全文获取类型
收费全文 | 448篇 |
免费 | 4篇 |
国内免费 | 11篇 |
专业分类
安全科学 | 26篇 |
废物处理 | 17篇 |
环保管理 | 94篇 |
综合类 | 51篇 |
基础理论 | 81篇 |
污染及防治 | 123篇 |
评价与监测 | 42篇 |
社会与环境 | 26篇 |
灾害及防治 | 3篇 |
出版年
2023年 | 5篇 |
2022年 | 12篇 |
2021年 | 15篇 |
2020年 | 4篇 |
2018年 | 10篇 |
2017年 | 9篇 |
2016年 | 15篇 |
2015年 | 11篇 |
2014年 | 14篇 |
2013年 | 48篇 |
2012年 | 10篇 |
2011年 | 24篇 |
2010年 | 19篇 |
2009年 | 16篇 |
2008年 | 20篇 |
2007年 | 22篇 |
2006年 | 19篇 |
2005年 | 11篇 |
2004年 | 16篇 |
2003年 | 17篇 |
2002年 | 17篇 |
2001年 | 7篇 |
2000年 | 5篇 |
1999年 | 4篇 |
1998年 | 9篇 |
1997年 | 10篇 |
1996年 | 7篇 |
1995年 | 3篇 |
1993年 | 8篇 |
1992年 | 6篇 |
1991年 | 5篇 |
1990年 | 4篇 |
1989年 | 3篇 |
1987年 | 3篇 |
1986年 | 2篇 |
1985年 | 5篇 |
1984年 | 4篇 |
1983年 | 2篇 |
1982年 | 4篇 |
1981年 | 2篇 |
1979年 | 4篇 |
1978年 | 2篇 |
1975年 | 2篇 |
1973年 | 2篇 |
1964年 | 2篇 |
1963年 | 2篇 |
1958年 | 2篇 |
1957年 | 2篇 |
1956年 | 3篇 |
1955年 | 3篇 |
排序方式: 共有463条查询结果,搜索用时 15 毫秒
21.
Roy E. Bickelhaupt Ralph F. Altman 《Journal of the Air & Waste Management Association (1995)》2013,63(8):831-838
Research has been conducted to develop a technique for predicting the effective volume resistivity of a fly ash layer that has been exposed to circumstances leading to a hot-side precipitator problem known as sodium depletion. Eight fly ashes, representing a major portion of U.S. coals, were evaluated by subjecting 0.5 cm ash layers to a continuously applied voltage gradient of 4 kV/cm for periods of time up to 35 days at a temperature of 350°C (662°F). Resistivity was determined at 350°C before the test started and after the long period of applied voltage used to create the sodium depleted situation. In this condition, resistivity was also determined at 280°C (536°F) for an average electric field Intensity of 4 kV/cm and immediately prior to breakdown. This experimental method can be used with any ash sample to estimate resistivity In a sodium depleted condition. But in addition, a correlation resulting from these resistivity data has been developed. This correlation Is combined with an existing technique for predicting resistivity to produce a method for calculating the expected ash layer resistivity after sodium depletion has occurred. 相似文献
22.
D. Bruce Henschel Roy C. Fortmann Nancy F. Roache Xiaoyu Liu 《Journal of the Air & Waste Management Association (1995)》2013,63(5):708-717
ABSTRACT A laboratory thermal desorption apparatus was used to measure emissions from a number of nominally identical photocopier toners—manufactured to meet the specifications of one specific model copier—when these toners were heated to fuser temperature (180-200 °C). The objective was to assess how potential volatile organic compound (VOC) emissions from the toner for a given copier can vary, depending upon the production run and the supplier. Tests were performed on a series of toner (and associated raw polymer feedstock) samples obtained directly from a toner manufacturer, representing two production runs using a nonvented extrusion process, and on toner cartridges purchased from two local retailers, representing three different production lots (histories unknown). The results showed that the retailer toners consistently had up to 350% higher emissions of some major compounds (expressed as |ig of compound emit-ted/g of toner), and up to 100% lower emissions of others, relative to the manufacturer toners (p ≤ 0.01). The manufacturer toners from one production run had emissions of certain compounds, and of total VOCs, that were modestly higher (13-18%) than those from the other run (p ≤ 0.01). The emission differences between the retailer and manufacturer toners are probably due to differences 相似文献
23.
Source apportionment study of PM10 (Particulate Matter) in a critically polluted area of Jharia coalfield, India has been carried out using Dispersion model, Principle Component Analysis (PCA) and Chemical Mass Balance (CMB) techniques. Dispersion model Atmospheric Dispersion Model (AERMOD) was introduced to simplify the complexity of sources in Jharia coalfield. PCA and CMB analysis indicates that monitoring stations near the mining area were mainly affected by the emission from open coal mining and its associated activities such as coal transportation, loading and unloading of coal. Mine fire emission also contributed a considerable amount of particulate matters in monitoring stations. Locations in the city area were mostly affected by vehicular, Liquid Petroleum Gas (LPG) & Diesel Generator (DG) set emissions, residential, and commercial activities. The experimental data sampling and their analysis could aid understanding how dispersion based model technique along with receptor model based concept can be strategically used for quantitative analysis of Natural and Anthropogenic sources of PM10. 相似文献
24.
Denitrification experiments have provided data showing the pitfalls and successes in developing a sustainable injection/extraction system in a sand and gravel aquifer. Experiments increase in complexity from continuous injection at one well to automated‐pulsed eight well injections. In both continuous and pulsed injection of organic carbon, 40 mg NO3‐N l?1 was reduced below the detection limit of < 0.1 mg NO3‐N l?1 in the denitrification zones. Under continuous injection, accumulation of bacterial exudates in the vicinity of the injection well resulted in injection well clogging within ten days. Periodic cleaning of the injection well and the adjacent gravel matrix was accomplished by using a tool developed to circulate a cleaning solution composed of 5 percent H2O2 and 0.02 percent NaOCl; but, biofouling could not be eliminated. In the later experiments, acetate became the carbon amendment because ethanol promoted more biomass development. A specialized pulse injection procedure was developed to separate nitrate from acetate‐C and was successful in alleviating the proliferation of bacterial exudates without affecting the performance of the denitrification system. Using pulsed injection, a maximum of 72 percent nitrate reduction was accomplished in the extraction well water, and denitrification was sustained for three months without clogging. © 2003 Wiley Periodicals, Inc. 相似文献
25.
Pratt C Walcroft AS Tate KR Ross DJ Roy R Reid MH Veiga PW 《Journal of environmental quality》2012,41(1):80-87
Soil methane (CH(4)) biofilters, containing CH(4)-oxidizing bacteria (methanotrophs), are a promising technology for mitigating greenhouse gas emissions. However, little is known about long-term biofilter performance. In this study, volcanic pumice topsoils (0-10 cm) and subsoils (10-50 cm) were tested for their ability to oxidize a range of CH(4) fluxes over 1 yr. The soils were sampled from an 8-yr-old and a 2-yr-old grassed landfill cover and from a nearby undisturbed pasture away from the influence of CH(4) generated by the decomposing refuse. Methane was passed through the soils in laboratory chambers with fluxes ranging from 0.5 g to 24 g CH(4) m(-3) h(-1). All topsoils efficiently oxidized CH(4). The undisturbed pasture topsoil exhibited the highest removal efficiency (24 g CH(4) m(-3) h(-1)), indicating rapid activation of the methanotroph population to the high CH(4) fluxes. The subsoils were less efficient at oxidizing CH(4) than the topsoils, achieving a maximum rate oxidation rate of 7 g CH(4) m(-3) h(-1). The topsoils exhibited higher porosities; moisture contents; surface areas; and total C, N, and available-P concentrations than the subsoils, suggesting that these characteristics strongly influence growth and activity of the CH(4)-oxidizing bacteria. Soil pH values and available-P levels gradually declined during the trial, indicating a need to monitor chemical parameters closely so that adjustments can be made when necessary. However, other key soil physicochemical parameters (moisture, total C, total N) increased over the course of the trial. This study showed that the selected topsoils were capable of continually sustaining high CH(4) removal rates over 1 yr, which is encouraging for the development of biofilters as a low-maintenance greenhouse gas mitigation technology. 相似文献
26.
The fate and transport processes of a toxic chemical such as atrazine, an herbicide, in a reservoir are significantly influenced
by hydrodynamic regimes of the reservoir. The two-dimensional (2D) laterally-integrated hydrodynamics and mass transport model,
CE-QUAL-W2, was enhanced by incorporating a submodel for toxic contaminants and applied to Saylorville Reservoir, Iowa. The
submodel describes the physical, chemical, and biological processes and predicts unsteady vertical and longitudinal distributions
of a toxic chemical. The simulation results from the enhanced 2D reservoir model were validated by measured temperatures and
atrazine concentrations in the reservoir. Although a strong thermal stratification was not identified from both observed and
predicted water temperatures, the spatial variation of atrazine concentrations was largely affected by seasonal flow circulation
patterns in the reservoir. In particular, the results showed the effect of flow circulation on spatial distribution of atrazine
during summer months as the river flow formed an underflow within the reservoir and resulted in greater concentrations near
the surface of the reservoir. Atrazine concentrations in the reservoir peaked around the end of May and early June. A good
agreement between predicted and observed times and magnitudes of peak concentrations was obtained. The use of time-variable
decay rates of atrazine led to more accurate prediction of atrazine concentrations, while the use of a constant half-life
(60 days) over the entire period resulted in a 40% overestimation of peak concentrations. The results provide a better understanding
of the fate and transport of atrazine in the reservoir and information useful in the development of reservoir operation strategies
with respect to timing, amount, and depth of withdrawal. 相似文献
27.
Becky L. Williams Vanessa Lovenburg Christine L. Huffard Roy L. Caldwell 《Chemoecology》2011,21(3):131-141
Some pelagic marine larvae possess anti-predator chemical defenses. Occasionally, toxic adults imbue their young with their
own defensive cocktails. We examined paralarvae of the greater blue-ringed octopus (Hapalochlaena lunulata) for the deadly neurotoxin tetrodotoxin (TTX), and if present, whether TTX conferred protection to individual paralarvae.
Paralarvae of H. lunulata possessed 150 ± 17 ng TTX each. These paralarvae appeared distasteful to a variety of fish and stomatopod predators, yet
food items spiked with 200 ng TTX were readily consumed by predators. We conclude that TTX alone does not confer individual
protection to paralarvae of H. lunulata, and that they possess an alternative defense. In larger doses, tetrodotoxin is a deterrent to the predatory stomatopod Haptosquilla trispinosa (mean dose = 3.97 μg/g). This corresponds to 12–13 paralarvae per predator based on the TTX levels of the clutch we examined.
Thus, the basic assumption that individual paralarvae of H. lunulata are defended by TTX alone was disproved. Instead, functionality of TTX levels in paralarvae may arise through alternative
selective pathways, such as deterrence to parasites, through kin selection, or against predator species not tested here. 相似文献
28.
Roy Mauldin Edward Kosciuch Fred Eisele Greg Huey David Tanner Steve Sjostedt Don Blake Gao Chen Jim Crawford Douglas Davis 《Atmospheric environment (Oxford, England : 1994)》2010,44(4):572-581
Measurements of OH, H2SO4, and MSA at South Pole (SP) Antarctica were recorded as a part of the 2003 Antarctic Chemistry Investigation (ANTCI 2003). The time period 22 November, 2003–2 January, 2004 provided a unique opportunity to observe atmospheric chemistry at SP under both natural conditions as well as those uniquely defined by a solar eclipse event. Results under natural solar conditions generally confirmed those reported previously in the year 2000. In both years the major chemical driver leading to large scale fluctuations in OH was shifts in the concentration levels of NO. Like in 2000, however, the 2003 observational data were systematically lower than model predictions. This can be interpreted as indicating that the model mechanism is still missing a significant HOx sink reaction(s); or, alternatively, that the OH calibration source may have problems. Still a final possibility could involve the integrity of the OH sampling scheme which involved a fixed building site. As expected, during the peak in the solar eclipse both NO and OH showed large decreases in their respective concentrations. Interestingly, the observational OH profile could only be approximated by the model mechanism upon adding an additional HOx radical source in the form of snow emissions of CH2O and/or H2O2. This would lead one to think that either CH2O and/or H2O2 snow emissions represent a significant HOx radical source under summertime conditions at SP. Observations of H2SO4 and MSA revealed both species to be present at very low concentrations (e.g., 5 × 105 and 1 × 105 molec cm?3, respectively), but similar to those reported in 2000. The first measurements of SO2 at SP demonstrated a close coupling with the oxidation product H2SO4. The observed low concentrations of MSA appear to be counter to the most recent thinking by glacio-chemists who have suggested that the plateau's lower atmosphere should have elevated levels of MSA. We speculate here that the absence of MSA may reflect efficient atmospheric removal mechanisms for this species involving either dynamical and/or chemical processes. 相似文献
29.
Development along the western beachfront of Port Alfred, which is situated along a sandy shoreline, increased markedly in
the 1960s as the coastal town became a popular holiday resort. This development included the removal of coastal vegetation,
which resulted in the destabilization of dunes and migration of sand westerly onto the road, West Beach parking lot, and lawns
of the cabanas. Sand traps were constructed to collect sand blowing across the dunes over set periods, and the net sand movement
along the mobile dune belt was calculated using Hunter's equation. The dunes show an easterly movement of sand at a rate of
3.5 m/yr, which is comparable with figures recorded along other areas of this coastline. Considering the wind regime and amount
of sand movement along this coast, it is inappropriate to clear vegetation and develop within the dune region. 相似文献
30.
Roy Burke James P. Heaney Edwin E. Pyatt 《Journal of the American Water Resources Association》1973,9(3):433-447
ABSTRACT The problem of water resources management can be viewed as one requiring the existence and application of some type of “collective decision” mechanism. Currently, the general water resource decision problem is solved using an “individual decision” format without explicit consideration of the dominant social decision system. This paper demonstrates the need for blending technical planning activities with organized societal processes and then proposes a specific public decision framework to satisfy this requirement. The key element in this planning framework is a generalized “bargaining arena” which serves to link technical activities with the social system. Using this bargaining device we can (1) specify policy at a local level, (2) incorporate “social decision” rules into the planning process, and (3) provide local access to the decision process. A simple case of regional water quality management is used to describe the application of this planning procedure and to offer encouragement for successful use in more complex real-world cases. 相似文献