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G. B. Davis C. Barber T. R. Power J. Thierrin B. M. Patterson J. L. Rayner Qinglong Wu 《Journal of contaminant hydrology》1999,36(3-4)
Data from long-term groundwater sampling, limited coring, and associated studies are synthesised to assess the variability and intrinsic remediation/natural attenuation of a dissolved hydrocarbon plume in sulphate-rich anaerobic groundwater. Fine vertical scale (0.25- and 0.5-m depth intervals) and horizontal plume-scale (>400 m) characteristics of the plume were mapped over a 5-year period from 1991 to 1996. The plume of dissolved BTEX (benzene, toluene, ethylbenzene, xylene) and other organic compounds originated from leakage of gasoline from a subsurface fuel storage tank. The plume was up to 420 m long, less than 50 m wide and 3 m thick. In the first few years of monitoring, BTEX concentrations near the point of leakage were in approximate equilibrium with non-aqueous phase liquid (NAPL) gasoline. NAPL composition of core material and long-term trends in ratios of BTEX concentrations in groundwater indicated significant depletion (water washing, volatilisation and possibly biodegradation) of benzene from residual NAPL after 1992. Large fluctuations in BTEX concentrations in individual boreholes were shown to be largely attributable to seasonal groundwater flow variations. A combination of temporal and spatial groundwater quality data was required to adequately assess the stationarity of plumes, so as to allow inference of intrinsic remediation. Contoured concentration data for the period 1991 to 1996 indicated that plumes of toluene and o-xylene were, at best, only partially steady state (pseudo-steady state) due to seasonal groundwater flow changes. From this analysis, it was inferred that significant remediation by natural biodegradation was occurring for BTEX component plumes such as toluene and o-xylene, but provided no conclusive evidence of benzene biodegradation. Issues associated with field quantification of intrinsic remediation from groundwater sampling are highlighted. Preferential intrinsic biodegradation of selected organic compounds within the BTEX plume was shown to be occurring, in parallel with sulphate reduction and bicarbonate production. Ratios of average hydrocarbon concentrations to benzene for the period 1991 to 1992 were used to estimate degradation rates (half-lives) at various distances along the plume. The estimates varied with distance, the narrowest range being, for toluene, 110 to 260 days. These estimates were comparable to rates determined previously from an in situ tracer test and from plume-scale modelling. 相似文献
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Glenn T. Crossin Scott G. Hinch Steven J. Cooke David W. Welch Sonia D. Batten David A. Patterson Glen Van Der Kraak J. Mark Shrimpton Anthony P. Farrell 《Marine Biology》2007,152(4):905-918
Adult sockeye salmon (Oncorhynchus nerka, N = 179) from six Fraser River populations (British Columbia) were intercepted in continental shelf waters ∼215 km from the
Fraser River mouth, gastrically implanted with acoustic transmitters, non-lethally biopsied for blood biochemistry, gill Na+,K+-ATPase activity and somatic energy density and then released. Migration behaviour and travel times to the river mouth and
into the river were monitored by underwater telemetry receivers positioned at the river mouth and in the river. Post-release
survival of salmon was excellent, with 84% (N = 150) of fish reaching the furthest receiving station ∼85 km upriver. Fish from Late-summer run populations (Adams and Weaver
Creek) averaged a migration rate of ∼20 km day−1 through the marine area and held at the river mouth and adjacent areas for 7–9 days before entering the river. Summer-run
populations (Birkenhead, Chilko, Horsefly and Stellako) had a migration rate ∼33 km day−1 and held for only 1–3 days. Once in river, similar patterns were observed: Late-run populations migrated at ∼28 km day−1 and Summer-run populations at ∼40 km day−1. From point of release to the river mouth, males migrated faster than females, but once in river migration rates did not
differ between sexes. Among all females, a correlation was discovered between levels of circulating testosterone and river
entry timing. This correlation was not observed among males. Plasma K+, Cl−, glucose, lactate and osmolality were also correlated with entry timing in both sexes. 相似文献
16.
Reproductive value and appropriateness of response to predators by White-Crowned Sparrows 总被引:2,自引:3,他引:2
Summary Twenty-five pair of breeding Whitecrowned Sparrows were presented with a live snake and models of a hawk, jay, and junco. Pairs were tested either when the female was brooding eggs, feeding nestlings, or fledglings. It was found that the snake was responded to the most when the pair had nestlings, very little when the female was brooding eggs, and at a moderate level with fledglings. The hawk and jay models were responded to the least with eggs, more with nestlings, and the most with fledglings. The junco model elicited little response. Both the pattern and level of response is influenced by whether or not the stimulus represents an effective predator at the particular stage of the breeding cycle. They also are influenced by the reproductive value of the progeny. A model is suggested that includes two factors: stimulus value and reproductive value. We propose that this combined model is more suitable than a single factor one. 相似文献
17.
We examined physiological stress responses in the edible crab, Cancer pagurus, subjected to the commercial fishery practice of manual de-clawing. We measured haemolymph glucose and lactate, plus muscular
glycogen and glycogen mobilisation, in three experiments where the crabs had one claw removed. In the first, crabs showed
physiological stress responses when ‘de-clawed’ as compared to ‘handled only’ over the short term of 1–10 min. In the second,
de-clawing and the presence of a conspecific both increased the physiological stress responses over the longer term of 24 h.
In the third, de-clawing was shown to be more stressful than ‘induced autotomy’ of claws. Further, the former practice caused
larger wounds to the body and significantly higher mortality than the latter. Since the fishery practice is to remove both
claws, the stress response observed and mortality data reported are conservative. 相似文献
18.
Saito K Sjödin A Sandau CD Davis MD Nakazawa H Matsuki Y Patterson DG 《Chemosphere》2004,57(5):373-381
A new analytical method has been developed for the quantification of 59 different persistent organohalogen compounds, such as polybrominated diphenyl ethers (PBDEs), polychlorinated naphthalenes (PCNs), polychlorinated biphenyls (PCBs), PCB metabolites, organochlorine pesticides (OCPs) in biological organ tissues. The optimum extraction and cleanup procedures were examined using accelerated solvent extraction (ASE), automated gel permeation chromatography (GPC) on Biobeads S-X3 and automated solid phase extraction (SPE) on silica-gel. The target compounds were divided into two fractions, non-polar compounds and more polar compounds, which in the latter fraction was subsequently methylated using diazomethane. Detection can be achieved by GC/MS in negative chemical ionization (NCI) mode. The average recoveries of the compounds spiked in swine liver, heart, kidney, and cattle adipose tissues were considered satisfactory, and it was confirmed that the method could be used in routine analysis. 相似文献
19.
Kang HK Dalager NA Needham LL Patterson DG Matanoski GM Kanchanaraksa S Lees PS 《Chemosphere》2001,43(4-7):943-949
The long-term health consequences of exposure to phenoxyherbicides used in Vietnam has been a great concern to the veterans. In addition to the Air Force Ranch Hand personnel, Army Chemical Corps personnel who served in Vietnam are thought to have had some of the highest herbicide exposures. The Department of Veterans Affairs commenced a study of veterans who served in Vietnam as members of the Army Chemical Corps and a comparison cohort of Army Chemical Corps personnel who served elsewhere. A total of 2872 Vietnam veterans and 2737 non-Vietnam veterans who served in the Army Chemical Corps were identified for inclusion in a telephone health interview survey with a random 20% sample of veterans receiving serum dioxin and other congeners assessments. In a feasibility study which included 284 Vietnam veterans and 281 non-Vietnam veterans, 100 serum assessments were conducted of which 95 were included in the analysis. Vietnam veterans with a history of spraying herbicides were found to have a statistically significant elevation in their current serum 2,3,7,8-TCDD concentrations compared to non-Vietnam veterans without a spray history (P = 0.05). Other 2,3,7,8-substituted dioxins levels were comparable to the levels found in the non-Vietnam veterans. This feasibility study demonstrated that serum dioxin concentrations from a sample of the study participants can be used to identify exposure variables in the health survey that can serve as a surrogate measure of phenoxyherbicide exposure. 相似文献
20.
Cardelino C Chang M St John J Murphey B Cordle J Ballagas R Patterson L Powell K Stogner J Zimmer-Dauphinee S 《Journal of the Air & Waste Management Association (1995)》2001,51(8):1227-1236
Ozone prediction has become an important activity in many U.S. ozone nonattainment areas. In this study, we describe the ozone prediction program in the Atlanta metropolitan area and analyze the performance of this program during the 1999 ozone-forecasting season. From May to September, a team of 10 air quality regulators, meteorologists, and atmospheric scientists made a daily prediction of the next-day maximum 8-hr average ozone concentration. The daily forecast was made aided by two linear regression models, a 3-dimensional air quality model, and the no-skill ozone persistence model. The team's performance is compared with the numerical models using several numerical indicators. Our analysis indicated that (1) the team correctly predicted next-day peak ozone concentrations 84% of the time, (2) the two linear regression models had a better performance than a 3-dimensional air quality model, (3) persistence was a strong predictor of ozone concentrations with a performance of 78%, and (4) about half of the team's wrong predictions could be prevented with improved meteorological predictions. 相似文献