全文获取类型
收费全文 | 21047篇 |
免费 | 359篇 |
国内免费 | 373篇 |
专业分类
安全科学 | 838篇 |
废物处理 | 887篇 |
环保管理 | 3316篇 |
综合类 | 3390篇 |
基础理论 | 5354篇 |
环境理论 | 10篇 |
污染及防治 | 5383篇 |
评价与监测 | 1268篇 |
社会与环境 | 1171篇 |
灾害及防治 | 162篇 |
出版年
2023年 | 102篇 |
2022年 | 197篇 |
2021年 | 203篇 |
2020年 | 230篇 |
2019年 | 204篇 |
2018年 | 357篇 |
2017年 | 367篇 |
2016年 | 520篇 |
2015年 | 421篇 |
2014年 | 567篇 |
2013年 | 1708篇 |
2012年 | 761篇 |
2011年 | 1089篇 |
2010年 | 824篇 |
2009年 | 947篇 |
2008年 | 1011篇 |
2007年 | 1055篇 |
2006年 | 906篇 |
2005年 | 752篇 |
2004年 | 757篇 |
2003年 | 686篇 |
2002年 | 660篇 |
2001年 | 730篇 |
2000年 | 579篇 |
1999年 | 370篇 |
1998年 | 255篇 |
1997年 | 285篇 |
1996年 | 263篇 |
1995年 | 313篇 |
1994年 | 263篇 |
1993年 | 256篇 |
1992年 | 209篇 |
1991年 | 210篇 |
1990年 | 203篇 |
1989年 | 206篇 |
1988年 | 172篇 |
1987年 | 148篇 |
1986年 | 172篇 |
1985年 | 165篇 |
1984年 | 207篇 |
1983年 | 175篇 |
1982年 | 189篇 |
1981年 | 189篇 |
1980年 | 145篇 |
1979年 | 164篇 |
1978年 | 108篇 |
1977年 | 101篇 |
1975年 | 92篇 |
1974年 | 95篇 |
1972年 | 102篇 |
排序方式: 共有10000条查询结果,搜索用时 885 毫秒
691.
This study has indicated that there is close relationship between development density and environmental quality; therefore,
it is necessary to decide the form of development carefully beforehand. The form of development is shaped either by new development
or urban renewal which is a major tactic nowadays adopted by the Hong Kong Government to improve the living condition of the
citizens and the quality of the built environment. This study is limited to urban renewal and aims to find out the major urban
design considerations for sustaining the environment. Through a questionnaire survey carried out in Hong Kong, the opinions
of architects, planners, property development managers, and local citizens were sought and evaluated, and critical design
factors for enhancing environmental sustainability of urban renewal projects are highlighted. The results derived from factor
analysis indicated that certain design considerations should be incorporated for sustaining the urban environment. “Land Use
Planning”, “Quality of Life”, “Conservation & Preservation”, “Integrated Design”, “Provision of Welfare Facilities”, and “Conservation
of Existing Properties” were believed to be the significant underlying factors for achieving environmental sustainability
of local urban renewal projects.
Readers should send their comments on this paper to: BhaskarNath@aol.com within 3 months of publication of this issue. 相似文献
692.
The potential adverse effects on human health of hazardous waste incinerators (HWIs) are a subject of concern. The construction of the first and till now only HWI in Spain finished in 1999. In 2007, after approximately 9 years of regular operations in the facility, the concentrations of polychlorinated dibenzo-p-dioxins and dibenzofurans (PCDD/F) were determined by HRGC/HRMS in samples of adipose tissue of 15 autopsied subjects living in the area under potential impact of the HWI (Constantí, Tarragona County, Catalonia). These data were compared with the levels found in two previous surveys performed in 1998 (baseline) and 2002. The current mean PCDD/F concentration in adipose tissue was 14.6 pg WHO-TEQ/g of fat (range: 3.3–55.4 pg WHO-TEQ/g of fat). It means significant changes (a reduction of 64% and an increase of 47%) in the mean PCDD/F levels in comparison to those found in 1998 and 2002: 40.1 and 9.9 pg WHO-TEQ/g of fat, respectively. Women showed higher levels of PCDD/F than men (23.8 vs 11.2 pg WHO-TEQ/g of fat). The increase in the last 5 years would not be directly attributable to exposure to PCDD/F emitted by the HWI, as other biological monitors such as human plasma and milk decreased during the same period. 相似文献
693.
April L. Pulvirenti Karen M. Needham Mohamad A. Adel-Hadadi Charles R. Marks Jeffrey A. Gorman Donald L. Shettel Aaron Barkatt 《Journal of contaminant hydrology》2009,109(1-4):62-81
Thermal evaporation of a variety of simulated pore waters from the region of Yucca Mountain, Nevada, produced acidic liquids and gases during the final stages of evaporation. Several simulated pore waters were prepared and then thermally distilled in order to collect and analyze fractions of the evolved vapor. In some cases, distillates collected towards the end of the distillation were highly acidic; in other cases the pH of the distillate remained comparatively unchanged during the course of the distillation. The results suggest that the pH values of the later fractions are determined by the initial composition of the water. Acid production stems from the hydrolysis of magnesium ions, especially at near dryness. Near the end of the distillation, magnesium nitrate and magnesium chloride begin to lose water of hydration, greatly accelerating their thermal decomposition to form acid. Acid formation is promoted further when precipitated calcium carbonate is removed. Specifically, calcium chloride-rich pore waters containing moderate (10–20 ppm) levels of magnesium and nitrate and low levels of bicarbonate produced mixtures of nitric and hydrochloric acid, resulting in a precipitous drop in pH to values of 1 or lower after about 95% of the original volume was distilled. Waters with either low or moderate magnesium content coupled with high levels of bicarbonate produced slightly basic fractions (pH 7–9). If calcium was present in excess of bicarbonate, waters containing moderate levels of magnesium produced acid even in the presence of bicarbonate, due to the precipitation of calcium carbonate. Other salts such as halite and anhydrite promote the segregation of acidic vapors from residual basic solids. The concomitant release of wet acid gas has implications for the integrity of the alloys under consideration for containers at the Yucca Mountain nuclear waste repository. Condensed acid gases at very low pH, especially mixtures of nitric and hydrochloric acid, are capable of corroding even alloys, such as nickel-based Alloy 22, which are considered to be corrosion-resistant under milder conditions. 相似文献
694.
Erik Krznaric Jan H.L. Wevers Jaco Vangronsveld 《Environmental pollution (Barking, Essex : 1987)》2009,157(5):1581-1588
Soil metal pollution can trigger evolutionary adaptation in soil-borne organisms. An in vitro screening test showed cadmium adaptation in populations of Suillus luteus (L.: Fr.) Roussel, an ectomycorrhizal fungus of pine trees. Cadmium stress was subsequently investigated in Scots pine (Pinus sylvestris L.) seedlings inoculated with a Cd-tolerant S. luteus, isolated from a heavy metal contaminated site, and compared to plants inoculated with a Cd-sensitive isolate from a non-polluted area. A dose-response experiment with mycorrhizal pines showed better plant protection by a Cd-adapted fungus: more fungal biomass and a higher nutrient uptake at high Cd exposure. In addition, less Cd was transferred to aboveground plant parts. Because of the key role of the ectomycorrhizal symbiosis for tree fitness, the evolution of Cd tolerance in an ectomycorrhizal partner such as S. luteus can be of major importance for the establishment of pine forests on Cd-contaminated soils. 相似文献
695.
Fate of pharmaceuticals and personal care products in wastewater treatment plants - Conception of a database and first results 总被引:1,自引:0,他引:1
C. Miège J.M. Choubert L. Ribeiro M. Eusèbe M. Coquery 《Environmental pollution (Barking, Essex : 1987)》2009,157(5):1721-1726
We created a database in order to quantitatively assess the occurrence and removal efficiency of pharmaceuticals and personal care products (PPCPs) in wastewater treatment plants (WWTPs). From 117 scientific publications, we compiled 6641 data covering 184 PPCPs. Data included the concentrations of PPCPs in WWTP influents and effluents, their removal efficiency and their loads to the aquatic environment. The first outputs of our database allowed to identify the most investigated PPCPs in WWTPs and the most persistent ones, and to obtain reliable and quantitative values on their concentrations, frequency of detection and removal efficiency in WWTPs. We were also able to compare various processes and pointed out activated sludge with nitrogen treatment and membrane bioreactor as the most efficient ones. 相似文献
696.
Yoram Tencer Gil Idan Marjorie Strom Uri Nusinow Dorit Banet Eli Cohen Peter Schröder Oren Shelef Shimon Rachmilevitch Ines Soares Amit Gross Avi Golan-Goldhirsh 《Environmental science and pollution research international》2009,16(7):862-875
Background, aim, and scope
The project was set to construct an extensive wetland in the southernmost region of Israel at Kibbutz Neot Smadar (30°02′45″ N and 35°01′19″ E). The results of the first period of monitoring, summary, and perspectives are presented. The constructed wetland (CW) was built and the subsequent monitoring performed in the framework of the Southern Arava Sustainable Waste Management Plan, funded by the EU LIFE Fund. The specific aims were: (1) To end current sewage disposal and pollution of the ground, the aquifer, and the dry river bed (wadi) paths by biologically treating the sewage as part of the creation of a sustainable wetland ecosystem. (2) Serve as an example of CW in the Negev highlands and the Arava Valley climates for neighboring communities and as a test ground for plants and building methods appropriate to hyper arid climate. (3) Serve as an educational resource and tourist attraction for groups to learn about water reuse, recycling, local wildlife and migrating birds, including serving the heart of a planned Ecological–Educational Bird Park. This report is intended to allow others who are planning similar systems in hyper arid climates to learn from our experience.Materials and methods
The project is located in an extreme arid desert with less than 40 mm of rain annually and temperature ranges of ?5°C to +42°C. The site receives 165–185 m3 of municipal and agricultural wastes daily, including cowshed and goat wastes and winery outflow.Results
The CW establishment at Neot Smadar was completed in October 2006. For 8 months, clean water flowed through the system while the plants were taking root. In June 2007, the wetland was connected to the oxidation pond and full operation began. Because of seepage and evaporation, during the first several months, the water level was not high enough to allow free flow from one bed to the next. To bed A, the water was pumped periodically from the oxidation pond (Fig. 1) and from there flowed by gravitation through the rest of the system. The initial results of the monitoring are promising. In nearly all measurements, the system succeeded as expected to reduce levels of contaminants at least to the level acceptable for irrigating fruit trees and often to the level of unlimited irrigation. The introduction of the plants in the system and their physiological performance were evaluated and were found to correlate well to the quality of water in the various beds.Discussion
It should be said at the outset that evaluation of the performance of a CW system is a long-term process. Thus, the main aim of this report is to present the problems, difficulties, preliminary results, and concepts concerned with the first stage of establishment of CW in an extremely dry region.Conclusions
The CW system was designed to dispose of municipal and agricultural wastes in a way that not merely reduces pollution, but adds to environmental quality by creating accessible parkland for local residents and tourists. Several factors affected the performance of the system at the initial stages of operation: ecological balance between microbes and plants, big seasonal variations, seepage and evaporation reduced the flow in the initial operation of the system. Despite the initial difficulties, the quality of water coming out the system is acceptable for irrigation.Recommendations and perspectives
The CW can function well under extreme dryland conditions. The oxidation pond was the major source of evaporation and bad odors. Therefore, alternatives to the oxidation pond are needed. Cost effectiveness of the system still has to be evaluated systematically. 相似文献697.
Shelly L. Miller Peter Scaramella Joseph Campe Cynthia W. Goss Sandra Diaz-Castillo Ed Hendrikson Carolyn DiGuiseppi Jill Litt 《Atmospheric environment (Oxford, England : 1994)》2009,43(35):5661-5667
An indoor air quality assessment was conducted on 100 homes of recent Mexican immigrants in Commerce City, Colorado, an urban industrial community north of Denver. Head of households were administered a family health survey, filled out an activity diary, and participated in a home inspection. Carbon monoxide (CO) and carbon dioxide (CO2) were measured for 24 h inside the main living area and outside of the homes. Harvard Impactors were used to collect 24-h samples of PM2.5 at the same locations for gravimetric analysis. Dust samples were collected by vacuuming carpeting and flooring at four locations within the home and analyzed by ELISA for seven allergens. Mean indoor and outdoor PM2.5 levels were 27.2 and 8.5 μg m−3, respectively. Indoor PM2.5 and CO2 were elevated in homes for which the number of hours with door/window open was zero compared to homes in which the number of hours was high (>15 h). Indoor PM2.5 levels did not correlate with outdoor levels and tended to increase with number of inhabitants, and results indicate that the source of indoor particles were occupants and their activities, excluding smoking and cooking. Mean indoor CO2 and CO levels were 1170 and 2.4 ppm, respectively. Carbon monoxide was higher than the 24-h National Ambient Air Quality Standard in 3 of the homes. The predominant allergens were cat (Fel d 1) and mouse (Mus m 1) allergens, found in 20 and 34 homes, respectively. 相似文献
698.
L.J. Deacon L.J. Pankhurst G.H. Drew E.T. Hayes S. Jackson P.J. Longhurst J.W.S. Longhurst J. Liu S.J.T. Pollard S.F. Tyrrel 《Atmospheric environment (Oxford, England : 1994)》2009,43(35):5698-5701
Information on the particle size distribution of bioaerosols emitted from open air composting operations is valuable in evaluating potential health impacts and is a requirement for improved dispersion simulation modelling. The membrane filter method was used to study the particle size distribution of Aspergillus fumigatus spores in air 50 m downwind of a green waste compost screening operation at a commercial facility. The highest concentrations (approximately 8 × 104 CFU m−3) of culturable spores were found on filters with pore diameters in the range 1–2 μm which suggests that the majority of spores are emitted as single cells. The findings were compared to published data collected using an Andersen sampler. Results were significantly correlated (p < 0.01) indicating that the two methods are directly comparable across all particles sizes for Aspergillus spores. 相似文献
699.
Andrea L. Clements Yuling Jia Allison Denbleyker Elena McDonald-Buller Matthew P. Fraser David T. Allen Donald R. Collins Edward Michel Jayanth Pudota David Sullivan Yifang Zhu 《Atmospheric environment (Oxford, England : 1994)》2009,43(30):4523-4534
Spatial gradients of vehicular emitted air pollutants were measured in the vicinity of three roadways in the Austin, Texas area: (1) State Highway 71 (SH-71), a heavily traveled arterial highway dominated by passenger vehicles; (2) Interstate 35 (I-35), a limited access highway north of Austin in Georgetown; and (3) Farm to Market Road 973 (FM-973), a heavily traveled surface roadway with significant truck traffic. A mobile monitoring platform was used to characterize the gradients of CO and NOx concentrations with increased distance from each roadway, while concentrations of carbonyls in the gas-phase and fine particulate matter mass and composition were measured at stationary sites upwind and at one (I-35 and FM-973) or two (SH-71) downwind sites. Regardless of roadway type or wind direction, concentrations of carbon monoxide (CO), nitric oxide (NO), and oxides of nitrogen (NOx) returned to background levels within a few hundred meters of the roadway. Under perpendicular wind conditions, CO, NO and NOx concentrations decreased exponentially with increasing distance perpendicular to the roadways. The decay rate for NO was more than a factor of two greater than for CO, and it comprised a larger fraction of NOx closer to the roadways than further downwind suggesting the potential significance of near roadway chemical processing as well as atmospheric dilution. Concentrations of most carbonyl species decreased with distance downwind of SH-71. However, concentrations of acetaldehyde and acrolein increased farther downwind of SH-71, suggesting chemical generation from the oxidation of primary vehicular emissions. The behavior of particle-bound organic species was complex and further investigation of the size-segregated chemical composition of particulate matter (PM) at increasing downwind distances from roadways is warranted. Fine particulate matter (PM2.5) mass concentrations, polycyclic aromatic hydrocarbons (PAHs), hopanes, and elemental carbon (EC) concentrations generally exhibited concentrations that decreased with distance downwind of SH-71. Concentrations of organic carbon (OC) increased from upwind concentrations immediately downwind of SH-71 and continued to increase further downwind from the roadway. This behavior may have primarily resulted from condensation of semi-volatile organic species emitted from vehicle sources with transport downwind of the roadway. 相似文献
700.
Marisia P. Esposito Mauricio L. Ferreira Silvia M.R. Sant'Anna Marisa Domingos Silvia R. Souza 《Atmospheric environment (Oxford, England : 1994)》2009,43(3):619-623
Previous studies have reported that the extent of leaf injury in Nicotiana tabacum “Bel-W3” exposed to environmental conditions in the city of São Paulo is influenced by weather conditions. This influence may occur by means of antioxidant responses. Thus, this study aimed to evaluate whether daily antioxidant responses to environmental variations interfere on the progression of leaf injury on plants of this cultivar during their exposure in a state park of São Paulo and to determine a linear combination of variables, among antioxidants and environmental factors, which mostly explain this visible response. Plants were exposed at the mentioned site for 14 days in four different experiments. During each experiment, three plants were daily sampled to determine the accumulated percentage of leaf area affected by necrosis and antioxidant responses (concentrations of total ascorbic acid (AA) and activity of superoxide dismutase (SOD) and peroxidases (POD)). Ozone concentrations and weather conditions were also daily measured. Pearson correlations and multivariate analyses assessed the relationship between biological and environmental variables. Leaf injury appeared between the 3rd and 6th days of exposure and increased over the exposure periods. The daily concentrations of AA tended to decrease with time of exposure in all experiments, but the activity of SOD and POD oscillated during plant exposure. Positive correlations were observed between AA or SOD and O3 concentrations, as well as negative correlations between AA and air temperature. The increasing percentage of leaf necrosis across the whole period was explained by decreasing levels of AA 2 days before injury estimation and by higher O3 concentrations 5 days before (R2 = 0.36; p < 0.001). The use of N. tabacum Bel-W3 as a bioindicator can be restricted by leaf antioxidant responses to both atmospheric contamination and weather conditions. 相似文献