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111.
The effects of soil amendments on heavy metal bioavailability in two contaminated Mediterranean soils 总被引:19,自引:0,他引:19
Walker DJ Clemente R Roig A Bernal MP 《Environmental pollution (Barking, Essex : 1987)》2003,122(2):303-312
Two heavy metal contaminated calcareous soils from the Mediterranean region of Spain were studied. One soil, from the province of Murcia, was characterised by very high total levels of Pb (1572 mg kg(-1)) and Zn (2602 mg kg(-1)), whilst the second, from Valencia, had elevated concentrations of Cu (72 mg kg(-1)) and Pb (190 mg kg(-1)). The effects of two contrasting organic amendments (fresh manure and mature compost) and the chelate ethylenediaminetetraacetic acid (EDTA) on soil fractionation of Cu, Fe, Mn, Pb and Zn, their uptake by plants and plant growth were determined. For Murcia soil, Brassica juncea (L.) Czern. was grown first, followed by radish (Raphanus sativus L.). For Valencia soil, Beta maritima L. was followed by radish. Bioavailability of metals was expressed in terms of concentrations extractable with 0.1 M CaCl2 or diethylenetriaminepentaacetic acid (DTPA). In the Murcia soil, heavy metal bioavailability was decreased more greatly by manure than by the highly-humified compost. EDTA (2 mmol kg(-1) soil) had only a limited effect on metal uptake by plants. The metal-solubilising effect of EDTA was shorter-lived in the less contaminated, more highly calcareous Valencia soil. When correlation coefficients were calculated for plant tissue and bioavailable metals, the clearest relationships were for Beta maritima and radish. 相似文献
112.
Dani Degenhardt David Humphries Allan J. Cessna Paul Messing Pascal H. Badiou Renata Raina 《Journal of environmental science and health. Part. B》2013,48(7):631-639
Glyphosate [N-(phosphonomethyl)glycine] is the active ingredient of several herbicide products first registered for use in 1974 under the tradename Roundup. The use of glyphosate-based herbicides has increased dramatically over the last two decades particularly in association with the adoption of glyphosate-tolerant crops. Glyphosate has been detected in a range of surface waters but this is the first study to monitor its fate in prairie wetlands situated in agricultural fields. An ephemeral wetland (E) and a semi-permanent wetland (SP) were each divided into halves using a polyvinyl curtain. One half of each wetland was fortified with glyphosate with the added mass simulating an accidental direct overspray. Glyphosate dissipated rapidly in the water column of the two prairie wetlands studied (DT50 values of 1.3 and 4.8 d) which may effectively reduce the impact of exposure of aquatic biota to the herbicide. Degradation of glyphosate to its major metabolite aminomethylphosphonic acid (AMPA) and sorption of the herbicide to bottom sediment were more important pathways for the dissipation of glyphosate from the water column than movement of the herbicide with infiltrating water. Presently, we are not aware of any Canadian guidelines for glyphosate residues in sediment of aquatic ecosystems. Since a substantial portion of glyphosate entering prairie wetlands will become associated with bottom sediments, particularly in ephemeral wetlands, guidelines would need to be developed to assess the protection of organisms that spend all or part of their lifecycle in sediment. 相似文献
113.
K. Bruce Jones Daniel T. Heggem Timothy G. Wade Anne C. Neale Donald W. Ebert Maliha S. Nash Megan H. Mehaffey Karl A. Hermann Anthony R. Selle Scott Augustine Iris A. Goodman Joel Pedersen David Bolgrien J. Max Viger Dean Chiang Cindy J. Lin Yehong Zhong Joan Baker Rick D. Van Remortel 《Environmental monitoring and assessment》2000,64(1):227-245
The Environmental Monitoring and Assessment Program (EMAP) is proposing an ambitious agenda to assess the status of streams and estuaries in a 12-State area of the western United States by the end of 2003. Additionally, EMAP is proposing to access landscape conditions as they relate to stream and estuary conditions across the west. The goal of this landscape project is to develop a landscape model that can be used to identify the relative risks of streams and estuaries to potential declines due to watershed-scale, landscape conditions across the west. To do so, requires an understanding of quantitative relationships between landscape composition and pattern metrics and parameters of stream and estuary conditions. This paper describes a strategic approach for evaluating the degree to which landscape composition and pattern influence stream and estuary condition, and the development and implementation of a spatially-distributed, landscape analysis approach. 相似文献
114.
Browne BA Kraft GJ Bowling JM Devita WM Mechenich DJ 《Journal of environmental quality》2008,37(4):1456-1467
In this study, we used chlorofluorocarbon (CFC) age-dating to investigate the geochemistry of N enrichment within a bedrock aquifer depth profile beneath a south central Wisconsin agricultural landscape. Measurement of N(2)O and excess N(2) allowed us to reconstruct the total NO(3)(-) and total nitrogen (TN) leached to ground water and was essential for tracing the separate influences of soil nitrification and ground water denitrification in the collateral geochemical chronology. We identify four geochemical impacts due to a steady ground water N enrichment trajectory (39 +/- 2.2 micromol L(-1) yr(-1), r(2) = 0.96) over two decades (1963-1985) of rapidly escalating N use. First, as a by-product of soil nitrification, N(2)O entered ground water at a stable (r(2) = 0.99) mole ratio of 0.24 +/- 0.007 mole% (N(2)O-N/NO(3)-N). The gathering of excess N(2)O in ground water is a potential concern relative to greenhouse gas emissions and stratospheric ozone depletion after it discharges to surface water. Second, excess N(2) measurements revealed that NO(3)(-) was a prominent, mobile, labile electron acceptor comparable in importance to O(2.) Denitrification transformed 36 +/- 15 mole% (mol mol(-1) x 100) of the total N within the profile to N(2) gas, delaying exceedance of the NO(3)(-) drinking water standard by approximately 6 yr. Third, soil acids produced from nitrification substantially increased the concentrations of major, dolomitic ions (Ca, Mg, HCO(3)(-)) in ground water relative to pre-enrichment conditions. By 1985, concentrations approximately doubled; by 2006, CFC age-date projections suggest concentrations may have tripled. Finally, the nitrification induced mobilization of Ca may have caused a co-release of P from Ca-rich soil surfaces. Dissolved P increased from an approximate background value of 0.02 mg L(-1) in 1963 to 0.07 mg L(-1) in 1985. The CFC age-date projections suggest the concentration could have reached 0.11 mg L(-1) in ground water recharge by 2006. These results highlight an intersection of the N and P cycles potentially important for managing the quality of ground water discharged to surface water. 相似文献
115.
Richards RP Baker DB Crumrine JP Kramer JW Ewing DE Merryfield BJ 《Journal of environmental quality》2008,37(5):1894-1908
Sediment is an important pollutant for Lake Erie and its tributaries as a carrier of other substances and as a pollutant in its own right. Environmental managers have called for major reductions in sediment loadings in Lake Erie tributaries. In this study, 30-yr (1975-2005) datasets with daily resolution are analyzed to identify and interpret trends in sediment concentrations and loads in major US tributaries to Lake Erie. The Maumee and Sandusky Rivers in agricultural northwest Ohio show continual decreases throughout this period, but the River Raisin shows increases, especially in the last decade. The urban and forested Cuyahoga River shows little trend before 2000 but shows increases since then. The mostly forested Grand River shows strong decreases before 1995, little change thereafter until the early 2000s, and then increases. In most cases, the greatest decreases or smallest increases, depending on the river, are associated with summer and fall and with low flow conditions, whereas the smallest decreases or greatest increases are associated with the spring and with high flow conditions. Analysis of concentration-flow relationships indicates that these changes are not due to weather but reflect positive and negative anthropogenic influences. Sediment decreases in the northwestern Ohio tributaries seem to reflect the successful use of agricultural practices to reduce erosion and prevent sediment loss. Opportunities for further reductions in sediment loads and concentrations lie in better management of sediment losses during winter and spring. 相似文献
116.
Kreutzweiser DP Good KP Chartrand DT Scarr TA Thompson DG 《Journal of environmental quality》2008,37(2):639-646
The systemic insecticide imidacloprid may be applied to deciduous trees for control of the Asian longhorned beetle, an invasive wood-boring insect. Senescent leaves falling from systemically treated trees contain imidacloprid concentrations that could pose a risk to natural decomposer organisms. We examined the effects of foliar imidacloprid concentrations on decomposer organisms by adding leaves from imidacloprid-treated sugar maple trees to aquatic and terrestrial microcosms under controlled laboratory conditions. Imidacloprid in maple leaves at realistic field concentrations (3-11 mg kg(-1)) did not affect survival of aquatic leaf-shredding insects or litter-dwelling earthworms. However, adverse sublethal effects at these concentrations were detected. Feeding rates by aquatic insects and earthworms were reduced, leaf decomposition (mass loss) was decreased, measurable weight losses occurred among earthworms, and aquatic and terrestrial microbial decomposition activity was significantly inhibited. Results of this study suggest that sugar maple trees systemically treated with imidacloprid to control Asian longhorned beetles may yield senescent leaves with residue levels sufficient to reduce natural decomposition processes in aquatic and terrestrial environments through adverse effects on non-target decomposer organisms. 相似文献
117.
We compared measures of ecosystem state across six adjacent land-tenure groups in the intact tropical savanna landscapes of
northern Australia. Tenure groups include two managed by Aboriginal owners, two national parks, a cluster of pastoral leases,
and a military training area. This information is of relevance to the debate about the role of indigenous lands in the Australian
conservation estate. The timing and frequency of fire was determined by satellite imagery; the biomass and composition of
the herb-layer and the abundance of large feral herbivores by field surveys; and weediness by analysis of a Herbarium database.
European tenures varied greatly in fire frequencies but were consistently burnt earlier in the dry season than the two Aboriginal
tenures, the latter having intermediate fire frequencies. Weeds were more frequent in the European tenures, whilst feral animals
were most abundant in the Aboriginal tenures. This variation strongly implies a signature of current management and/or recent
environmental history. We identify indices suitable for monitoring of management outcomes in an extensive and sparsely populated
landscape. Aboriginal land offers a unique opportunity for the conservation of biodiversity through the maintenance of traditional
fire regimes. However, without financial support, traditional practices may prove unsustainable both economically and because
exotic weeds and feral animals will alter fire regimes. An additional return on investment in Aboriginal land management is
likely to be improved livelihoods and health outcomes for these disadvantaged communities. 相似文献
118.
We demonstrate an approach for evaluating the level of protection attained using a variety of forms and levels of past, current,
and proposed Air Quality Standards (AQSs). The U.S. Clean Air Act requires the establishment of ambient air quality standards
to protect health and public welfare. However, determination of attainment of these standards is based on ambient pollutant
concentrations rather than prevention of adverse effects. To determine if a given AQS protected against adverse effects on
vegetation, hourly ozone concentrations were adjusted to create exposure levels that “just attain” a given standard. These
exposures were used in combination with a physiologically-based tree growth model to account for the interactions of climate
and ozone. In the evaluation, we used ozone concentrations from two 6-year time periods from the San Bernardino Mountains
in California. There were clear differences in the level of vegetation protection achieved with the various AQSs. Based on
modeled plant growth, the most effective standards were the California 8-hr average maximum of 70 ppb and a seasonal, cumulative,
concentration-weighted index (SUM06), which if attained, resulted in annual growth reductions of 1% or less. Least effective
was the 1-hr maximum of 120 ppb which resulted in a 7% annual reduction. We conclude that combining climate, exposure scenarios,
and a process-based plant growth simulator was a useful approach for evaluating effectiveness of current or proposed air quality
standards, or evaluating the form and/or level of a standard based on preventing adverse growth effects. 相似文献
119.
Snowmobile use in Yellowstone National Park has been shown to impact air quality, with implications for the safety and welfare
of Park staff and other Park resource values. Localized impacts have been documented at several high-use sites in the Park,
but the broader spatial variability of snowmobile emissions and air quality was not understood. Measurements of 87 volatile
organic compounds (VOCs) were made for ambient air sampled across the Park and West Yellowstone, Montana, during 2 days of
the 2002–2003 winter use season, 1 year before the implementation of a new snowmobile policy. The data were compared with
similar data from pristine West Coast sites at similar latitudes. Backward trajectories of local air masses, alkyl nitrate-parent
alkane ratios, and atmospheric soundings were used to identify the VOC sources and assess their impact. Different oversnow
vehicle types used in the Park were sampled to determine their relative influence on air mass pollutant composition. VOCs
were of local origin and demonstrated strong spatiotemporal variability that is primarily influenced by levels of snowmobile
traffic on given road segments at different times of day. High levels of snowmobile traffic in and around West Yellowstone
produced consistently high levels of benzene, toluene, and carbon monoxide. 相似文献
120.
Perceiving the Environment from the Lay Perspective in Desertified Areas,Northern China 总被引:1,自引:0,他引:1
Investigating local people’s environmental perceptions can produce useful information that could be incorporated into decision
making processes that help resolve environmental problems. Although China is undergoing severe desertification, the perceptions
of the local people toward their degraded environment and the related issues have so far not been actively solicited. This
article, which is a supplement to Lee and Zhang’s (2004, 2005) studies, seeks to further investigate the lay public’s general environmental attitudes, perceptions of desertification, interpretations
of land-degrading activities, and particularly their interrelations in severely desertified areas. Minqin County in Gansu
Province, northern China, was chosen to be the study area. Data was collected via a questionnaire survey (n = 1138) administered in December 2002. Major findings were: (1) Most respondents had only weak altruistic environmental attitudes,
with educational level to be a significant determinant. (2) Respondents’ perceptions of desertification and interpretations
of land-degrading activities were contingent on personal attributes, general environmental attitudes, and other conceptions
related to desertification. It is recommended that the interrelations between the various aspects of the public’s environmental
perceptions should be thoroughly examined to facilitate their participation in environmental management. 相似文献