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91.
Removing nitric oxide from flue gas using iron(II) citrate chelate absorption with microbial regeneration 总被引:1,自引:0,他引:1
The addition of metal chelates such as Fe(II)EDTA or Fe(II)Cit to wet flue gas desulfurization systems has been shown to increase the amount of NO(x) absorption from gas streams containing SO(2). This paper attempts to demonstrate the advantage of not only using Fe(II)Cit chelate to absorb nitrogen oxides from flue gas but also the advantage gained from adding microorganisms to the system. Two distinct classes of microorganisms are needed: denitrifying and iron-reducing bacteria. The presence of oxygen in flue gas will affect the absorption efficiency of NO by Fe(II)Cit chelate. The oxidation of Fe(II) can be slowed with the help of bacteria in two ways: bacteria can serve to directly reduce Fe(III) to Fe(II) or they can serve to keep levels of dissolved oxygen in the solution low. As a result, after NO absorption, Fe(II)(Cit)NO will be reduced by denitrifying bacteria to Fe(II)Cit while Fe(III) is reduced by anaerobic bacteria back to Fe(II). Our experiments have shown that the implementation of our protocol allowed for an NO reduction rate constant increase from standard levels of 0.0222-0.100 m Mh(-1) with inlet NO changed from 250 to 1000 ppm. We have also found that total Fe concentration tends to decrease after prolonged periods of operation due to the loss of some Fe to the formation of Fe(OH)(3) that settles together with the sludge at the bottom of bioreactor tank. 相似文献
92.
Huang WJ Lin TP Chen JS Shih FH 《Journal of environmental biology / Academy of Environmental Biology, India》2011,32(3):301-307
Cyanobacteria were inactivated by using zinc oxide (ZnO)coated on the surface of gamma-AI2O3 as a photocatalyst and combining with sunlight. In vitro experiments indicate that axenic cultures of planktonic cyanobacteria lost their photosynthetic activity after photocatalyzed with sunlight exposure exceeding 24 hr. As for Oscillatoria tenuisa, nearly 92% of the cells lost their photosynthetic activity and the cell morphology was severely damaged during 24 hr of the reaction. However, in the case of Microcystis aeruginosa, lower photocatalytic inactivity efficiency was observed, which was attributed to extracellular polymeric secretions (EPSs) surrounding the cells. With a high dosage ZnO catalyst, the dissolved organic carbon (DOC) concentration of the Oscillatoria tenuisa suspension was increased by up to about 190% during photocatalysis. The increased suspension of DOC was attributed to increase liberation of extracellular organic and cell-wall polysaccharides during photocatalysis. 相似文献
93.
Yu-Ling Chen Yi-Hsuan Shih Chao-Heng Tseng Sy-Yuan Kang Huang-Chin Wang 《Mitigation and Adaptation Strategies for Global Change》2013,18(8):1125-1139
This study examines the monetary value of social costs—private costs and negative externalities—that could be avoided by energy conservation actions. A novel Air Resource Co-Benefits (ARCoB) model has been developed in this study to assess the comprehensive social benefits of greenhouse gas GHG mitigation policy. The rollback model is used to estimate changes in air pollutant concentrations attributed to the emission reductions. Change in ozone concentration is converted from non-methane hydrocarbons based on the maximum ozone increment reactivity. In addition to saved medical expenditure, years of potential life lost (YPLL) is estimated based on the exposure-response coefficients for mortality and is calculated with abridged life table. Two cases of energy efficiency improvement in different scales are analyzed to estimate the annual co-benefits of abatements of air pollutants and greenhouse gas in 2009: 1) the energy intensity reduction in the industrial sector and 2) energy saving at Taipei Taiwan City Hall. Results indicate the saved energy cost accounted for 66 % and 70 % in the first and second case, respectively, and was a major part of the total benefit from energy conservation. The saved air pollution fee was 7.8–8.5 times lower than the averted health cost of medical expenditure, which was US$10.34 million in the first case, in which there were also averted YPLL of 3,478 person-years or averted deaths of 311 persons per year. 相似文献
94.
The cyanobacteria-bloom in raw waters frequently causes an unpredictable chemical dosing of preoxidation and coagulation for an effective removal of algal cells in water treatment plants. This study investigated the effects of preoxidation with NaOCl and ClO_2 on the coagulation-flotation effectiveness in the removal of two commonly blooming cyanobacteria species, Microcystis aeruginosa(MA) and Cylindrospermopsis raciborskii(CR), and their corresponding trihalomethane(THM) formation potential. The results showed that dual dosing with NaOCl plus ClO_2 was more effective in enhancing the deformation of cyanobacterial cells compared to single dosing with Na OCl, especially for CR-rich water.Both preoxidation approaches for CR-rich water effectively reduced the CR cell count with less remained dissolved organic carbon(DOC), which benefited subsequent coagulation–flotation. However, preoxidation led to an adverse release of algogenic organic matter(AOM) in the case of MA-rich water. The release of AOM resulted in a poor removal in MA cells and a large amount of THM formation after oxidation-assisted coagulation-flotation process. The reduction in THM formation potential of CR-rich waters is responsible for effective algae and DOC removal by alum coagulation. It is concluded that the species-specific characteristic of cyanobacteria and their AOM released during chlorination significantly influences the performance of coagulation–flotation for AOM removal and corresponding THM formation. 相似文献
95.
96.
ABSTRACT: Geostationary Operational Environmental Satellite (GOES) thermal infrared (IR) data were used to study regional cold nocturnal temperature fluctuations that are important in assessing citrus freeze damage. Dummy variables techniques were used to analyze the temperature difference between the east and west sides of Central Florida, which was obtained from both ground measurement minimum temperature (TGMM) and the GOES mean temperature (TGOES) on low-temperature nights. The low temperature pattern, which was closely related to the citrus freeze damage pattern in Central Florida, was identified by GOES thermal IR data but not by conventional ground measurements. The low surface temperature in the west side and east side appears to be attributable to differences in soil types, water tables, and drainage classes in both regions. 相似文献
97.
ABSTRACT: The San Antonio River Walk is considered a unique tourist attraction as well as an urban rejuvenation catalyst for San Antonio, Texas. This utilization of the mile-long horseshoe bend in the downtown area of San Antonio is as successful and imaginative as can be found in the United States. Testimony is very strong from San Antonio voters and outside visitors of the great social and economic value of the River Walk. This overwhelming success has led to plans for expansion of the present River Walk. The River Walk expansion decision should not be evaluated merely on a benefit-cost ratio. It has become the recommendation of the Water Resources Council that intangible attributes such as recreational values and social impacts should be considered as well as tangible attributes such as cost. This prevailing attitude has highlighted the application of decision analysis techniques with multiattribute utility ratings. Decision analysis is a systematic solution procedure which can be used to crystallize a complicated decision problem into manageable subproblems by ranking the decision alternatives in accordance with cardinal utility values attached to their consequences. Recent advances in multiattribute utility theory allow a decision maker to weigh utility assessment over tangible and intangible attributes according to their relative importance. This insures that the intangible attributes will receive due consideration in the final decision-making. 相似文献
98.
Jobs Versus the Environment: An Industry-Level Perspective 总被引:3,自引:0,他引:3
Richard D. Morgenstern William A. Pizer Jhih-Shyang Shih 《Journal of Environmental Economics and Management》2002,43(3):412
The possibility that workers could be adversely affected by increasingly stringent environmental policies has led to claims of a “jobs versus the environment” trade-off by both business and labor leaders. The present research examines this claim at the industry level for four heavily polluting industries: pulp and paper mills, plastic manufacturers, petroleum refiners, and iron and steel mills. Combining a unique plant-level data set with industry-level demand information, we find that increased environmental spending generally does not cause a significant change in employment. Our average across all four industries is a net gain of 1.5 jobs per $1 million in additional environmental spending, with a standard error of 2.2 jobs—an economically and statistically insignificant effect. There are statistically significant and positive effects in two industries, but total number of affected jobs remains quite small. These small positive effects can be linked to labor-using factor shifts and relatively inelastic estimated demand. 相似文献
99.
Ying-Liang Chen Juu-En Chang Pai-Haung Shih Ming-Sheng Ko Yi-Kuo Chang Li-Choung Chiang 《Journal of environmental management》2010,91(9):1892-1897
The purpose of this study was to combine the physical pretreatments of grinding, sieving, and magnetic-separation processes to reclaim iron-rich materials from the desulfurization slag, and to use the remainder for cement clinker production. The iron-rich materials can be separated out efficiently by grinding for 30 min and sieving with a 0.3 mm mesh. The non-magnetic fraction of the particles smaller than 0.3 mm was in the majority, and proved to be suitable for use as a cement raw material. The raw mixes prepared with a pretreated desulfurization slag had a relatively high reactivity, and the temperature at which alite forms was significantly reduced during the clinkerization process. The clinkers produced with 10% desulfurization slag had a high level of alite and good grindability. Generally, the improvements in clinkerization and clinker grindability are beneficial to energy conservation in cement manufacture. 相似文献
100.
The PCDD/Fs in the ambient air associated with concentration and dry deposition flux of four seasons were characterized in rural area. The mean PCDD/F concentrations were 0.342, 0.221, 0.675, 0.741 pg m(-3) and the mean I-TEQ values were 0.027, 0.016, 0.024, 0.063 pg m(-3) in spring, summer, fall and winter, respectively. Ambient air in winter was higher by a factor of 3.4 and 3.9 for PCDD/F concentration and I-TEQ, respectively, than in summer. The study area is located in a Tropical region. Hence, domestic heating is not found in this area and is not responsible for the elevated winter concentration in comparison to other studies. A smooth plate with a sharp leading edge that is pointed into the wind by a wind vane was used for measuring dry deposition flux of PCDD/Fs. Atmospheric dry deposition fluxes of total PCDD/Fs were 140, 116, 137, and 207 pg m(-2)day(-1) in spring, summer, fall, and winter, respectively, and averaged approximately 150 pg m(-2)day(-1). The total dry deposition flux was found to decrease as the temperature increased. Calculated dry deposition velocities of total PCDD/Fs were 0.45, 0.52, 0.32 and 0.39 cm s(-1) in spring, summer, fall, and winter, respectively, and averaged 0.42 cm s(-1). 相似文献