全文获取类型
收费全文 | 2566篇 |
免费 | 134篇 |
国内免费 | 988篇 |
专业分类
安全科学 | 159篇 |
废物处理 | 138篇 |
环保管理 | 208篇 |
综合类 | 1550篇 |
基础理论 | 410篇 |
环境理论 | 1篇 |
污染及防治 | 883篇 |
评价与监测 | 115篇 |
社会与环境 | 105篇 |
灾害及防治 | 119篇 |
出版年
2024年 | 5篇 |
2023年 | 58篇 |
2022年 | 152篇 |
2021年 | 112篇 |
2020年 | 104篇 |
2019年 | 95篇 |
2018年 | 89篇 |
2017年 | 117篇 |
2016年 | 145篇 |
2015年 | 167篇 |
2014年 | 187篇 |
2013年 | 246篇 |
2012年 | 221篇 |
2011年 | 243篇 |
2010年 | 209篇 |
2009年 | 182篇 |
2008年 | 170篇 |
2007年 | 162篇 |
2006年 | 151篇 |
2005年 | 70篇 |
2004年 | 68篇 |
2003年 | 89篇 |
2002年 | 74篇 |
2001年 | 60篇 |
2000年 | 71篇 |
1999年 | 75篇 |
1998年 | 63篇 |
1997年 | 56篇 |
1996年 | 55篇 |
1995年 | 45篇 |
1994年 | 39篇 |
1993年 | 35篇 |
1992年 | 17篇 |
1991年 | 11篇 |
1990年 | 9篇 |
1989年 | 7篇 |
1988年 | 4篇 |
1987年 | 4篇 |
1986年 | 4篇 |
1985年 | 2篇 |
1984年 | 3篇 |
1983年 | 3篇 |
1982年 | 2篇 |
1981年 | 1篇 |
1977年 | 1篇 |
1972年 | 2篇 |
1918年 | 1篇 |
1917年 | 1篇 |
1916年 | 1篇 |
排序方式: 共有3688条查询结果,搜索用时 538 毫秒
801.
802.
The consumption of heavy metals is detrimental to human health and most countries restrict the concentration of metals such as lead (Pb) in food and beverages. Recent tests have detected high Pb concentrations in certain commercial brands of tea leaves and this finding has raised concerns for both producers and consumers. To investigate what factors may be contributing to the increase in Pb accumulation in the tea leaves we collected tea leaves and soils from tea producing areas and analyzed them for Pb concentration, pH and organic matter content. The result showed the Pb concentration of 47% investigated tea leaves samples was beyond 2 mg kg(-1), the permissible levels given by China. The total Pb concentration in the surface and subsurface soil layers averaged 36.4 and 32.2 mg kg(-1), respectively which fall below of the 60 mg kg(-1) limit provided for organic tea gardens in China. The pH of the tea garden soils was severely acidic with the lowest pH of 3.37. Soils under older tea gardens tended to have a lower pH and a higher Pb bioavailability which was defined as the amount of lead extracted by CaCl2 solution than those under younger tea gardens. We found that the concentration of bioavailable Pb and the percentage of bioavailable Pb (bioavailable Pb relative to total Pb concentration) were positively correlated with soil H+ activity and soil organic matter content, and the organic matter accumulation contribute more effects on Pb bioavailability in these two factors. We conclude that soil acidification and organic matter accumulation could contribute to increasing Pb bioavailability in soil and that these could increase Pb uptake and accumulation in the tea leaves. 相似文献
803.
According to the theory of photocatalysis, the efficiency of photocatalysis decreases mostly due to the recombination of photo-generated electron-hole pairs. An electric field across a photocatalyst can promote the separation of photo-generated electrons and holes and prevent them from recombination so as to enhance the efficiency of photocatalysis. And the synergetic decomposition efficiency of photocatalysis and an electric field is greater than that of the simple combine of their single efficiency. The performance of photocatalysis enhanced by electric field (PEEF) and operating conditions such as the direction of the electric field, the voltages between the two electrodes, the material of the electrodes, which may affect the efficiency of PEEF, were investigated in this paper. The results indicate that the system of PEEF abides the established theory of photocatalysis. 相似文献
804.
Performance of three-phase three-dimensional electrode reactor for the reduction of COD in simulated wastewater-containing phenol 总被引:18,自引:0,他引:18
The removal of chemical oxygen demand (COD) from wastewater-containing phenol was investigated using three-phase three-dimensional electrode reactor. Special attention was paid to experimentally probe the performance of the reactor in COD removal in the process of repeated batch runs. The experimental results showed that the reactor could remove COD from phenol-containing wastewater much more efficiently than both granulated activated carbon (GAC) adsorption bed and conventional three-dimensional electrode. For 200th batch run, the three-phase three-dimensional electrode reactor with an airflow of 5 l min(-1) and a cell voltage of 30 V could remove 1350 ppm COD from the wastewater in 30 min while conventional three-dimensional electrode reactor with a same cell voltage and GAC adsorption bed with a same airflow only could remove 610 and 1000 ppm, respectively, at the same reaction duration. Although it was found that COD removal decreased with increasing repeated batch runs in our experimental range, due to adsorption saturation of GAC and electrode passivation, the extent of decrease for the three-phase three-dimensional electrode is much less than those for conventional three-dimensional electrodes and GAC adsorption beds. The passivated reactor could be partly re-activated by electrolysis in the presence of MnO2. 相似文献
805.
A microbial consortium consisting of a white-rot fungus 8-4* and a Pseudomonas 1-10 was isolated from wastewater treatment facilities of a local dyeing house by enrichment, using azo dye Direct Fast Scarlet 4BS as the sole source of carbon and energy, which had a high capacity for rapid decolorization of 4BS. To elucidate the decolorization mechanisms, decolorization of 4BS was compared between individual strains and the microbial consortium under different treatment processes. The microbial consortium showed a significant improvement on dye decolorization rates under either static or shaking culture, which might be attributed to the synergetic reaction of single strains. From the curve of COD values and the UV-visible spectra of 4BS solutions before and after decolorization cultivation with the microbial consortium, it was found that 4BS could be mineralized completely, and the results had been used for presuming the degrading pathway of 4BS. This study also examined the kinetics of 4BS decolorization by immobilized microbial consortium. The results demonstrated that the optimal decolorization activity was observed in pH range between four and 9, temperature range between 20 and 40 degrees C and the maximal specific decolorization rate occurred at 1,000 mg l(-1) of 4BS. The proliferation and distribution of microbial consortium were also microscopically observed, which further confirmed the decolorization mechanisms of 4BS. 相似文献
806.
调理剂对CAF污泥浓缩工艺影响的试验研究 总被引:1,自引:0,他引:1
涡凹气浮(CAF)已广泛应用于工业废水和城市污水的预处理中.由于污泥本身的特性原因,CAF在污泥处理中尚没有应用.通过试验投加污泥调理剂改变污泥的特性,以达到将CAF工艺用于浓缩活性污泥的目的.试验表明,CAF工艺浓缩低浓度剩余活性污泥效果很好,但正确选择污泥调理剂的投加点和投加量对CAF污泥浓缩工艺至关重要. 相似文献
807.
808.
809.
针对城市产业水污染状况,应用产业结构和工业行业结构优化模型,试图找出城市产业结构调整方法。研究以株洲市为例,根据株洲市产业结构和行业结构特点对模型进行改进和最优化计算。计算结果表明,产业和行业生产用水的调整可以减少废水排放量和实现经济增长。在此基础上,提出了株洲市产业和行业凋整方案,以期实现城市经济发展与环境保护协调发雇。 相似文献
810.
滇池底泥微生物菌群对微囊藻毒素的生物降解 总被引:9,自引:0,他引:9
采用滇池水华蓝藻中提取提纯的微囊藻毒素(microcystins,MCs)作为微生物生长的碳源和氮源,从长期暴露于蓝藻水华的滇池底泥中,通过从含低浓度到高浓度MCs的逐步培养驯化,获得了高效降解MCs的微生物混合菌群,在初始MC-RR和LR浓度大约分别为50mg/L和30mg/L下,3d内可将MCs全部降解。进一步活性研究显示,不同含碳和含氮化合物虽然能够促进混合微生物菌群的生长,但对降解MCs却无明显的促进作用,说明MCs既可以作为微生物生长的碳源,又可以作为微生物生长的氮源,在富含有机物的天然水体中并不一定能够促进微生物对MCs的生物降解。 相似文献