全文获取类型
收费全文 | 9838篇 |
免费 | 113篇 |
国内免费 | 93篇 |
专业分类
安全科学 | 283篇 |
废物处理 | 459篇 |
环保管理 | 1243篇 |
综合类 | 1193篇 |
基础理论 | 2668篇 |
环境理论 | 2篇 |
污染及防治 | 2773篇 |
评价与监测 | 708篇 |
社会与环境 | 667篇 |
灾害及防治 | 48篇 |
出版年
2022年 | 100篇 |
2021年 | 76篇 |
2020年 | 65篇 |
2019年 | 72篇 |
2018年 | 145篇 |
2017年 | 139篇 |
2016年 | 229篇 |
2015年 | 164篇 |
2014年 | 237篇 |
2013年 | 743篇 |
2012年 | 296篇 |
2011年 | 440篇 |
2010年 | 362篇 |
2009年 | 395篇 |
2008年 | 470篇 |
2007年 | 475篇 |
2006年 | 422篇 |
2005年 | 367篇 |
2004年 | 323篇 |
2003年 | 375篇 |
2002年 | 325篇 |
2001年 | 503篇 |
2000年 | 331篇 |
1999年 | 192篇 |
1998年 | 137篇 |
1997年 | 133篇 |
1996年 | 138篇 |
1995年 | 162篇 |
1994年 | 125篇 |
1993年 | 102篇 |
1992年 | 123篇 |
1991年 | 118篇 |
1990年 | 130篇 |
1989年 | 130篇 |
1988年 | 94篇 |
1987年 | 87篇 |
1986年 | 65篇 |
1985年 | 90篇 |
1984年 | 89篇 |
1983年 | 86篇 |
1982年 | 82篇 |
1981年 | 73篇 |
1980年 | 61篇 |
1979年 | 68篇 |
1977年 | 53篇 |
1976年 | 48篇 |
1975年 | 53篇 |
1974年 | 51篇 |
1973年 | 53篇 |
1970年 | 45篇 |
排序方式: 共有10000条查询结果,搜索用时 10 毫秒
281.
Application of a constructed wetland for industrial wastewater treatment: a pilot-scale study 总被引:9,自引:0,他引:9
The main objective of this study was to examine the efficacy and capacity of using constructed wetlands on industrial pollutant removal. Four parallel pilot-scale modified free water surface (FWS) constructed wetland systems [dimension for each system: 4-m (L)x1-m (W)x1-m (D)] were installed inside an industrial park for conducting the proposed treatability study. The averaged influent contains approximately 170 mg l(-1) chemical oxygen demand (COD), 80 mg l(-1) biochemical oxygen demand (BOD), 90 mg l(-1) suspend solid (SS), and 32 mg l(-1) NH(3)-N. In the plant-selection study, four different wetland plant species including floating plants [Pistia stratiotes L. (P. stratiotes) and Ipomoea aquatica (I. aquatica)] and emergent plants [Phragmites communis L. (P. communis) and Typha orientalis Presl. (T. orientalis)] were evaluated. Results show that only the emergent plant (P. communis) could survive and reproduce with a continuous feed of 0.4m(3)d(-1) of the raw wastewater. Thus, P. communis was used in the subsequent treatment study. Two different control parameters including hydraulic retention time (HRT) (3, 5, and 7d) and media [vesicles ceramic bioballs and small gravels, 1cm in diameter] were examined in the treatment study. Results indicate that the system with a 5-d HRT (feed rate of 0.4m(3)d(-1)) and vesicles ceramic bioballs as the media had the acceptable and optimal pollutant removal efficiency. If operated under conditions of the above parameters, the pilot-plant wetland system can achieve removal of 61% COD, 89% BOD, 81% SS, 35% TP, and 56% NH(3)-N. The treated wastewater meets the current industrial wastewater discharge standards in Taiwan. 相似文献
282.
Eshleman KN Wigington PJ Davies TD Tranter M 《Environmental pollution (Barking, Essex : 1987)》1992,77(2-3):287-295
Field studies of chemical changes in surface waters associated with rainfall and snowmelt events have provided evidence of episodic acidification of lakes and streams in Europe and North America. Modelling these chemical changes is particularly challenging because of the variability associated with hydrological transport and chemical transformation processes in catchments. This paper provides a review of mathematical models that have been applied to the problem of episodic acidification. Several empirical approaches, including regression models, mixing models and time series models, support a strong hydrological interpretation of episodic acidification. Regional application of several models has suggested that acidic episodes (in which the acid neutralizing capacity becomes negative) are relatively common in surface waters in several regions of the US that receive acid deposition. Results from physically based models have suggested a lack of understanding of hydrological flowpaths, hydraulic residence times and biogeochemical reactions, particularly those involving aluminum. The ability to better predict episodic chemical responses of surface waters is thus dependent upon elucidation of these and other physical and chemical processes. 相似文献
283.
Bioavailability of persistent organic pollutants in soils and sediments--a perspective on mechanisms, consequences and assessment 总被引:27,自引:0,他引:27
It has been observed that as soil-pollutant contact time increases, pollutant bioavailability and extractability decreases. This phenomenon has been termed 'ageing'. Decreased chemical extractability with increased soil-chemical contact time is evident where both 'harsh' techniques, e.g. dichloromethane Soxhlet extraction, and 'non-exhaustive' techniques, e.g. butanol shake extraction, have been used. It has also been observed that the amount of chemical extracted by these techniques varies considerably over time. Similarly, decreases in bioavailability with increased soil-pollutant contact time have been described in bacterial, earthworm and other organism studies. From these investigations, it has been shown that the fraction of pollutant determined to be bioavailable can vary between organisms. Thus, there is an immediate definition problem, what is bioavailability? Additionally, if bioavailability is to be assessed by a chemical means, which organisms should (or can) be mimicked by the extraction procedure? This review provides a background to the processes inherent to ageing, a discussion of its consequences on bioavailability and ends with some reflections on the appropriateness of chemical extraction techniques to mimic bioavailability 相似文献
284.
285.
Exposure to secondary metabolites of airborne fungi in waste handling facilities is discussed in regard to potential toxic impacts on human health. The relevance of mycotoxins has been intensely studied in connection with contamination of food and feed. Toxic secondary metabolites are expected to be present in airborne spores, but exposure to mycotoxins in bioaerosols has not been studied sufficiently. Aspergillus fumigatus is one of the most frequent species in the air of compost plants. A wide range of secondary metabolites was found in pure cultures of freshly isolated strains of A. fumigatus. Tryptoquivaline, a compound with tremorgenic properties, and trypacidin, for which no toxic properties are described, were found in native bioaerosols in a compost facility. The highly toxic metabolites gliotoxin and verruculogen were not found in the bioaerosols. 相似文献
286.
287.
Benkó Tímea Lukács Dávid Li Mingtao Pap József S. 《Environmental Chemistry Letters》2022,20(6):3657-3695
Environmental Chemistry Letters - Given the rising socioeconomic issues of fossil fuels, efficient artificial photosynthesis would be an important milestone toward a sustainable world. A key step... 相似文献
288.
Geostatistical analyses and hazard assessment on soil lead in Silvermines area, Ireland 总被引:42,自引:0,他引:42
Spatial distribution and hazard assessment of soil lead in the mining site of Silvermines, Ireland, were investigated using statistics, geostatistics and geographic information system (GIS) techniques. Positively skewed distribution and possible outlying values of Pb and other heavy metals were observed. Box-Cox transformation was applied in order to achieve normality in the data set and to reduce the effect of outliers. Geostatistical analyses were carried out, including calculation of experimental variograms and model fitting. The ordinary point kriging estimates of Pb concentration were mapped. Kriging standard deviations were regarded as the standard deviations of the interpolated pixel values, and a second map was produced, that quantified the probability of Pb concentration higher than a threshold value of 1000 mg/kg. These maps provide valuable information for hazard assessment and for decision support. 相似文献
289.
Photocatalytic oxidation of triclosan 总被引:1,自引:0,他引:1
In the spring of 2003, there was an outbreak of the severe respiratory syndrome (SARS) in Hong Kong. Health concerns have thus triggered an increased and predominant use of various types of household cleansing agents such as triclosan (5-chloro-2-(2,4-dichlorophenoxy)phenol). However, it has been reported recently that triclosan could be photochemically converted to toxic 2,8-dichlorodibenzo-p-dioxin (2,8-Cl(2)DD) in the environment. It is therefore necessary to develop environmentally friendly methods for the treatment of triclosan. To this end, photocatalytic degradation of triclosan in aqueous solution was conducted using TiO(2) (Degussa P25) under irradiation of UV light (lambda < 365 nm). It was found that triclosan could be degraded by this approach. Hydrogen peroxide was added to enhance the degradation process, and the optimal initial hydrogen peroxide concentration for triclosan degradation was 0.005% (w/v). Product identification indicated that triclosan oxidation occurred at its phenol moiety and yielded quinone and hydroquinone intermediates. The formation of a dichlorophenol intermediate in triclosan degradation suggested bond-breaking of the ether linkage occurred during the process. Moreover, no chlorinated dibenzo-p-dioxin congener was detected. These findings confirm that the photocatalytic degradation of triclosan is an environmentally friendly process. 相似文献
290.
Tong HY Hung WT Cheung CS 《Journal of the Air & Waste Management Association (1995)》2000,50(4):543-554
This paper reports on the analysis of on-road vehicle speed, emission, and fuel consumption data collected by four instrumented vehicles. Time-, distance-, and fuel-based average fuel consumption, as well as CO, HC, NOx, and soot emission factors, were derived. The influences of instantaneous vehicle speed on emissions and fuel consumption were studied. It was found that the fuel-based emission factors varied much less than the time- and distance-based emission factors as instantaneous speed changed. The trends are similar to the results obtained from laboratory tests. The low driving speed contributed to a significant portion of the total emissions over a trip. Furthermore, the on-road data were analyzed using the modal approach. The four standard driving modes are acceleration, cruising, deceleration, and idling. It was found that the transient driving modes (i.e., acceleration and deceleration) were more polluting than the steady-speed driving modes (i.e., cruising and idling) in terms of g/km and g/sec. These results indicated that the on-road emission measurement is feasible in deriving vehicle emissions and fuel consumption factors in urban driving conditions. 相似文献