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891.
Hanwant Bir Singh L. J. Salas L. A. Cavanagh 《Journal of the Air & Waste Management Association (1995)》2013,63(4):332-336
Based on two comprehensive field studies conducted in California, background concentration (parts per trillion) of N2O (296.0 X 103), SF6 (0.16), CCI2F2 (180.8), CCI3F (103.8), CCI2FCCIF2 (16.3), CCI4 (114.2), CH3CI (952.9), CHCI3 (23.4), CH3I (2.4), CH3CCI3 (84.0), CCI2CCI2 (43.1), CHCICCI2 (14.5) and CH3Br (—) have been reported. These trace constituents were identified using retention data on eight GC columns, their electron attachment properties, and their EC thermal response. All but CHCICCI2 and CH3Br were measurable 100% of the time at both sites. Cryogenic procedures for SF6 ambient measurement were developed and successfully used. By an analysis of worldwide emissions of these trace constituents, their ambient levels, and their atmospheric lifetimes, it was possible to determine their origin (natural or anthropogenic). Our results indicate that 27% of organic chlorine contribution to the troposphere comes from fluorocarbons as opposed to a 73% contribution from the chloro-carbons. Further, the anthropogenic organic content in the troposphere was found to be about twice the natural content. Very high CHCI3 concentrations in onshore ocean waters were measured. Ambient data supporting the anthropogenic origin of CCI4 have been presented. 相似文献
892.
A Wind Tunnel Study of Gaseous Pollutants in City Street Canyons 总被引:1,自引:0,他引:1
James B. Wedding David J. Lombardi Jack E. Cermak 《Journal of the Air & Waste Management Association (1995)》2013,63(6):557-566
Steady state mean concentrations of tracer gas were measured in a 400:1 scale model of an idealized city with variable geometry placed within a wind tunnel at various orientations to the mean flow for a free stream velocity of 6.8 ft/sec. The tracer gas was released from two parallel line sources to simulate lanes of traffic in an effort to quantify the persistence of pollution as well as the mean values realized at street levels. An aerodynamically rough turbulent boundary layer of neutral thermal stratification was employed to simulate the atmosphere. Values of concentration measured in the model city were converted to prototype concentrations in ppm and compared to National Ambient Air Quality Standards. It was shown that single isolated structures may cause favorable mixing of pollution downwind but very high concentrations exist in the immediate leeward vicinity of the building. Two favorable geometries for city blocks tested were found to reduce pedestrian exposure to pollution both near heavy traffic congestion and downwind. It was concluded that the pollutant dilution was controlled by the mean flow rather than by turbulent diffusion and that the lateral spread of the plume was slight as one proceeded downwind of the line source. The combination of favorable geometry and higher dilution velocities may bring pollution levels down to existing Air Quality Standards. The body of information presented in this paper should interest city planners and air quality monitoring personnel, as well as those researchers attempting to study and model flow in city street canyons. It provides order of magnitude estimates on pedestrian and office worker exposure to pollutants under a wide range of conditions. 相似文献
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894.
Brian P. Leaderer Theodore R. Holford Jan A. J. Stolwijk 《Journal of the Air & Waste Management Association (1995)》2013,63(2):154-157
A PM10 monitoring network was established throughout the South Coast Air Basin (SOCAB) in the greater Los Angeles region during the calendar year 1986. Annual average PM10 mass concentrations within the Los Angeles metropolitan area ranged from 47.0 µg m-3 along the coast to 87.4 µg m-3 at Rubldoux, the furthest inland monitoring station. Measurements made at San Nicolas Island suggest that regional background aerosol contributes between 28 to 44 percent of the PM10 aerosol at monitoring sites In the SOCAB over the long term average. Five major aerosol components (carbonaceous material, NO- 3, SO= 4, NH+ 4, and soil-related material) account for greater than 80 percent of the annual average PM10 mass at all on-land monitoring stations. Peak 24-h average mass concentrations of nearly 300 µg m-3 were observed at inland locations, with lower peak values (?130–150 µg m-3) measured along the coast. Peak-day aerosol composition was characterized by increased NO- 3 Ion and associated ammonium ion levels, as compared to the annual average. There appears to be only a weak dependence of PM10 mass concentration on season of the year. This lack of a pronounced seasonal dependence results from the complex and contradictory seasonal variations in the major chemical components (carbonaceous material, nitrate, sulfate, ammonium ion and crustal material). At most sites within the Los Angeles metropolitan area, PM10 mass concentrations exceeded both the annual and 24-h average federal and state of California PM10 regulatory standards. 相似文献
895.
G. Van Houte B. Delmon J.C. Maon Ph. Dumont 《Journal of the Air & Waste Management Association (1995)》2013,63(10):1030-1033
This publication concerns the dry removal of SO2 from gases using limestone absorbents. It reports bench-scale experiments made with commercial samples of powdered limestone (CaCO3) activated by addition of a cheap substance, namely CaCl2. The absorption was carried out in a fluidized bed traversed by the flue gases, between 600° and 900° C. The degree and rate of transformation of CaCO3 to CaSO4 in the presence of SO2 and air have been compared for unmodified and modified absorbents. Initial rates of reaction, and the variation of the rate of absorption with time have been measured. The influence of the SO2 content of the gas has been assessed. At 700° C, the maximum degree of transformation of activated limestone to sulfate exceeds 90%, whereas untreated CaCO3 transforms only to 16–20%. At the same temperature, more than 90% of SO2 contained In a gas carrying 0.35% SO2 is removed. Because of the much smaller quantity of solid absorbent required, dry absorption processes based on the modified absorbents might get renewed interest. The modified absorbents might also be used for in situ absorption in fluidized bed combustion, in which the temperatures are in the range studied in the present paper. 相似文献
896.
897.
David Leith Michael J. Ellenbecker 《Journal of the Air & Waste Management Association (1995)》2013,63(8):877-881
Presently, there is no effective way to interpret or predict dust penetration through a pulse-jet cleaned fabric filter. This paper presents a model which considers penetration straight through the filter and penetration by seepage. A considerable number of studies have been devoted to penetration by the straight through process; however, a comparison of data from the literature with the present model indicates that seepage and not straight through penetration accounts for virtually all penetrating dust. Although insufficient information is presently available to use the model to predict penetration, the model does show trends that should occur with changes in filter operating variables such as filtration velocity and pulse pressure, and suggests areas in which further research is necessary. 相似文献
898.
899.
900.