全文获取类型
收费全文 | 28160篇 |
免费 | 240篇 |
国内免费 | 215篇 |
专业分类
安全科学 | 617篇 |
废物处理 | 1155篇 |
环保管理 | 3231篇 |
综合类 | 6840篇 |
基础理论 | 6377篇 |
环境理论 | 13篇 |
污染及防治 | 6997篇 |
评价与监测 | 1717篇 |
社会与环境 | 1558篇 |
灾害及防治 | 110篇 |
出版年
2022年 | 223篇 |
2021年 | 226篇 |
2019年 | 187篇 |
2018年 | 374篇 |
2017年 | 337篇 |
2016年 | 558篇 |
2015年 | 434篇 |
2014年 | 638篇 |
2013年 | 1924篇 |
2012年 | 756篇 |
2011年 | 1033篇 |
2010年 | 862篇 |
2009年 | 961篇 |
2008年 | 1084篇 |
2007年 | 1195篇 |
2006年 | 1043篇 |
2005年 | 855篇 |
2004年 | 891篇 |
2003年 | 883篇 |
2002年 | 810篇 |
2001年 | 1004篇 |
2000年 | 715篇 |
1999年 | 502篇 |
1998年 | 326篇 |
1997年 | 354篇 |
1996年 | 340篇 |
1995年 | 395篇 |
1994年 | 384篇 |
1993年 | 343篇 |
1992年 | 314篇 |
1991年 | 367篇 |
1990年 | 326篇 |
1989年 | 292篇 |
1988年 | 296篇 |
1987年 | 259篇 |
1986年 | 236篇 |
1985年 | 250篇 |
1984年 | 293篇 |
1983年 | 277篇 |
1982年 | 298篇 |
1981年 | 238篇 |
1980年 | 224篇 |
1979年 | 229篇 |
1978年 | 230篇 |
1977年 | 194篇 |
1976年 | 178篇 |
1975年 | 185篇 |
1974年 | 203篇 |
1967年 | 195篇 |
1965年 | 172篇 |
排序方式: 共有10000条查询结果,搜索用时 265 毫秒
891.
892.
Elvis G. Ngwenya Maud Walsh Caroline A. Metosh‐Dickey Ralph J. Portier 《补救:环境净化治理成本、技术与工艺杂志》2006,16(2):79-90
Biological and physicochemical approaches were utilized in a treatment train for acid mine dis charge (AMD) waters. Anaerobic bioreactors, chemical precipitation reactors, and biopolymer chelation reactors, operated in static, semicontinuous, and continuous flow modes, removed significant quantities of metals and sulfates associated with AMD water. Static tests indicated accept able copper removal via precipitation by generation of hydrogen sulfide in anaerobic reactors. However, low pH affected the biopolymer coating in the chelation reactor, resulting in loss of bed surface. Corrections of AMD to pH > 7 resulted in some metal precipitationprior to biopolymer treatment. A series of static semicontinuous tests at pH 5.0 provided improved metal and sulfate removal. Copper (Cu+) was reduced to trace concentrations, while manganese (Mn+), although reduced, proved to be the most recalcitrant of the metals. © 2006 Wiley Periodicals, Inc. 相似文献
893.
894.
The Muggah Creek estuary in Sydney, Nova Scotia, received liquid and solid wastes from a steel mill and its associated coke ovens for approximately 100 years. This resulted in pollution of soils and sediments with polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs), heavy metals, and other pollutants, including those in untreated domestic wastewaters. The Canadian federal and Nova Scotia provincial governments organized the Sydney Tar Ponds Agency (STPA) to develop a remediation approach for the Coke Ovens site soils and Sydney Tar Ponds sediments. The STPA developed a remediation approach for the Sydney Tar Ponds sediments, involving solidification/stabilization (S/S) through mixing cement and other materials into the sediments, and then capping them as a waste pile. High‐density polyethylene (HDPE) plastic sheeting vertical barriers are proposed to be used to divert groundwater and surface water from entering into the S/S‐treated sediments and to collect any water and associated pollutants released from the S/S‐treated sediments. The Coke Ovens site soils are proposed to be landfarmed to reduce some of the PAHs and other pollutants and then capped with a layer of soil. This remediation program is estimated to cost on the order of $400 million (CAN). This article presents a review of the significant potential problems with the STPA proposed remediation strategy of the Sydney Tar Ponds sediments and Coke Ovens site soils. © 2006 Wiley Periodicals, Inc. 相似文献
895.
896.
M. R. Theobald U. Dragosits C. J. Place J. U. Smith M. Sozanska L. Brown D. Scholefield A. Del Prado J. Webb P. G. Whitehead A. Angus I. D. Hodge D. Fowler M. A. Sutton 《Water, Air, & Soil Pollution: Focus》2004,4(6):135-142
The distribution and impacts of different nitrogen pollutants are inextricably linked. To understand the problem fully, the interactions between the different pollutants need to be taken into account. This is particularly important when it comes to abatement techniques, since measures to reduce emissions of one nitrogen pollutant can often lead to an increase in another. This project represents a step towards greater understanding of these issues by linking together new and existing nitrogen flux models into a larger framework. The modelling framework has been constructed and some of the nitrogen flows between fields, farms and the atmosphere have been modelled for a UK study area for typical farm management scenarios. 相似文献
897.
Davey L. Jones John F. Farrar Kevin K. Newsham 《Water, Air, & Soil Pollution: Focus》2004,4(6):169-175
Amino acids constitute one of the largest inputs of organic nitrogen (N) to most polar soils and have been hypothesized to be important in regulating vegetational succession and productivity in Arctic ecosystems. Our understanding of amino acid cycling in these soils, however, is poor. The aim of this study was to investigate the size and rate of turnover of the amino acid pool in a range of Arctic and Antarctic soils. Our results indicate that in polar soils with either high or low ornithogenic inputs the amino acid pool is small in comparison to the inorganic N pool (NO–3 and NH+4). The free amino acid pool constituted only a small proportion of the total dissolved organic nitrogen (DON) pool in these soils. Here we show that these low concentrations may be due to rapid use by the soil microbial community in both Arctic and Antarctic soils. The turnover of the amino acid pool in soil was extremely rapid, with a half-life ranging from 2 to 24 h, indicating that this N pool can be turned over many hundred times each summer when polar soils are frequently unfrozen. The implications of amino acids in N cycling and plant and microbial nutrition are discussed. 相似文献
898.
Steven N. Chillrud Richard F. Bopp James M. Ross Damon A. Chaky Sidney Hemming Edward L. Shuster H. James Simpson Frank Estabrooks 《Water, Air, & Soil Pollution: Focus》2004,4(2-3):469-482
Radionuclide, radiogenic lead isotope and trace metal analyses on fine-grained sediment cores collected along 160 km of the upper and tidal Hudson River were used to examine temporal trends of contaminant loadings and to develop radiogenic lead isotopes both as a stratigraphic tool and as tracers for resolving decadal particle transport fluxes. Very large inputs of Cd, Sb, Pb, and Cr are evident in the sediment record, potentially from a single manufacturing facility. The total range in radiogenic lead isotope ratios observed in well-dated cores collected about 24 km downstream of the plant is large (e.g., maximum difference in 206Pb/207Pb is 10%), characterized by four major shifts occurring in the 1950s, 1960s, 1970s and 1980s. The upper Hudson signals in Cd and radiogenic lead isotopes were still evident in sediments collected 160 km downstream in the tidal Hudson. The large magnitude and abrupt shifts in radiogenic lead isotope ratios as a function of depth provide sensitive temporal constraints that complement information derived from radionuclide analyses to significantly improve the precision of dating assignments. Application of a simple dilution model to data from paired cores suggests much larger sediment inputs in one section of the river than previously reported, suggesting particle influxes to the Hudson have been underestimated. 相似文献
899.
Miskewitz R. J. Hires R. I. Su T. L. Korfiatis G. P. Sidhoum M. 《Water, Air, & Soil Pollution: Focus》2004,4(4-5):45-54
A 50 ha known contaminated site in Bayonne, New Jersey, U.S.A. is permitted to receive up to 3 × 106 m3 of sediment dredged from navigation channels in the New York/New Jersey Harbor. Much of the sediment is expected to contain low to moderate concentrations of industrial and agricultural chemicals, including Polychlorinated Biphenyls (PCBs). The dredged material brought to the site is stabilized with cement and then placed as a capping and grading layer. The flux of PCBs from drying stabilized dredged material has been estimated from measurements of PCB air concentrations at two heights above the ground along with micrometeorological observations. A statistically significant gradient in PCB concentrations has been consistently measured in the first 3 m above the ground. Observed PCB fluxes were highest over freshly placed stabilized dredged sediment and decreased as it cured. The highest flux observed in this study was 7214 ng/m2/h, but during subsequent sampling intervals at the same site, the flux estimates decreased by an order of magnitude over a 5-day interval. 相似文献
900.
In this investigation, all the techniques used in the chemical recycling of polyethylene terephthalate (PET) are critically reviewed according to the overall benefits together with the environmental surcharge that they cause. Those, which are consistent with the principles of sustainable development, are indicated. Experimental data are presented for the acid hydrolysis of PET and compared with previous results on the alkaline hydrolysis of PET with, or without, the use of a phase transfer catalyst. Overall material balances are carried out for the hydrolysis of PET. Finally, it can be postulated that recycling according to the scheme: is the only one within the framework of sustainable development. Therefore, the recycling of PET does not only serve as a partial solution to the solid waste problem but also contributes to the conservation of raw petrochemical products and energy. 相似文献