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921.
Attention has been focused on the treatment of lignite-fired flue gas in order to use lignite in an environmentally friendly way – (i) low-CO2 emission, (ii) production of a valuable by-product, (iii) no discharge of wastewater, (iv) direct removal of SO3 (strong toxicity), and (v) treatment of high SO2 concentration. Based on these criteria, electron beam irradiation with ammonia injection was tested on a semi-pilot scale: 800 Nm3 h?1 flow rate, 5500 ppm SO2, 70 ppm NOx, 22% flue gas moisture, and 75–80 °C at the reactor outlet.As an energy-saving measure, a low dose (5 kGy) of irradiation was applied: the problem lay in the by-product quality. It is considered that (NH4)2SO3 and NH4HSO3 produced by thermal reactions are oxidized to form (NH4)2SO4 (fertilizer) by an electron beam. However, not all reactions were complete because the by-product contained small amounts of H2SO4 and NH2SO3NH4 (herbicide), so a vegetable pot test was performed to study the by-product quality: no adverse effect was observed. It is inferred from the pot test that slightly acidic soil may protect vegetables from disease and a small amount of NH2SO3NH4 probably affects woody species and not herbaceous species.It is concluded that the electron beam system is noted as a multi-component pollution control process (removal of NOx, SO3, SO2 and dioxins) and this system will contribute to environmentally friendly use of lignite as well as agricultural productivity via fertilizer supply. 相似文献
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Managing the nitrogen cycle to reduce greenhouse gas emissions from crop production and biofuel expansion 总被引:1,自引:0,他引:1
Stephen M. Ogle Bruce A. McCarl Justin Baker Stephen J. Del Grosso Paul R. Adler Keith Paustian William J. Parton 《Mitigation and Adaptation Strategies for Global Change》2016,21(8):1197-1212
Public policies are promoting biofuels as an alternative to fossil fuel consumption in order to mitigate greenhouse gas (GHG) emissions. However, the mitigation benefit can be at least partially compromised by emissions occurring during feedstock production. One of the key sources of GHG emissions from biofuel feedstock production, as well as conventional crops, is soil nitrous oxide (N2O), which is largely driven by nitrogen (N) management. Our objective was to determine how much GHG emissions could be reduced by encouraging alternative N management practices through application of nitrification inhibitors and a cap on N fertilization. We used the US Renewable Fuel Standards (RFS2) as the basis for a case study to evaluate technical and economic drivers influencing the N management mitigation strategies. We estimated soil N2O emissions using the DayCent ecosystem model and applied the US Forest and Agricultural Sector Optimization Model with Greenhouse Gases (FASOMGHG) to project GHG emissions for the agricultural sector, as influenced by biofuel scenarios and N management options. Relative to the current RSF2 policy with no N management interventions, results show decreases in N2O emissions ranging from 3 to 4 % for the agricultural sector (5.5–6.5 million metric tonnes CO2?eq.?year?1; 1 million metric tonnes is equivalent to a Teragram) in response to a cap that reduces N fertilizer application and even larger reductions with application of nitrification inhibitors, ranging from 9 to 10 % (15.5–16.6 million tonnes CO2?eq.?year?1). The results demonstrate that climate and energy policies promoting biofuel production could consider options to manage the N cycle with alternative fertilization practices for the agricultural sector and likely enhance the mitigation of GHG emissions associated with biofuels. 相似文献
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H.P. Jarvie P.J.A. Withers M.J. Bowes E.J. Palmer-Felgate D.M. Harper K. Wasiak P. Wasiak R.A. Hodgkinson A. Bates C. Stoate M. Neal H.D. Wickham S.A. Harman L.K. Armstrong 《Agriculture, ecosystems & environment》2010,135(4):238-252
This paper provides an overview of the impacts of rural land use on lowland streamwater phosphorus (P) and nitrogen (N) concentrations and P loads and sources in lowland streams. Based on weekly water quality monitoring, the impacts of agriculture on streamwater P and N hydrochemistry were examined along a gradient of rural–agricultural land use, by monitoring three sets of ‘paired’ (near-adjacent) rural headwater streams, draining catchments which are representative of the major geology, soil types and rural/agricultural land use types of large areas of lowland Britain. The magnitude and timing of P and N inputs were assessed and the load apportionment model (LAM) was applied to quantify ‘continuous’ (point) source and ‘flow-dependent’ (diffuse) source contributions of P to these headwater streams. The results show that intensive arable farming had only a comparatively small impact on streamwater total phosphorus (TP loads), with highly consistent stream diffuse-source TP yields of ca. 0.5 kg-P ha?1 year?1 for the predominantly arable catchments with both clay and loam soils, compared with 0.4 kg-P ha?1 year?1 for low agricultural intensity grassland/woodland on similar soil types. In contrast, intensive livestock farming on heavy clay soils resulted in dramatically higher stream diffuse-source TP yields of 2 kg-P ha?1 year?1. The streamwater hydrochemistry of the livestock-dominated catchment was characterised by high concentrations of organic P, C and N fractions, associated with manure and slurry sources. Across the study sites, the impacts of human settlement were clearly identifiable with effluent inputs from septic tanks and sewage treatment works resulting in large-scale increases in soluble reactive phosphorus (SRP) loads and concentrations. At sites heavily impacted by rural settlements, SRP concentrations under baseflow conditions reached several hundred μg-P L?1. Load apportionment modelling demonstrated significant ‘point-source’ P inputs to the streams even where there were no sewage treatment works within the upstream catchment. This indicates that, even in sparsely populated rural headwater catchments, small settlements and even isolated groups of houses are sufficient to cause significant nutrient pollution and that septic tank systems serving these rural communities are actually operating as multiple point sources, rather than a diffuse input. 相似文献
929.
Daniela C.A. Pigosso Evelyn T. Zanette Américo Guelere Filho Aldo R. Ometto Henrique Rozenfeld 《Journal of Cleaner Production》2010,18(1):21-31
Understanding the product's ‘end-of-life’ is important to reduce the environmental impact of the products' final disposal. When the initial stages of product development consider end-of-life aspects, which can be established by ecodesign (a proactive approach of environmental management that aims to reduce the total environmental impact of products), it becomes easier to close the loop of materials. The ‘end-of-life’ ecodesign methods generally include more than one ‘end-of-life’ strategy. Since product complexity varies substantially, some components, systems or sub-systems are easier to be recycled, reused or remanufactured than others. Remanufacture is an effective way to maintain products in a closed-loop, reducing both environmental impacts and costs of the manufacturing processes. This paper presents some ecodesign methods focused on the integration of different ‘end-of-life’ strategies, with special attention to remanufacturing, given its increasing importance in the international scenario to reduce the life cycle impacts of products. 相似文献
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