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461.
Mingjie Zhang Gang Yang Shuai Liu Jiahui Yu Hongzhe Li Liwen Zhang Yipei Chen Ruitang Guo Tao Wu 《环境科学学报(英文版)》2022,34(6):163-174
Due to the ever-tightening regulation on mercury emission in recent decades, there is an urgent need to develop novel materials for the removal of elemental mercury at coal-fired power plants. In this study, a series of MoS2 quantum dots (QDs)-based MoS2/HKUST-1 composite materials were prepared. It is found that MoS2 QDs were encapsulated by HKUST-1 and enhanced the crystallinity and specific surface area of HKUST-1. The MoS2/HKUST-1 showed excellent performance in catalytic oxidation of Hg0 as compared with pristine HKUST-1. It is found that surface layer of lattice oxygens is active and participates in Hg0 oxidation, while the consumption of surface oxygens then leads to the formation of oxygen vacancies on the surface. These vacancies are effective in the adsorption and dissociation of O2, which subsequently participates in the oxidation of Hg0. Moreover, the study on the influence of commonly seen gas components, such as SO2, NO, NH3 and H2O, etc., on Hg0 oxidation demonstrated that synergistic effects exist among these gas species. It is found that the presence of NO promotes the oxidation of Hg0 using oxygen as the oxidant. 相似文献
462.
External organic carbon sources are needed to provide electron donors for the denitrification of wastewater with a low COD/NO3--N(C/N) ratio, increasing the treatment cost. The economic strategy is to enhance the bioactivity and/or biodiversity of denitrifiers to efficiently utilize organic substances in wastewater. In this study, novel zero-valent iron(ZVI) composite carriers were prepared and implemented in a suspended carrier biofilm reactor to enhance the bioactivity an... 相似文献
463.
为研究枯水期巢湖水体悬浮颗粒物(SPM)营养元素组成及其潜在环境效应,分析了2020年1月巢湖18个采样点表层水体SPM含量、颗粒有机质(SPOM)含量及氮磷组成,并利用颗粒有机碳、氮同位素组成及C/N研究了冬季巢湖SPOM的来源及其空间变化. 结果表明,悬浮颗粒物总磷(PP)浓度为0.032~0.065 mg/L,平均值为0.049 mg/L;悬浮颗粒物无机磷(PIP)浓度为0.018~0.046 mg/L,平均值为0.032 mg/L,是PP的主要组分,二者浓度均呈西湖区>东湖区>中湖区的空间分布特征. 悬浮颗粒物总氮(PN)浓度为0.254~0.424 mg/L,平均值为0.342 mg/L,其中悬浮颗粒物有机氮(PON)占比较高,表明颗粒态氮以湖泊内源性有机来源为主. 巢湖表层水体SPOM的δ13C范围在?28.72‰~?26.68‰之间,δ15N为3.34‰~9.97‰,C/N为2.51±0.95,指示冬季枯水期水体SPOM主要来自内源水生生物碎屑,而陆源径流输入对湖泊颗粒物影响较小. 研究显示:冬季巢湖悬浮颗粒有机质主要来自湖泊内源,具有潜在的营养盐效应,污染控制需要相应的策略. 相似文献
464.
近年来,渤、黄海海域呈现溶解氧浓度降低并导致季节性低氧的特征,对海洋生态环境形成潜在危害。在此背景下,本文基于2011年6月(低氧形成期)和2011年11-12月初(低氧消亡期)在渤、黄海的观测数据,通过分析水体表观耗氧量(AOU)、pH、溶解无机碳(DIC)及营养盐之间的相关关系,探讨了生源要素在低氧形成期与消亡期的变化特征及主要控制机制。结果表明,生物的光合作用与有机物的降解过程是调控低氧事件前后渤海生源要素变化的主要因素之一,而黄海底层水体有机物的降解过程是调控水体溶解氧浓度及营养盐浓度变化的主要原因之一。 相似文献
465.
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467.
本文分析了我国当前水污染区域治理的难度,沿海地区水污染的主要问题,探讨了污染区域治理的基本原则,提出了水污染治理的重点区域和水污染区域治理的主要途径,并以浑河流域沈阳地区2000年水污染物总量控制为例,概述总量控制方法和目标 相似文献
468.
陶战 《中国人口.资源与环境》1994,4(1):62-64
中国农业经历了多种策略阶段,可持续发展策略是新近出现的最先进、最适合现在和将来农业发展的策略。新策略带有系统性原理,其实质是发展与生态环境保护协调的农业。因此,可持续发展措施应同时重视解决农业经济发展与生态环境保护两方面的问题。据此,本文提出了六项措施。 相似文献
469.
Daily Bank Erosion Rates in the Lower Yellow River Before and After Dam Construction 总被引:1,自引:0,他引:1
Junqiang Xia Tao Li Xiaojuan Li Xiaolei Zhang Quanli Zong 《Journal of the American Water Resources Association》2014,50(5):1325-1337
During the period of water impoundment and sediment detention of the Sanmenxia Reservoir, riverbank erosion processes played a key role in the channel evolution of the Lower Yellow River (LYR). However, research into bank erosion rates of the LYR has been neglected due to the lack of direct field monitoring. In this study, an indirect method is proposed to determine bank erosion rates at daily time scales by outlining a detailed calculation procedure using measured hydrological data. A total of 810 data points of daily bank erosion rates before and after the construction of Sanmenxia Dam was calculated at seven hydrometric sections along the LYR, with the corresponding values of the bank stability coefficient and the width‐to‐depth ratio also being calculated. Empirical relations were then developed to estimate the daily bank erosion rates, using these parameters at the sections. Temporal and spatial variability in daily bank erosion rates in the LYR before and after dam construction were also investigated, revealing that: (1) the bank erosion rates had a mean value of 16.7‐29.1 m/day in the braided reach, with a maximum value of 290.0 m/day, while they were relatively low in the meandering reach, with a mean value of 2.5 m/day; (2) the erosion rates before dam construction were slightly greater than those after dam construction, with the difference reaching 5‐10 m/day in the braided reach, decreasing in the transitional reach gradually, and being slight in the meandering reach. 相似文献
470.