Environmental Chemistry Letters - Heterogeneous reactions involving aerosol water, i.e., haze chemistry, are responsible for high aerosol concentrations observed during severe haze events in... 相似文献
• The resistance of phage PhiX174 to nZVI was much stronger than that of MS2.• The nZVI damaged the surface proteins of both bacteriophages.• The nZVI could destroy the nucleic acid of MS2, but not that of PhiX174.•The phage inactivation was mainly attributed to the damage of the nucleic acid. Pathogenic enteric viruses pose a significant risk to human health. Nanoscale zero-valent iron (nZVI), a novel material for environmental remediation, has been shown to be a promising tool for disinfection. However, the existing research has typically utilized MS2 or f2 bacteriophages to investigate the antimicrobial properties of nZVI, and the resistance difference between bacteriophages, which is important for the application of disinfection technologies, is not yet understood. Here, MS2 and PhiX174 containing RNA and DNA, respectively, were used as model viruses to investigate the resistances to nZVI. The bacteriophage inactivation mechanisms were also discussed using TEM images, protein, and nucleic acid analysis. The results showed that an initial concentration of 106 PFU/mL of MS2 could be completely inactivated within 240 min by 40 mg/L nZVI at pH 7, whereas the complete inactivation of PhiX174 could not be achieved by extending the reaction time, increasing the nZVI dosage, or changing the dosing means. This indicates that the resistance of phage PhiX174 to nZVI was much stronger than that of MS2. TEM images indicated that the viral particle shape was distorted, and the capsid shell was ruptured by nZVI. The damage to viral surface proteins in both phages was examined by three-dimensional fluorescence spectrum and sodium dodecyl sulfate polyacrylamide gel electrophoresis (SDS-PAGE). However, the nucleic acid analysis demonstrated that the nucleic acid of MS2, but not PhiX174, was destroyed. It indicated that bacteriophage inactivation was mainly attributed to the damage of nucleic acids. 相似文献
Environmental Science and Pollution Research - Effects of prenatal ambient air pollution exposure could increase the risk of adverse pregnancy outcomes, which have been well documented by various... 相似文献
Environmental Science and Pollution Research - In this study, a new straw-iron composite material (ST@Fe) was synthesized through impregnation and freeze-drying process for persulfate (PS)... 相似文献
Environmental Science and Pollution Research - The coordination relationship between new-type urbanization and urban low-carbon development under the goal of carbon neutrality has become a hot... 相似文献
Journal of Polymers and the Environment - In this study, the nanohybrid drug carrier were synthesized by Pickering emulsion-templated encapsulation (PETE) method to control the... 相似文献
An axial symmetry augmented vertical axis wind turbine, which is suitable for arbitrary wind directions, is proposed in this paper. In order to improve the power generation ability of the S-type vertical axis wind turbine, a set of so-called “collection-shield boards” are installed symmetrically around the rotating S-type rotor. The flow fields around this type of wind turbine are numerically simulated with the aid of CFD method. The optimized design of geometrical parameters of the rotor and collection-shield boards is conducted by using the orthogonal design method. The obtained results suggest that the power output of the optimized augmented wind turbine can reach nearly three times higher than that of the conventional S-type vertical axis wind turbine. 相似文献
Ambient PM2.5 samples were collected at four sites in Xiamen, including Gulangyu (GLY), Hongwen (HW), Huli (HL) and Jimei (JM) during January, April, July and October 2013. Local source samples were obtained from coal burning power plants, industries, motor vehicles, biomass burning, fugitive dust, and sea salt for the source apportionment studies. The highest value of PM2.5 mass concentration and species related to human activities (SO42–, NO3–, Pb, Ni, V, Cu, Cd, organic carbon (OC) and elemental carbon (EC)) were found in the ambient samples from HL, and the highest and lowest loadings of PM2.5 and its components occurred in winter and summer, respectively. The reconstructed mass balance indicated that ambient PM2.5 consisted of 24% OM (organic matter), 23% sulfate, 14% nitrate, 9% ammonium, 9% geological material, 6% sea salt, 5% EC and 10% others. For the source profiles, the dominant components were OC for coal burning, motor vehicle, biomass burning and sea salt; SO42– for industry; and crustal elements for fugitive dust. Source contributions were calculated using a chemical mass balance (CMB) model based on ambient PM2.5 concentrations and the source profiles. GLY was characterized by high contributions from secondary sulfate and cooking, while HL and JM were most strongly affected by motor vehicle emissions, and biomass burning and fugitive dust, respectively. The CMB results indicated that PM2.5 from Xiamen is composed of 27.4% secondary inorganic components, 20.8% motor vehicle emissions, 11.7% fugitive dust, 9.9% sea salt, 9.3% coal burning, 5.0% biomass burning, 3.1% industry and 6.8% others.
