostis epigeios, Triarrhena sacchariflora and Phragmites australis are suitable species for riparian vegetation rehabilitation. 相似文献
998.
Common shrimp, Crangon crangon (L.), were exposed to inorganic arsenic (arsenate), trimethylarsine oxide, or arsenobetaine in sea water (100 μg As l−1) or in food (1 mg As g−1 wet wt) for up to 24 d, followed by 16 d depuration in clean sea water with undosed food, in order to determine the efficiency
of uptake and retention of the compounds. Accumulation of arsenic in the tail muscle, gills, midgut gland, exoskeleton, and
remaining tissues was found to depend on the chemical form of the arsenic and the route of exposure. No arsenic was accumulated
by C. crangon exposed to arsenate or trimethylarsine oxide in sea water. Shrimps exposed to waterborne arsenobetaine initially accumulated
a small amount of arsenic in their tail muscle and gills. After 16 d, C. crangon fed arsenate, trimethylarsine oxide, or arsenobetaine had accumulated arsenic in their tail muscle to levels ∼2-, 2-, or
40-times, respectively, that of the control group. A roughly linear rate of accumulation was shown by shrimps fed trimethylarsine
oxide or arsenobetaine, but C. crangon fed arsenate accumulated arsenic for 16 d, then lost arsenic such that their concentration on Day 24 was not significantly
different from that of the control group. Patterns of arsenic accumulation in the gills of shrimps fed the compounds were
similar to those seen in the tail muscle. On a whole animal basis, C. crangon retained ∼1.2% of the arsenate, 1.6% of the trimethylarsine oxide, and 42% of the arsenobetaine consumed over the first 16 d
of exposure, with roughly half present in the tail muscle in each case. Data obtained support the view that the direct uptake
of arsenobetaine from sea water does not make a significant contribution to the relatively high concentrations of this compound
in marine crustaceans, and that food is the primary source. Naturally occurring arsenic compounds in C. crangon and possible transformations of the administered arsenic compounds were examined by high performance liquid chromatography
using an inductively coupled plasma mass spectrometer as the arsenic-specific detector. Control C. crangon contained arsenobetaine as the major arsenic compound (>95% of total arsenic); tetramethylarsonium ion (0.7%) and an unknown
arsenic compound (1.7%) were also present as minor constituents. Shrimp ingesting arsenobetaine accumulated it unchanged.
Shrimp ingesting arsenate did not form methylated arsenic compounds; they appeared to contain their accumulated arsenic as
unchanged arsenate only, although the possibility that some of the arsenic was reduced to arsenite could not be excluded.
C. crangon ingesting trimethylarsine oxide biotransformed the compound predominantly to dimethylarsinate.
Received: 9 October 1997 / Accepted: 11 February 1998 相似文献
999.
E. Blondeel M. Chys V. Depuydt K. Folens G. Du laing A. Verliefde S.W.H. Van Hulle 《Waste management (New York, N.Y.)》2014,34(12):2674-2686
Scrap material recovery and recycling companies are confronted with waste water that has a highly fluctuating flow rate and composition. Common pollutants, such as COD, nutrients and suspended solids, potentially toxic metals, polyaromatic hydrocarbons and poly chlorinated biphenyls can exceed the discharge limits. An analysis of the leaching behaviour of different scrap materials and scrap yard sweepings was performed at full-scale, pilot-scale and lab-scale in order to find possible preventive solutions for this waste water problem. The results of these leaching tests (with concentrations that frequently exceeded the Flemish discharge limits) showed the importance of regular sweeping campaigns at the company, leak proof or covered storage of specific scrap materials and oil/water separation on particular leachates. The particulate versus dissolved fraction was also studied for the pollutants. For example, up to 98% of the polyaromatic hydrocarbons, poly chlorinated biphenyls and some metals were in the particulate form. This confirms the (potential) applicability of sedimentation and filtration techniques for the treatment of the majority of the leachates, and as such the rainwater run-off as a whole. 相似文献
1000.
Alexander Lorenz Matthias G. W. Schmidt Elmar Kriegler Hermann Held 《Environmental Modeling and Assessment》2012,17(1-2):163-175
Several integrated assessment studies have concluded that future learning about the uncertainties involved in climate change has a considerable effect on welfare but only a small effect on optimal short-term emissions. In other words, learning is important but anticipation of learning is not. We confirm this result in the integrated assessment model “model of investment and technological development” for learning about climate sensitivity and climate damages. If learning about an irreversible threshold is included, though, we show that anticipation can become crucial both in terms of necessary adjustments of pre-learning emissions and resulting welfare gains. We specify conditions on the time of learning and the threshold characteristic, for which this is the case. They can be summarized as a narrow “anticipation window.” 相似文献