This study investigated the characteristics of iron corrosion scales in pipes at tube well, overhead tank, and consumers’ end in older untreated water distribution system in Peshawar city, Pakistan. Effect of water quality conditions on corrosion scales and that of scales on drinking water quality in such systems was also assessed by undertaking a comparison with new piped distribution systems. The scales were analyzed for chemical composition and morphology using X-ray diffraction (XRD), inductively coupled plasma (ICP), and a scanning electron microscope (SEM), while water quality was examined for physicochemical and biological characteristics. The main crystalline phases of corrosion scales were goethite, magnetite, siderite, and quartz. From tube well to consumers’ end, goethite increased from 36 up to 48%, quartz declined from 22 to 15%, while magnetite fluctuated and siderite disappeared. Elemental composition of scales showed the deposition of Zn, Al, Mn, Cr, Pb, Cu, As, and Cd with Zn (13.9 g/kg) and Al (3.6 g/kg) in highest proportion. The SEM analysis illustrated the presence of microbial communities indicating the formation of biofilms in the corrosion scales. The significant difference (P <?0.05) in levels of dissolved oxygen (DO), Cl?, SiO44?, electrical conductivity (EC), SO42?, NO3?, alkalinity, hardness, and trace metals between old (DS-O) and new piped systems indicated their role in corrosion scale formation/destabilization and the effect of scale dissolution on water quality. In DS-O, EC, Cu, and Mn were significantly higher (P?<?0.05), whereas turbidity, EC, DO, and SiO44? significantly increased from source to consumers’ end implying a higher dissolution of scales and lowered corrosion rates in DS-O to utilize SiO44? and DO for iron oxidation.
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2H-1,4-Benzoxazines are major heterocyclic compounds with interesting biological and synthetic applications. Therefore, it would be very interesting to develop new efficient methods for their synthesis. Here, we synthesized 2H-1,4-benzoxazines in one pot using K2CO3/H2O in the ionic liquid of choice, [omim][BF4]. After reactions, products are extracted from [omim][BF4] by Et2O and the ionic liquid is recovered and successfully reused over several recycles. Results show that high yields of 3-aryl-2H-1,4-benzoxazine derivatives are obtained chemoselectively at room temperature from their corresponding o-aminophenols and phenacyl bromides. To our knowledge, our method represents the most efficient and straightforward route for the synthesis of 3-aryl-2H-1,4-benzoxazine derivatives in short times and under environmentally benign conditions. 相似文献
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The purpose of the study is to predict drought changes in Dariun, Fars Province, and their impact on water and soil quality. To prepare drought, water, and soil quality zoning maps, Landsat satellite images and the kriging method were used. The fuzzy maps and weights for each parameter were then determined using fuzzy and analytic hierarchy process (AHP) methods. Additionally, cellular automata (CA)-Markov chains were used in order to predict the impact of drought changes on water and soil quality. Using the fuzzy-AHP method, water quality and soil fertility in 2020 were lower compared to previous years, mainly because of land use changes that increased pollution. Based on results of the Markov and CA-Markov chains, approximately 31% of the region will have very poor levels of soil fertility and water quality in 2050. Further, based on remote sensing indicators, it is determined that about 25% of the region will be at high risk of drought in 2050. Thus, if adequate management of the region is not done, the possibility of living in these areas may diminish in the coming years due to drought and deteriorated water and soil quality.
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