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331.
332.
Fernández-Guisuraga José Manuel Castro Amaya Alves Célia Calvo Ana Alonso-Blanco Elisabeth Blanco-Alegre Carlos Rocha Alfredo Fraile Roberto 《Environmental science and pollution research international》2016,23(17):17171-17182
Environmental Science and Pollution Research - This study provides an analysis of the spatial distribution and trends of NO, NO2 and O3 concentrations in Portugal between 1995 and 2010.... 相似文献
333.
Eric M. Fujita David E. Campbell William R. Stockwell Emily Saunders Rosa Fitzgerald Roberto Perea 《Journal of the Air & Waste Management Association (1995)》2016,66(2):201-214
This study examined the effects of varying future reductions in emissions of oxides of nitrogen (NOx) and volatile organic compounds (VOC) on the location and magnitude of peak ozone levels within California’s South Coast Air Basin (SoCAB or Basin). As ozone formation is currently VOC-limited in the Basin, model simulations with 2030 baseline emissions (?61% for NOx and ?32% for VOC from 2008) predict 10–20% higher peak ozone levels (i.e., NOx disbenefit) in the western and central SoCAB compared with the 2008 base simulation. With additional NOx reductions of 50% beyond the 2030 baseline emissions (?81% from 2008), the predicted ozone levels are reduced by about 15% in the eastern SoCAB but remain comparable to 2008 levels in the western and central Basin. The Basin maximum ozone site shifts westward to more populated areas of the Basin and will result potentially in greater population-weighted exposure to ozone with even a relatively small shortfall in the required NOx reductions unless accompanied by additional VOC reductions beyond 2030 baseline levels. Once committed to a NOx-focused control strategy, NOx reductions exceeding 90% from 2008 levels will be necessary to attain the ozone National Ambient Air Quality Standards (NAAQS). The findings from this study and other recent work that the current VOC emission estimates are underestimated by about 50% suggest that greater future VOC reductions will be necessary to reach the projected 2030 baseline emissions. Increasing the base year VOC emissions by a factor of 1.5 result in higher 2008 baseline ozone predictions, lower relative response factors, and about 20% lower projected design values. If correct, these findings have important implications for the total and optimum mix of VOC and NOx emission reductions that will be required to attain the ozone NAAQS in the SoCAB.Implications: Results of this study indicate that ozone levels in the western and central SoCAB would remain the same or increase with even a relatively small shortfall in the projected NOx reductions under planned NOx-focused controls. This possibility, therefore, warrants a rigorous analysis of the costs and effects of varying reductions of VOC and NOx on the formation and combined health impacts of ozone and secondary particles. Given the nonlinearity of ozone formation, such analyses should include the implications of gradually increasing global background ozone concentrations and the Basin’s topography and meteorology on the practical limits of alternative emission control strategies. 相似文献
334.
Cíntia Melazo Dias Everaldo C. Telles Roberto Ventura Santos Kristina Stenström Iêda Gomes Nícoli Rosangela da Silveira Corrêa Göran Skog 《Journal of environmental radioactivity》2009
Nuclear power plants release 14C during routine operation mainly as airborne gaseous effluents. Because of the long half-life (5730 years) and biological importance of this radionuclide (it is incorporated in plant tissue by photosynthesis), several countries have monitoring programs in order to quantify and control these emissions. This paper compares the activity of 14C in soils taken within 1 km from a Brazilian nuclear power plant with soils taken within a reference area located 50 km away from the reactor site. Analyses of total carbon, δ13C and 137Cs were also performed in order to understand the local soil dynamics. Except for one of the profiles, the isotopic composition of soil organic carbon reflected the actual forest vegetation present in both areas. The 137Cs data show that the soils from the base of hills are probably allocthonous. 相似文献
335.
PCDD/Fs in ambient air in north-east Italy: The role of a MSWI inside an industrial area 总被引:1,自引:0,他引:1
Andrea Colombo Emilio Benfenati Giulio Mariani Marco Lodi Roberto Marras Giuseppe Rotella Vincenzo Senese Elena Fattore Roberto Fanelli 《Chemosphere》2009,77(9):1224-1229
The stack gases of a municipal solid waste incinerator (MSWI), and ambient air were sampled in four locations around the plant for the analysis of polychlorinated dibenzo-p-dioxins and polychlorinated dibenzofurans (PCDDs/Fs). The sampling area was close to an industrial area near Trieste, in north-east Italy. The purpose of the study was to estimate the impact of the MSWI emissions and to distinguish the contribution of these emissions from other potential emission sources in the industrial area.PCDD/F atmospheric concentrations were similar to those generally detected in urban–rural areas with one location about 2–3 times more contaminated than the others. Since the most contaminated location was inside the industrial area but upwind of the MSWI, principal component analysis (PCA) was used to establish whether other sources were the cause. This analysis clearly showed that a local steel plant’s emission was the main source of PCDDs/Fs in ambient air. This study highlights the usefulness of multivariate data analysis such as PCA to identify, among different potential emission sources, the one really responsible for the contamination. 相似文献
336.
Gerosa G Marzuoli R Rossini M Panigada C Meroni M Colombo R Faoro F Iriti M 《Environmental pollution (Barking, Essex : 1987)》2009,157(5):1727-1736
Stomatal ozone uptake, determined with the Jarvis' approach, was related to photosynthetic efficiency assessed by chlorophyll fluorescence and reflectance measurements in open-top chamber experiments on Phaseolus vulgaris. The effects of O3 exposure were also evaluated in terms of visible and microscopical leaf injury and plant productivity. Results showed that microscopical leaf symptoms, assessed as cell death and H2O2 accumulation, preceded by 3-4 days the appearance of visible symptoms. An effective dose of ozone stomatal flux for visible leaf damages was found around 1.33 mmol O3 m−2. Significant linear dose-response relationships were obtained between accumulated fluxes and optical indices (PRI, NDI, ΔF/Fm′). The negative effects on photosynthesis reduced plant productivity, affecting the number of pods and seeds, but not seed weight. These results, besides contributing to the development of a flux-based ozone risk assessment for crops in Europe, highlight the potentiality of reflectance measurements for the early detection of ozone stress. 相似文献
337.
Mike F. Quartacci Barbara Irtelli Roberto Gabbrielli 《Environmental pollution (Barking, Essex : 1987)》2009,157(10):2697-2703
Due to relatively high chelant dosages and potential environmental risks it is necessary to explore different approaches in the remediation of metal-contaminated soils. The present study focussed on the removal of metals (As, Cd, Cu, Pb and Zn) from a multiple metal-contaminated soil by growing Brassica carinata plants in succession to spontaneous metallicolous populations of Pinus pinaster, Plantago lanceolata and Silene paradoxa. The results showed that the growth of the metallicolous populations increased the extractable metal levels in the soil, which resulted in a higher accumulation of metals in the above-ground parts of B. carinata. Root exudates of the three metallicolous species were analysed to elucidate their possible role in the enhanced metal availability. The presence of metals stimulated the exudation of organic and phenolic acids as well as flavonoids. It was suggested that root exudates played an important role in solubilising metals in soil and in favouring their uptake by roots. 相似文献
338.
Josef CF Adriano LR De França EJ Arantes de Carvalho GG Ferreira JR 《Environmental pollution (Barking, Essex : 1987)》2008,152(3):592-596
An analytical procedure for the determination of Hg in otter (Lontra longicaudis) feces was developed, to separate fish scales for the identification of the animal diet. Samples were washed with ultra-pure water and the suspension was sampled and transferred for digestion. The solubilization was performed with nitric-perchloric acid mixture, and detection carried out by the atomic fluorescence spectrometry (AFS). The quality of the analytical procedure was assessed by analyzing in-house standard solutions and certified reference materials. Total Hg concentrations were in the range of 7.6-156 ng g(-1) (July 2004), 25.6-277 ng g(-1) (January 2005) and 14.6-744 ng g(-1) (May 2005) that is approximately the same order of magnitude for all samples collected in two reservoirs at the Tiete River, Brazil. Although Hg concentrations varied with sampling periods and diet, high levels were correlated to the percentage of carnivorous fish scales present in the otter feces. 相似文献
339.
340.
D'Alessandro W Bellomo S Parello F Bonfanti P Brusca L Longo M Maugeri R 《Environmental monitoring and assessment》2012,184(5):2845-2855
Water samples collected from public drinking water supplies in Sicily were analysed for electric conductivity and for their
chloride, sulphate and nitrate contents. The samples were collected as uniformly as possible from throughout the Sicilian
territory, with an average sampling density of about one sample for every 7,600 inhabitants. Chloride contents that ranged
from 5.53 to 1,302 mg/l were correlated strongly with electric conductivity, a parameter used as a proxy for water salinity.
The highest values are attributable to seawater contamination along the coasts of the island. High chloride and sulphate values
attributable to evaporitic rock dissolution were found in the central part of Sicily. The nitrate concentrations ranged from
0.05 to 296 mg/l, with 31 samples (4.7% of the total) exceeding the maximum admissible concentration of 50 mg/l. Anomalous
samples always came from areas of intensive agricultural usage, indicating a clear anthropogenic origin. The same parameters
were also measured in bottled water sold in Sicily, and they all were within the ranges for public drinking water supplies.
The calculated mean nitrate intake from consuming public water supplies (16.1 mg/l) did not differ significantly from that
of bottled water (15.2 mg/l). Although the quality of public water supplies needs to be improved by eliminating those that
do not comply with the current drinking water limits, at present it does not justify the high consumption of bottled water
(at least for nitrate contents). 相似文献