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41.
Theodora Adamopoulou Maria I. Papadaki Manolis Kounalakis Victor Carreto Alba Pineda M. Sam Mannan 《Journal of Loss Prevention in the Process Industries》2012,25(5):803-808
Hydroxylamine, NH2OH, thermal decomposition has been responsible for two serious accidents. However, its reactive behavior and the synergy of factors affecting the rate of its decomposition are not understood. In this work, isoperibolic calorimetric measurements were performed in a metal reactor, in the temperature range 130–150 °C, employing 30–80 ml solutions containing 1.4–20 g of pure hydroxylamine (2.8–40 g of the supplied reagent). The calorimetric measurements were performed in order to assess the effects that NH2OH concentration, temperature and reactor venting has on NH2OH rate of decomposition. The measurements showed that increased concentration or temperature, results in faster reactions and probably higher pressure generation per mass of reactant, with concentration having a more pronounced effect. However, when both factors work synergistically the result is dramatically worse in terms of reaction rate. The pressure generation is also different, thus indicating that different reaction pathways predominate each time. Venting the produced gases in stages resulted in the highest mass loss of the solution. 相似文献
42.
Alfred J. Vella Bernardette Mintoff Victor Axiak Dorita Agius Roberto Cassone 《毒物与环境化学》2013,95(3-4):491-510
The speciation of organotins in seawater, surface microlayer and sediments in the marine environment of Malta is described. Concentrations of tributyltin (TBT) in bulk seawater inside the harbours were as high as 0.3 μg Sn L‐1 but were below detection limits (5 ng Sn L‐1) in open sea, 1.6 km offshore. In sediments, TBT levels were highest for the yacht marinas and ranged between 0.03 and 1.5 ug Sn g‐1. Dibutyltin is more common in the surface microlayer than TBT. Diphenyl and monophenyltin were found infrequently in bulk seawater and in sediments. Tetrasubstituted organotins, namely, MenBu(4_n)Sn, where n = 1, 2, and 3, were found frequently in TBT‐contaminated sediments (0.1–9μg Sng‐1), in seawater and in the microlayer where concentrations as high as 140 μg Sn L‐1 (Me3BuSn) were measured. Direct environmental methylation of TBT and that of its debutylated analogues may play a significant role in the geochemical cycling of tin under certain environmental conditions. 相似文献
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Tov Elperin Nathan Kleeorin Michael A. Liberman Victor S. L’vov Igor Rogachevskii 《Environmental Fluid Mechanics》2007,7(2):173-193
A mechanism of formation of small-scale inhomogeneities in spatial distributions of aerosols and droplets associated with
clustering instability in the atmospheric turbulent flow is discussed. The particle clustering is a consequence of a spontaneous
breakdown of their homogeneous space distribution due to the clustering instability, and is caused by a combined effect of
the particle inertia and a finite correlation time of the turbulent velocity field. In this paper a theoretical approach proposed
in Elperin et al. (2002) Phys Rev E 66:036302 is further developed and applied to investigate the mechanisms of formation
of small-scale aerosol inhomogeneities in the atmospheric turbulent flow. The theory of the particle clustering instability
is extended to the case when the particle Stokes time is larger than the Kolmogorov time scale, but is much smaller than the
correlation time at the integral scale of turbulence. We determined the criterion of the clustering instability for the Stokes
number larger than 1. We discussed applications of the analyzed effects to the dynamics of aerosols and droplets in the atmospheric
turbulent flow. 相似文献
46.
Malanichev A Mantseva E Shatalov V Strukov B Vulykh N 《Environmental pollution (Barking, Essex : 1987)》2004,128(1-2):279-289
The numerical evaluation of selected PCB congener (28, 118, 153, 180) transport over the Northern Hemisphere is carried out for 1996 using MSCE-POP model. This model is a multicompartment three-dimensional one and includes various environmental media such as the atmosphere, soil, vegetation, seawater, and sea ice. The spatial resolution is 2.5 degrees x2.5 degrees for all media except marine one (1.25 degrees x1.25 degrees ). The main model output information is deposition fluxes, spatial distribution of concentrations in environmental media, pathways and source-receptor relationships. Calculation results are analysed for the whole hemisphere and the Arctic region. In particular, this gives an opportunity to estimate the contributions of individual emission source groups to the Arctic pollution. The reliability of the model assessment is analysed by comparison between calculated and observed data. 相似文献
47.
Accumulation of two heavy metals (Al and Fe) by bryophytes was examined in a northern Pennsylvania stream system affected by acid-mine drainage. Four sites within one watershed were selected on the basis of their pH and dissolved metal concentrations. Significant differences among sites were found with regard to bioaccumulation of Al and Fe. A negative relationship between pH and Fe concentrations in bryophyte tissues was found, with the highest accumulation of Fe observed at the most acidic site (pH 3.5), whereas accumulation of Al was highest at a site with an intermediate pH of 5.2. Bryophytes transplanted from a circum-neutral site to acidic sites showed highly significant increases in Fe and Al concentrations in tissues after 6 weeks, and transplants from more acidic sites to a circum-neutral site generally showed highly significant declines in Fe and Al concentrations in tissues after the incubation period. 相似文献
48.
Cheuk W Lo KV Copeman R Joliffe P Fraser BS 《Journal of environmental science and health. Part. B》2005,40(3):449-461
This study investigated the disease suppression abilities of a compost amendment that was added to the conventional growing medium, yellow cedar sawdust, used in most British Columbia vegetable greenhouses. The compost amendment was produced in a controlled, in-vessel process primarily from greenhouse crop waste materials. The pathogen and cultivar under study were Fusarium oxysporum f. sp. radicis-lycopersici (FORL) on Dombito (FORL-susceptible) beefsteak greenhouse tomatoes. Significant reduction of Fusarium crown and root rot was also realized in tomato seedlings by applying compost amendment from several different batches, as a seed cover or plug substitute. In a greenhouse trial, disease suppression using a mixture of 2:1 sawdust to amendment by volume was shown to be most effective. As a result, the tomato yield over a nine-month growing season was improved by 74% where the medium was deliberately infested with FORL. 相似文献
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