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971.
Guan-yong Su Zi-shen Gao Yijun Yu Jia-chun Ge Si Wei Jian-fang Feng Feng-yan Liu John P. Giesy Hong-xia Yu 《Environmental science and pollution research international》2010,17(3):634-642
Background, aim, and scope
Polybrominated diphenyl ethers (PBDEs) and their metabolites are toxic to animals, and concentrations of the PBDEs metabolites can exceed those of the parent materials. But no information was available on concentrations of PBDEs metabolites in the lower Yangtze River in the region around Jiangsu Province of China, which is heavily urbanized and industrialized area. The aims of this study were to determine whether PBDEs and their methoxylated PBDEs (MeO-PBDEs) were accumulated in Coilia sp. in this area and to investigate the potential sources for these two kinds of brominated organic pollutants. 相似文献972.
不同模糊评价方法在水环境质量评价中的应用比较 总被引:7,自引:0,他引:7
近年来,运用模糊评价方法对水质和水体营养化程度进行评价逐渐受到重视。目前,对模糊评价方法的研究多集中在实测数据标准化、权重的确定和模糊模式识别模型研究几个方面。以滇池历年营养物质数据为实测数据,通过对几种实测数据标准化方法、权重确定方法和模糊模式识别方法的组合应用,获得水环境质量模糊评价最优组合方法。结果表明,在评价方法中,实测数据标准化方法采用线性内插法,权重的确定采用超标倍数法,模糊模式识别模型采用广义海明距离和加权海明距离法,即采用超标倍数法的广义海明距离和加权海明距离法能够更真实反映水环境质量的实际情况。 相似文献
973.
维生素和酮苷生产废水中难降解污染物的溯源研究 总被引:2,自引:1,他引:1
研究了维生素和酮苷生产过程中各生产工段排水的生物降解特性,评价了各生产工段对生产废水中难降解有机物的贡献率,追溯了可能的难降解特征污染物。结果表明,维生素生产废水中的难降解物质主要来自W1-1、W1-3、W1-5和W1-6生产工段,甲醛、丁烯酮、醛酮聚合物和吡啶可能是导致生产废水难降解的重要原因;酮苷生产废水中的难降解物质主要来自W2-1、W2-3和W2-7生产工段,氯代有机溶剂和苯环类物质可能是导致生产废水难降解的重要原因。建议根据具体生产工段排水的水质特征,有针对性地进行物化处理,提高废水可生化性。 相似文献
974.
Xueyuan Wang Xin-Zhong Liang Weimei Jiang Zhining Tao Julian X.L. Wang Hongnian Liu Zhiwei Han Shuyan Liu Yuyan Zhang Georg A. Grell Steven E. Peckham 《Atmospheric environment (Oxford, England : 1994)》2010,44(5):660-669
This study develops fine temporal (seasonal, day-of-week, diurnal) and vertical allocations of anthropogenic emissions for the TRACE-P inventory and evaluates their impacts on the East Asian air quality prediction using WRF-Chem simulations in July 2001 at 30-km grid spacing against available surface measurements from EANET and NEMCC. For NO2 and SO2, the diurnal and vertical redistributions of emissions play essential roles, while the day-of-week variation is less important. When all incorporated, WRF-Chem best simulates observations of surface NO2 and SO2 concentrations, while using the default emissions produces the worst result. The sensitivity is especially large over major cities and industrial areas, where surface NO2 and SO2 concentrations are reduced by respectively 3–7 and 6–12 ppbv when using the scaled emissions. The incorporation of all the three redistributions of emissions simulates surface O3 concentrations higher by 4–8 ppbv at night and 2–4 ppbv in daytime over broad areas of northern, eastern and central China. To this sensitivity, the diurnal redistribution contributes more than the other two. 相似文献
975.
Chuan-Yao Lin C.-C. Chang C.Y. Chan C.H. Kuo W.-C. Chen D. Allen Chu Shaw C. Liu 《Atmospheric environment (Oxford, England : 1994)》2010,44(2):182-193
To quantify the possible sources of the high ambient ozone concentration in the low troposphere over Taiwan, ozone sounding data from a two-year intensive field measurement program conducted in April and early May of 2004 and 2005 in northern Taiwan has been examined. We found that the vertical ozone distributions and occurrence of enhanced ozone in the lower troposphere (below 6 km) mainly resulted from (1)Type NE: the long-range transport of ozone controlled by the prevailing northeasterly winds below 2 km, (2)Type LO: the local photochemical ozone production process, and (3)Type SW: the strong southwest/westerly winds aloft (2–6 km). In the boundary layer (BL), where Asian continental outflow prevails, the average profile for type NE is characterized by a peak ozone concentration of nearly 65 ppb at about 1500 m altitude. For type LO, high ozone concentration with an average ozone concentration greater than 80 ppb was also found in the BL in the case of stagnant atmospheric and sunny weather conditions dominated. For type SW, significant ozone enhancement with average ozone concentration of 70–85 ppb was found at around 4 km altitude. It is about 10 ppb greater than that of the types NE and LO at the same troposphere layer owing to the contribution of the biomass burning over Indochina. Due to Taiwan's unique geographic location, the complex interaction of these ozone features in the BL and aloft, especially features associated with northeasterly and south/southwesterly winds, have resulted in complex characteristics of ozone distributions in the lower troposphere over northern Taiwan. 相似文献
976.
Renbin Zhu Yashu Liu Hua Xu Tao Huang Jianjun Sun Erdeng Ma Liguang Sun 《Atmospheric environment (Oxford, England : 1994)》2010,44(3):304-311
During the summertime of 2007/2008, carbon dioxide (CO2) and methane (CH4) fluxes across air–water interface were investigated in the littoral zones of Lake Mochou and Lake Tuanjie, east Antarctica, using a static chamber technique. The mean fluxes of CO2 and CH4 were ?70.8 mgCO2 m?2 h?1 and 144.6 μgCH4 m?2 h?1, respectively, in the littoral zone of Lake Mochou; The mean fluxes were ?36.9 mgCO2 m?2 h?1 and 109.8 μgCH4 m?2 h?1, respectively, in the littoral zone of Lake Tuanjie. Their fluxes showed large temporal and spatial dynamics. The CO2 fluxes showed a significantly negative correlation with daily total radiation (DTR) and a weakly negative correlation with air temperature and water temperature, indicating that sunlight intensity controlled the magnitude of CO2 fluxes from the open lakes. The CH4 fluxes significantly correlated with local air temperature, water table and total dissolved solids (TDS), indicating that they were the predominant factors influencing CH4 fluxes. Summertime CO2 budgets in the littoral zones of Lake Mochou and Lake Tuanjie were estimated to be ?152.9 gCO2 m?2 and ?79.7 gCO2 m?2, respectively, and net CH4 emissions were estimated to be 312.3 mgCH4 m?2 and 237.2 mgCH4 m?2, respectively. Our results show that shallow, open, alga-rich lakes might be strong summertime CO2 absorbers and small CH4 emitters during the open water in coastal Antarctica. 相似文献
977.
X.X. Zhang P.J. Shi L.Y. Liu Y. Tang H.W. Cao X.N. Zhang X. Hu L.L. Guo Y.L. Lue Z.Q. Qu Z.J. Jia Y.Y. Yang 《Atmospheric environment (Oxford, England : 1994)》2010,44(13):1641-1648
Based on environmental monitoring data in 93 major cities and meteorological records at 398 weather stations in China from 1981 to 2007, total suspended particle (TSP) concentration, the intensity of dustfall, and sand and dust storm frequency (Fd) were analysed. During the past 27 years, the annual average TSP concentration (CTSP) in 93 cities was 402 μg m?3. Annual average CTSP decreased from the north to the south and from inland to the coast areas with a peak value of 628.8 μg m?3 in Lanzhou. In the 1980s, 1990s and 2000s, annual average CTSP was 628.7, 319.2, and 250.1 μg m?3, respectively. Annual average intensity of dustfall (Id) was 240.5 t km?2 a?1, decreased from northern to southern China and from inland to the coast areas with the maximum value of 717.2 t km?2 a?1 in Baotou. In the 1980s, 1990s and 2000s, annual average Id was 334.8, 220.9, 146 t km?2 a?1 respectively. Annual average Id in the Loess Plateau region was commonly higher than 200 t km?2 a?1. The annual average Fd decreased from arid regions in northwestern China to humid areas in southeastern China with two sand and sand storm centers existing in Xinjiang Taklamakan Desert and western Inner Mongolia. The annual average Fd in the 1980s, 1990s, 2000s was 16, 8, 6 days respectively, decreased steadily from 18 days in 1981–5 days in 2007. Annual average Id had a positive linear relation to annual average CTSP (R2 = 0.96). Annual average Fd had a positive relation with annual average CTSP (R2 = 0.97) as well as annual average Id (R2 = 0.94). TSP was the chief pollutant influencing Air Pollution Index (API) in northern China in spring and winter seasons. Sand and dust storm might be a major factor affecting the temporal variability and spatial distribution of TSP and dustfall in China. 相似文献
978.
979.
Beilei Lei Yimeng Ma Jiazhong Li Huanxiang Liu Xiaojun Yao Paola Gramatica 《Atmospheric environment (Oxford, England : 1994)》2010,44(25):2954-2960
Accurate quantitative structure–property relationship (QSPR) models based on a large data set containing a total of 3483 organic compounds were developed to predict chemicals’ adsorption capability onto activated carbon in gas phrase. Both global multiple linear regression (MLR) method and local lazy regression (LLR) method were used to develop QSPR models. The results proved that LLR has prediction accuracy 10% higher than that of MLR model. By applying LLR method we can predict the test set (787 compounds) with Q2ext of 0.900 and root mean square error (RMSE) of 0.129. The accurate model based on this large data set could be useful to predict adsorption property of new compounds since such model covers a highly diverse structural space. 相似文献
980.
David Widory Xiande Liu Shuping Dong 《Atmospheric environment (Oxford, England : 1994)》2010,44(30):3679-3687
Even after its being phased out in gasoline in the late 90s, lead (Pb) is still present at relatively high levels in the atmosphere of Beijing, China (0.10–0.18 μg m?3). Its origin is subject to debate as several distinct sources may contribute to the observed pollution levels. This study proposes to constrain the origin(s) of Pb and strontium (Sr) in aerosols, by coupling both Pb and Sr isotope systematics. The characterisation of the main pollution sources (road traffic, smelters, metal refining plants, coal combustion, cement factories, and soil erosion) shows that they can unambiguously be discriminated by the multi-isotope approach (206Pb/204Pb and 87Sr/86Sr). The study of total suspended particulates (TSP) and fine particles (PM2.5) from Beijing and its vicinity indicates that both size fractions are controlled by the same sources. Lead isotopes indicate that metal refining plants are the major source of atmospheric lead, followed by thermal power stations and other coal combustion processes. The role of this latter source is confirmed by the study of strontium isotopes. Occasionally, emissions from cement plants and/or input from soil alteration are isotopically detectable. 相似文献