全文获取类型
收费全文 | 2231篇 |
免费 | 195篇 |
国内免费 | 758篇 |
专业分类
安全科学 | 215篇 |
废物处理 | 136篇 |
环保管理 | 162篇 |
综合类 | 1450篇 |
基础理论 | 307篇 |
环境理论 | 1篇 |
污染及防治 | 566篇 |
评价与监测 | 98篇 |
社会与环境 | 157篇 |
灾害及防治 | 92篇 |
出版年
2024年 | 8篇 |
2023年 | 40篇 |
2022年 | 135篇 |
2021年 | 138篇 |
2020年 | 115篇 |
2019年 | 91篇 |
2018年 | 109篇 |
2017年 | 124篇 |
2016年 | 110篇 |
2015年 | 129篇 |
2014年 | 175篇 |
2013年 | 232篇 |
2012年 | 198篇 |
2011年 | 208篇 |
2010年 | 173篇 |
2009年 | 161篇 |
2008年 | 155篇 |
2007年 | 109篇 |
2006年 | 161篇 |
2005年 | 97篇 |
2004年 | 65篇 |
2003年 | 58篇 |
2002年 | 58篇 |
2001年 | 51篇 |
2000年 | 55篇 |
1999年 | 41篇 |
1998年 | 37篇 |
1997年 | 25篇 |
1996年 | 22篇 |
1995年 | 32篇 |
1994年 | 13篇 |
1993年 | 13篇 |
1992年 | 12篇 |
1991年 | 9篇 |
1990年 | 5篇 |
1989年 | 6篇 |
1988年 | 3篇 |
1987年 | 2篇 |
1986年 | 4篇 |
1984年 | 2篇 |
1983年 | 1篇 |
1982年 | 1篇 |
1981年 | 1篇 |
排序方式: 共有3184条查询结果,搜索用时 934 毫秒
241.
常温低基质厌氧氨氧化反应器启动及其稳定性 总被引:5,自引:0,他引:5
以上向流生物滤池为反应器,以实验室内氧化沟回流污泥为接种污泥,采用先培育好氧生物膜,后转为厌氧环境培育厌氧氨氧化生物膜的方式,成功实现了常温低基质浓度下厌氧氨氧化反应器的启动。控制反应器进水pH为7.50~7.80,NH4+-N为30~40 mg/L,NO2--N为35~50 mg/L,温度为20~25℃。224 d以后,反应器启动成功。在稳定运行阶段,出水亚硝氮和氨氮的平均浓度分别为1.4 mg/L和4.6 mg/L,平均去除率分别为95.3%和90.1%,去除比例为1~1.8∶1,主要集中在1.4~1.5∶1,亚硝氮和氨氮去除的容积负荷分别为104.2 mg/(L.d)和146.0 mg/(L.d)。 相似文献
242.
响应面分析法优化稀土废水MAP沉淀法脱氮 总被引:1,自引:0,他引:1
经过预处理后的稀土生产废水,其氨氮浓度大幅降低,但并未达到中华人民共和国《稀土工业污染物排放标准》(GB26451-2011)中氨氮浓度限值。实验通过响应面分析法中的Box-Behnken实验设计(BBD),取pH、n(Mg):n(N)、n(P):n(N)3因素,采用Design-Expert 8.0.6,建立合适的剩余氨氮浓度及剩余总磷浓度模型,得到回归方程,并分析模型各项指标,各因素及其相互作用对剩余氨氮浓度及剩余总磷浓度的影响。利用预测模型预测最佳实验条件,在最佳实验条件下验证预测结果,并对沉淀物进行X射线衍射(XRD)分析。结果显示,二次响应模型适用于剩余氨氮浓度及剩余总磷浓度,2个模型均拥有较好的拟合程度、可信度及精密度,最优反应条件为:pH=9.88、n(Mg):n(N)=1.50:1、n(P):n(N)=1.38:1时,剩余氨氮浓度为46.58 mg/L,剩余总磷浓度为7.85 mg/L。在最优条件下所得到的沉淀物并非纯净的MgNH4PO4·6H2O,还有Mg3(PO4)2·22H2O生成。 相似文献
243.
244.
The effect of polarity on the oxidation of Hg0 was examined in the presence of O2 via a pulsed corona discharge (PCD). The experimental result showed no difference in the energy yield of Hg0 oxidation at both positive and negative PCDs (∼8 μg Hg W h−1 at following conditions: total flow rate = 2 L min−1 (Hg0 = 50 μg N m−3, O2 = 10%, and N2 balance), temperature = 150 °C, and specific energy density = 5-15 W h N m−3). This suggests that the positive PCD process used to control gaseous air pollutants may play an essential key role in Hg0 oxidation because it consumes enough energy (∼15 W h N m−3) but an electrical precipitator could not because it consumes less energy (∼0.3 W h N m−3) to oxidize Hg0. 相似文献
245.
PCDDs and PCDFs in sewage sludges from two wastewater treatment plants in Beijing, China 总被引:2,自引:0,他引:2
The levels of polychlorinated dibenzo-p-dioxins (PCDDs) and dibenzofurans (PCDFs) were analyzed by an isotope-dilution high-resolution mass spectrometric in 16 sewage sludges, sampled from 2004 to 2009, from two municipal wastewater treatment plants (WWTPs) in Beijing. Total toxicity equivalent (TEQ) values were evaluated using the toxicity equivalent factors proposed by International for PCDD/Fs. The I-TEQs for these sewage sludges were from 0.97 to 15.0 pg g−1 dry weight (dw) with a mean value 4.43 pg g−1 dw, indicating that all I-TEQs were below Chinese legislation limit value regulated for agricultural use in soils.The results from limited samples (16 samples) showed that the levels of PCDD/Fs might be correlated with the sludge age. Meanwhile, the temporal trends of PCD/Fs suggested that the I-TEQs may correlate with rainfall in the present study. 相似文献
246.
The dissipation of carbendazim and chloramphenicol alone and in combination and their effects on soil fungal:bacterial ratios and soil enzyme activities were investigated. The results revealed that carbendazim dissipation was little affected by chloramphenicol, whereas chloramphenicol dissipation was found to be retarded significantly by the presence of carbendazim. The inhibitory effect of carbendazim on the fungal:bacterial ratios was increased by the presence of chloramphenicol, and the inhibitory effect of chloramphenicol on neutral phosphatase was increased by the presence of carbendazim. Carbendazim increased soil catalase and urease activities, but this increase was partially diminished by the presence of chloramphenicol. Little interaction was observed between carbendazim and chloramphenicol with regard to their influence on soil invertase. The results obtained in this study suggest that combinations of fungicides and antibiotics may alter the compounds’ individual behaviors in soil and their effects on soil enzymes. 相似文献
247.
Kim SS Lee SM Park KH Kwon DW Hong SC 《Journal of the Air & Waste Management Association (1995)》2011,61(5):552-558
This study investigated the effect of adding vanadium (V) to natural manganese oxide (NMO) in ammonia (NH3) selective catalytic reduction (SCR). The addition of V to NMO decreased the catalytic activity at low temperatures by blocking the active site. However, the enhancement of catalytic activity was achieved by controlling NH3 oxidation at high temperatures. From the NH3 temperature programmed desorption and oxygen on/off test, it was confirmed that the amount of Lewis acid site and active lattice oxygen of the catalyst affects the catalytic performance at low temperature. 相似文献
248.
文中综述了氰化物的危害和含氰废水的来源以及目前处理含氰废水的方法。以工程实例重点介绍亚铁蓝法处理此废水的应用。亚铁蓝法除氰可分二级进行,第一级在中性条件总氰去除率达到80%以上,第二级直接在一级出水加碱调pH至8~9沉淀即可,通过二级处理总氰去除率达到95%左右。 相似文献
249.
Chang-Qing Ke Dong Zhang Fu-Qiang Wang Shu-Xing Chen Christance Schmullius Wolfgang-Martin Boerner Hui Wang 《Regional Environmental Change》2011,11(1):161-173
Coastal zones provide habitat cores and corridors that maintain the diversity of entire landscapes, and they can form the
cornerstone elements of regional conservation strategies. Natural environmental driving factors and excessive anthropogenic
activities play important roles in coastal wetland change. Many studies have used remote sensing images to map and assess
coastal wetland change on local or regional scales. This paper aims to provide insight into coastal wetland change in the
Yancheng National Nature Reserve (YNNR) using remote sensing technology and landscape metrics analysis. The results reveal
that grass flat and reed areas have significantly decreased, whereas agriculture fields, aquaculture ponds and built-up areas
have continuously increased from 1988 to 2006. The spatial pattern of the coastal landscape has become fragmented and heterogeneous
under great pressure from rapid economic development and population growth. The wetland changes have important impacts on
natural habitat of the red-crowned cranes. The results of this study provide basic information that is required for developing
measures toward a sustainable management and conservation of the YNNR. 相似文献
250.
To estimate the impacts of invasive plants on ecosystems, a survey has been conducted in three sites including both buffer zones and core zones. 13, 19 species are found in the Yuntai Mountain and Longchi Mountain natural reserve respectively, and 23 in the Purple Mountain Natural Park. Altogether 25 species belonging to 12 families, the majority of which are native to North America, some of them have set up stable reproducible populations. Among them, Solidago canadensis is found in Longchi Mountain and Purple Mountain. Communities of Galinsoga parviflora, Gynura crepidioides, Ageratum conyzoides, and Ambrosia artemisiifolia pose a serious threat to local biodiversity. 相似文献