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961.
Estimating temperature dependence of solubility and octanol-water partition coefficient for organic compounds using RP-HPLC. 总被引:1,自引:0,他引:1
Temperature dependence data for physical-chemical properties is increasingly required for modelling the fate of chemicals in the environment. Solubility and octanol-water partition coefficient (Kow) are among the most important parameters. A simple and fast method is presented to determine solubility and Kow of organic chemicals at different temperatures (5 degrees C, 15 degrees C, 25 degrees C, 35 degrees C) utilising a variable temperature RP-HPLC column. Correlations between capacity factors (k') and solubility and Kow were determined for some halogenated and methylated benzenes and showed that this approach could be used to predict acceptable results. New values for solubility and Kow as function of temperature for several compounds are presented. 相似文献
962.
Joke Muys Yves Jacquemyn Bettina Blaumeiser Laura Bourlard Nathalie Brison Saskia Bulk Patrizia Chiarappa Anne De Leener Marjan De Rademaeker Julie Désir Anne Destrée Koenraad Devriendt Annelies Dheedene Armelle Duquenne Annelies Fieuw Erik Fransen Jean-Stéphane Gatot Mauricette Jamar Sandra Janssens Jorien Kerstjens Kathelijn Keymolen Damien Lederer Björn Menten Bruno Pichon Sonia Rombout Yves Sznajer Ann Van Den Bogaert Kris Van Den Bogaert Joris Vermeesch Katrien Janssens 《黑龙江环境通报》2020,40(10):1272-1283
963.
Hari Eswaran Diana Escalona-Vargas Elijah H. Bolin James D. Wilson Curtis L. Lowery 《黑龙江环境通报》2017,37(2):193-196
Fetal magnetocardiography provides the requisite precision for diagnostic measurement of electrophysiological events in the fetal heart. Despite its significant benefits, this technique with current cryogenic based sensors has been limited to few centers, due to high cost of maintenance. In this study, we show that a less expensive non-cryogenic alternative, optically pumped magnetometers, can provide similar electrophysiological and quantitative characteristics when subjected to direct comparison with the current technology. Further research can potentially increase its clinical use for fetal magnetocardiography. © 2016 John Wiley & Sons, Ltd. 相似文献
964.
965.
966.
Eucalyptus forest; and in the composition of understorey herbs, sedges, and grasslands. Pollen concentration and charcoal and organic
content also exhibit post-European changes. Thus, pollen analysis provides a technique for determining changes in sediment
budgets and identifying major vegetation changes in floodplains. 相似文献
967.
Designing chemical processes for the environment requires consideration of several indexes of environmental impact including ozone depletion, global warming potentials, human and aquatic toxicity, photochemical oxidation, and acid rain potentials. Current methodologies, such as the generalized waste reduction algorithm (WAR), provide a first step towards evaluating these impacts. However, to address the issues of accuracy and the relative weights of these impact indexes, one must consider the problem of uncertainties. Environmental impacts must also be weighted and balanced against other concerns, such as their cost and long-term sustainability. These multiple, often conflicting, goals pose a challenging and complex optimization problem, requiring multi-objective optimization under uncertainty. This paper will address the problem of quantifying and analyzing the various objectives involved in process design for the environment. Towards this goal, we proposed a novel multi-objective optimization framework under uncertainty. This framework is based on new and efficient algorithms for multi-objective optimization and for uncertainty analysis. This approach finds a set of potentially optimal designs where trade-offs can be explicitly identified, unlike cost-benefit analysis, which deals with multiple objectives by identifying a single fundamental objective and then converting all the other objectives into this single currency. A benchmark process for hydrodealkylation (HDA) of toluene to produce benzene modeled in the ASPEN simulator is used to illustrate the usefulness of the approach in finding environmentally friendly and cost-effective designs under uncertainty. 相似文献
968.
969.
Carbon monoxide (CO) in the surface sea waters is produced predominantly by photochemical processes, oxidized by micro-organisms and outgassed to the atmosphere. to assess carbon monoxide flux from the oceans to the atmosphere, the photochemical production and microbial oxidation of carbon monoxide in the oceanic mixed-layer was investigated during several oeanographic cruises and in the laboratory. the photoproduction rate of carbon monoxide was found to be well correlated to the concentration of dissolved organic carbon (DOC) in coastal and open ocean surface waters. Taking a global average carbon monoxide production rate of 10 ± 2 nmole litre-1 (mg DOC hr)-1 in the surface open ocean water, and 25 ± 7 nmole litre-1 (mg DOC hr)-1 in coastal sea water, at cloud-free summer solar noon, the photochemical production of carbon monoxide in the global oceans is estimated to be at a rate of 1200 ± 200 Tg CO y-1. the microbial carbon monoxide turnover time in the mixed-layer was observed to range from hours in a coastal estuary to 16 days in the Pacific along 1057deg; W in dark incubations. Natural sunlight can largely inhibit the microbial consumption of carbon monoxide in surface water. On a global scale, microbial consumption is responsible for the loss of less than 10% of photochemical produced carbon monoxide in the surface ocean. Field measurements have shown that the net transport of carbon monoxide from the euphotic zone to the underlying deeper ocean water is limited and that the overall life time in surface sea waters is less than 3-4 hours. When combined, these field measurements with the photoproduction and microbial consumption rates obtained, we estimate the oceanic flux to the atmosphere is about 1000 ± 200 Tg CO y-1, which represents the largest single source of atmospheric carbon monoxide. 相似文献
970.
The purpose of this review was to summarize the literature on occupational, acute, traumatic hand injury and suggest directions for future research. In 1996, the leading occupational injury treated in United States' hospital emergency departments was an acute hand injury (e.g. laceration, crush or fracture). These injuries affected 30% of an estimated 3.3 million injured workers (990,000). Cuts and lacerations of the fingers ranked third after back and leg strains in the number of lost workday cases in the USA in 1994. The incidence rate of hand injuries studied in seven manufacturing environments around the world ranged from 4 to 11 per 100 workers per year. Workers aged 24 years or less had the highest risk of hand injury. Men had higher rates of severe hand injury than women.Despite the high frequency and significant amount of lost work time associated with these injuries, they are poorly understood from an etiological perspective. There is only one case-control study of occupational hand injury in the literature. That study suggested an important role for both fixed (age) and transient risk factors (doing an unusual task) at the time of the injury. More analytic epidemiological research is needed to identify potentially modifiable risk or protective factors (e.g. glove use) for acute hand injuries. In this regard, the case-crossover design, a relatively new epidemiological approach using cases as their own controls, could prove an efficient method for determining transient, modifiable risk factors for acute, occupational hand injury. 相似文献