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31.
Photocatalytic degradation of lignin was studied with the use of catalysts TiO(2) and Pt/TiO(2). The influence of several experimental parameters, i.e. pH, catalyst dosage and illumination on lignin degradation was investigated. The results showed that application of UV irradiation alone has almost no effect on the reduction of dissolved organic carbon (DOC) and American Dye Manufacture Institute value (ADMI). However, the addition of TiO(2) and Pt/TiO(2) reduced the original DOC (251 mg l(-1)) by more than 40% within 30 min of treatment and the reaction can be simulated with pseudo-first order kinetics. Rapid degradation of lignin was observed in acidic solution using either TiO(2) or Pt/TiO(2) as the catalyst compared to high pH cases. The content of Pt in the Pt/TiO(2) catalyst is 1%. In addition, too much catalyst addition has not increased the DOC and ADMI reduction proportionally. The investigation also indicated that the photocatalytic degradation rates could be enhanced 1-6 times faster after doping TiO(2) with Pt in different pH cases. A modified Nernst type model was adopted to simulate the decoloring process using TiO(2) and Pt/TiO(2) based on the profiles of oxidation reduction potential during the photocatalytic reaction. The developed equation can be used to predict the color removal efficiency of lignin wastewater by the photocatalytic process. 相似文献
32.
Determination of volatile organic profiles and photochemical potentials from chemical manufacture process vents 总被引:2,自引:0,他引:2
Hsu YC Chen SK Tsai JH Chiang HL 《Journal of the Air & Waste Management Association (1995)》2007,57(6):698-704
The main objective of this study was to monitor the volatile organic compounds (VOCs) in the stack gas released from organic chemical industrial plants to determine emission factors. Samples from 52 stacks, with or without air pollution control devices (APCDs), from seven industrial processes were taken and VOCs measured using U.S. Environmental Protection Agency (EPA) Method 18. These 7 processes, including 26 plants, were the manufacturers of acrylonitrile-butadiene-styrene (ABS), polyvinyl chloride (PVC), polystyrene (PS), acrylic resin (ACR), vinyl chloride (VC), para-terephthalic acid (PTA), and synthetic fiber (SYF). The results clearly indicate significant variations of emission factors among the various industrial processes, particularly emission factors for those without APCDs. As expected, those with APCDs yield much less emission factors. Regardless of those with or without APCDs, the order of manufacturing processes with regard to VOC emission factors is SYF > ABS > PS >ACR > PTA > PVC > VC. The emission factors for some processes also differ from those in EPA-42 data file. The VOC profiles further indicate that some VOCs are not listed in the U.S. VOC/Particulate Matter Speciation Data System (SPECIATE). The potential O3 formation is determined from the total amount of VOC emitted for each of seven processes. The resultant O3 yield varied from 0.22 (ACR) to 2.33 g O3 g(-1) VOC (PTA). The significance of this O3 yield is discussed. 相似文献
33.
Ke‐Sheng Cheng Tsu‐Chiang Lei 《Journal of the American Water Resources Association》2001,37(5):1321-1334
ABSTRACT: Reservoir water quality is traditionally monitored and evaluated based on field data. Collecting and analyzing field water quality data are costly and time consuming tasks, and whether a limited number of field data truly characterize the spatial variation of the trophic state within a vast water body is often disputed. In this study we utilize Landsat TM data to estimate the water quality and trophic state of the Te‐Chi reservoir in Central Taiwan. A modified multi‐parameter model of Carlson's trophic state index (TSI) was developed for the Te‐chi reservoir. Water quality parameters (concentration of chlorophyll‐a, total phosphorous measurement, and secchi disk depth) required by the model are found to have high correlations with combinations of TM bands. Therefore, TM data are used to map the trophic state of the reservoir. TM‐derived TSI maps of the reservoir reveal that, in summer, the trophic state in the reservoir generally improves from upstream to downstream and that zones of distinct trophic state exist. A trophic state index based on secchi disk depth may give erroneous values in the upstream section of the reservoir pool due to high sediment concentration in the reservoir inflow. We conclude that the Te‐Chi reservoir is eutrophic or worse in summer and meso‐eutrophic in winter. Implementation of best management practices to reduce nonpoint source pollution in the upstream watershed is highly recommended. This study demonstrates the capability of mapping the trophic state in impounded water bodies using the Landsat TM data. 相似文献
34.
Chiou Yung-Chuan Shen Ming-Yuan Chiang Chin-Lung Li Yi-Luen Lai Wei-Min 《Journal of Polymers and the Environment》2022,30(4):1300-1313
Journal of Polymers and the Environment - Outdoor building materials made of wood require preservatives containing chromated copper arsenate and other carcinogenic substances but still are subject... 相似文献
35.
Both raw water and chlorinated drinking water samples were collected from and the Liu‐Du water treatment plant in northern Taiwan from October 1990 to April 1992. The polycyclic aromatic hydrocarbons (PAHs) and mutagenicity in these water samples were analyzed by GC/MS and Ames test. The Mutagenicity/DMSO (Dimethyl Sulfoxide) ratio in S. typhimurium TA98 and TA100 with or without S9 mixture increased, even higher than 2, following the sequence of unit process. It was observed that the mutagenicity with TA98 (S9+) was highly related to most of PAHs in the raw water; while the mutagenicity with TA98 (S9+) was only correlated with DbA and BghiPr in the treated water. It could be expected that the mutagenicity level was controlled by other predominant components after the raw water was treated, for example, the chlorination process. 相似文献
36.
The objectives of this research were to identify the surface chemical features of activated carbons made of peat, bituminous coal and coconut shell, as well as examine the specific relationship of these properties by using statistical analyses. The results showed that the peat carbons contained much more amounts of Ca, S, P and Mg; however, the bituminous carbons possessed higher contents of Si, Al and Fe. In addition, the content ratios of Al to Si exhibited the Al enrichment phenomenon occurred after the heat treatment. A nonlinear correlation between the pH value and the difference in the amounts of basic and acidic groups was developed. Unfortunately, there were no specific mass ratios found among the acidic functional groups. The results of correspondence analysis (CA) gave a promising confirmation about the EDXRF analysis; moreover, the results of factor analysis (FA) fairly agreed with the findings suggested by CA. Both could explain the specific chemical features of activated carbons made from different materials, especially the CA could differentiate each other in detail. 相似文献
37.
Tsai JH Chang LT Huang YS Chiang HL 《Journal of the Air & Waste Management Association (1995)》2011,61(7):796-805
Particulate compositions including elemental carbon (EC), organic carbon (OC), water-soluble ionic species, and elemental compositions were investigated during the period from 2004 to 2006 in southern Taiwan. The correlation between the pollutant standard index (PSI) of ambient air quality and the various particle compositions was also addressed in this study. PSI revealed a correlation with fine (r = 0.74) and coarse (r = 0.80) particulate matter (PM). PSI manifested a significant correlation with the amount of analyzed ionic species (r approximately 0.80) in coarse and fine particles and a moderate correlation with carbon content (r = 0.63) in fine particles; however, it showed no correlation with elemental content. Although the ambient air quality ranged from good to moderate, the ionic species including chloride (Cl-), nitrate (NO3-), sulfate (SO4(2-)), sodium (Na+), ammonium (NH4+), magnesium (Mg2+), and calcium (Ca2+) increased significantly (1.5-3.7 times for Daliao and 1.8-6.9 times for Tzouying) in coarse PM. For fine particles, NO3-, SO4(2-), NH4+, and potassium (K+) also increased significantly (1.3-2.4 times for Daliao and 2.8-9.6 times for Tzouying) when the air quality went from good to moderate. For meteorological parameters, temperature evidenced a slightly negative correlation with PM concentration and PSI value, which implied a high PM concentration in the low-temperature condition. This reflects the high frequency of PM episodes in winter and spring in southern Taiwan. In addition, the mixing height increase from 980 to 1450 m corresponds to the air quality condition changing from unhealthy to good. 相似文献
38.
Hung-Lung Chiang Kuo-Hsiung Lin Chih-Yu Chen Ching-Guan Choa Ching-Shyung Hwu Nina Lai 《Journal of the Air & Waste Management Association (1995)》2013,63(5):591-600
Abstract This study selected biosolids from a petrochemical waste-water treatment plant as the raw material. The sludge was immersed in 0.5-5 M of zinc chloride (ZnCl2) solutions and pyrolyzed at different temperatures and times. Results indicated that the 1-M ZnCl2-immersed biosolids pyrolyzed at 500 °C for 30 min could be reused and were optimal biosolid adsorbents for benzene adsorption. Pore volume distribution analysis indicated that the mesopore contributed more than the macropore and micropore in the biosolid adsorbent. The benzene adsorption capacity of the biosolid adsorbent was 65 and 55% of the G206 (granular-activated carbon) and BPL (coal-based activated carbon; Calgon, Carbon Corp.) activated carbons, respectively. Data from the adsorption and desorption cycles indicated that the benzene adsorption capacity of the biosolid adsorbent was insignificantly reduced compared with the first-run capacity of the adsorbent; therefore, the biosolid adsorbent could be reused as a commercial adsorbent, although its production cost is high. 相似文献
39.
Chung-Yih Kuo Hao-Jan Yang Yi-Chen Chiang Dian-Jheng Lai Ying-Hsuan Shen Pang-Min Liu 《Environmental science and pollution research international》2014,21(21):12354-12363
Aeolian river dust can seriously affect the air quality in central Taiwan. The main purpose of this study was to assess the concentration variations of PM10 and metals at different elementary schools during river dust episodes. River dust samples were taken from eight sites in the main bare soil areas of the Choshui River. PM10 aerosols from four elementary schools in Yulin County were collected by means of high-volume samplers. Fifteen elements (Fe, Al, Ca, Mg, Mn, Zn, Ti, Ni, V, Cr, As, Pb, Cu, Co, and Cd) in the river dust and PM10 were analyzed in this study. The coefficients of divergence (CDs) were obtained by comparing the metal compositions in PM10 aerosols at the four schools on the sampling days with the mean metal contents in the river soil samples as reference. The CD values showed that metal compositions in the aerosols at high-exposure sites during river dust episodes were similar to those compositions in the river dust. The concentrations of PM10 at the high-exposure schools during river dust episodes were much higher than those during non-river-dust episodes. This study also indicated that at the high-exposure sites, both the PM10 and metal concentrations were higher than at the low-exposure and control sites, not only during the river dust episodes, but also after the river dust episodes. The concentrations of toxic metals (Ni, Cr, As, and Cd) at the high-exposure sites were about 11.3 times higher during the river dust episodes (189 ng/m3) than during non-river-dust episodes (16.7 ng/m3) and about 8.9 times higher during the same periods at the control site (21.3 ng/m3). 相似文献
40.
Guor-Cheng Fang Hung-Che Chiang Yu-Cheng Chen You-Fu Xiao Yuan-Jie Zhuang 《Environmental Forensics》2014,15(4):296-305
This study characterized the dry deposition flux and dry deposition velocity (Vd) of metallic elements attached on particulate matter. Specifically, large particles (>10 μm), coarse particles (10 μm~2.5 μm), and fine particles (<2.5 μm) were studied at the Gong Ming Junior High School (Taichung Airport) and Taichung Harbor sampling sites in central Taiwan. Ambient air samples were collected to determine total suspended particulate matter (TSP), dry deposition plate (DDP), Vd, coarse particulate matter (PM2.5–10) and fine particulate matter (PM2.5), and metallic elements concentrations at the Airport and Taichung Harbor sites between June 17, 2013, and November 14, 2013. The results revealed that the average TSP, DDP, Vd, PM2.5–10, and PM2.5 particulate at the Airport were 54.55 (μg/m3), 902.25 (μg/m2-min), 17.11 (m/sec), 0.003 (μg/m3), and 0.010 (μg/m3), respectively; while these values at Taichung Harbor were 63.66 (μg/m3), 539.69 (μg/m2-min), 9.94 (m/sec), 0.003 (μg/m3), and 0.014 (μg/m3), respectively. In addition, the results showed that the average Cu and Pb concentrations were higher than Cr, Ni, and Cd for both the airport and harbor sampling sites. Furthermore, Cr, N, Cu, Cd, and Pb had the highest average concentrations versus those reported for other study areas, with one exception: The results obtained in Kacanik, Kosovo, during 2005. The average metallic elements concentrations order was Cu > Pb > Cr > Ni > Cd. 相似文献