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111.
112.
Givens ML Small CM Terrell ML Cameron LL Michels Blanck H Tolbert PE Rubin C Henderson AK Marcus M 《Chemosphere》2007,69(8):1295-1304
Understanding the influence of maternal exposures on gestational age and birth weight is essential given that pre-term and/or low birth weight infants are at risk for increased mortality and morbidity. We performed a retrospective analysis of a cohort exposed to polybrominated biphenyls (PBB) through accidental contamination of cattle feed and polychlorinated biphenyls (PCB) through residual contamination in the geographic region. Our study population consisted of 444 mothers and their 899 infants born between 1975 and 1997. Using restricted maximum likelihood estimation, no significant association was found between estimated maternal serum PBB at conception or enrollment PCB levels and gestational age or infant birth weight in unadjusted models or in models that adjusted for maternal age, smoking, parity, infant gender, and decade of birth. For enrollment maternal serum PBB, no association was observed for gestational age. However, a negative association with high levels of enrollment maternal serum PBB and birth weight was suggested. We also examined the birth weight and gestational age among offspring of women with the highest (10%) PBB or PCB exposure, and observed no significant association. Because brominated compounds are currently used in consumer products and therefore, are increasingly prevalent in the environment, additional research is needed to better understand the potential relationship between in utero exposure to brominated compounds and adverse health outcomes. 相似文献
113.
Waldner P Schaub M Graf Pannatier E Schmitt M Thimonier A Walthert L 《Environmental monitoring and assessment》2007,128(1-3):5-17
Air pollution affects forest health through atmospheric deposition of acidic and nitrogen compounds and elevated levels of
tropospheric ozone (O3). In 1985, a monitoring network was established across Europe and various research efforts have since been undertaken to
define critical values. We measured atmospheric deposition of acidity and nitrogen as well as ambient levels of O3 on 12, 13, and 14 plots, respectively, in the framework of the Swiss Long-Term Forest Ecosystem Research (LWF) in the period
from 1995 to 2002. We estimated the critical loads of acidity and of nitrogen, using the steady state mass balance approach,
and calculated the critical O3 levels using the AOT40 approach. The deposition of acidity exceeded the critical loads on 2 plots and almost reached them
on 4 plots. The median of the measured molar ratio of base nutrient cations to total dissolved aluminium (Bc/Al) in the soil
solution was higher than the critical value of 1 for all depths, and also at the plots with an exceedance of the critical
load of acidity. For nitrogen, critical loads were exceeded on 8 plots and deposition likely represents a long-term ecological
risk on 3 to 10 plots. For O3, exceedance of critical levels was recorded on 12 plots, and led to the development of typical O3-induced visible injury on trees and shrubs, but not for all plots due to (1) the site specific composition of O3 sensitive and tolerant plant species, and (2) the influence of microclimatic site conditions on the stomatal behaviour, i.e.,
O3 uptake. 相似文献
114.
Thu Nguyen Marcus Hilliard Gary T. Rochelle 《International Journal of Greenhouse Gas Control》2010,4(5):707-715
Amine volatility is a key screening criterion for amines to be used in CO2 capture. Excessive volatility may result in significant economic losses and environmental impact. It also dictates the capital cost of the water wash. This paper reports measured amine volatility in 7 m MEA (monoethanolamine), 8 m PZ (piperazine), 7 m MDEA (n-methyldiethanolamine)/2 m PZ (piperazine), 12 m EDA (ethylenediamine), and 5 m AMP (2-amino-2-methyl-1-propanol) at 40–60 °C with lean and rich loadings giving CO2 partial pressures of 0.5 and 5 kPa at 40 °C. The amine concentrations were chosen to maximize CO2 capture capacity at acceptable viscosity. At the lean loading condition (where volatility is of greatest interest), the amines are ranked in order of increasing volatility: 7 m MDEA/2 m PZ (6/2 ppm), 8 m PZ (8 ppm), 12 m EDA (9 ppm), 7 m MEA (31 ppm), and 5 m AMP (112 ppm). The apparent amine partial molar excess enthalpies in these systems were estimated to range from ~10 to 87 kJ/mol of amine. 相似文献
115.
Richard R. Marcus Stephen Kiebzak 《Journal of the American Water Resources Association》2008,44(6):1578-1590
Abstract: Alabama is a water rich state. Yet, agriculture is limited in both scale and productivity and the state regularly suffers from drought. Climate variability adds to this paradox even while water users, particularly farmers, have few coping mechanisms. In this paper, we argue that more significant than the water resource itself in Alabama is the governance structure of that resource. The riparian doctrine, as it stands, stymies effective management. The role of water doctrines, and resultant policy, is, therefore, crucial to enhancing decision‐making opportunities for agricultural end‐users in Alabama. After exploring different doctrine types as applied across the states we conclude that a move towards “regulated riparianism” consistent with the American Society of Civil Engineers Regulated Riparian Water Code (2004) would enhance opportunities for both the state and agriculturalists to cope with variable water supply conditions while maximizing environmental benefits. The paper then concludes with a review of the primary objectives of the Water Code and key places where Alabama’s Water Code would need revision to meet these objectives. 相似文献
116.
Severo Amanda M. C. Nicácio Pedro H. M. Fook Marcus Vinícius Lia Wellen Renate M. R. 《Journal of Polymers and the Environment》2022,30(9):4014-4022
Journal of Polymers and the Environment - Epoxidized soybean oil (ESO) compounds were cured with methyl tetrahydrophthalic anhydride (MTHPA) as hardener and 2,4,6-tris (dimethylaminomethyl) phenol... 相似文献
117.
Han Zhu Marcus O. Letzel Martin Reiser Martin Kranert Wolfgang Bächlin Thomas Flassak 《Waste management (New York, N.Y.)》2013,33(12):2713-2719
Methane emission monitoring has become increasingly essential for diffusive area sources, especially for landfills, which contribute to a significant fraction of the total anthropogenic methane emission globally. Statutorily, methane emission rate from landfills in Germany shall be examined on a semiannual basis; however, an appropriate approach has yet to be developed and adopted for general use. In this study, a new method is proposed based on experimental results, which utilizes a TDLAS (Tunable Diode Laser Absorption Spectroscopy) instrument – GasFinder2.0® system and a dispersion model LASAT (Lagrangian Simulation of Aerosol Transport) as the measurement device and calculation model, respectively. Between April 2010 and December 2011, a research project was conducted at a pilot scale landfill in the south of Germany. Drawing on the extensive research into this pilot project, an effective strategy of measurement setup was determined. Methane concentration was measured with GasFinder2.0® system in the upstream and downstream sections of the project site, while wind and turbulence data were measured simultaneously by an ultrasonic anemometer. The average methane emission rate from the source can be calculated by using the results as input data in the dispersion model. With this method, site-specific measurement approaches can be designed for not only landfills, but also different diffusive area sources with less workload and lower cost compared to conventional FID (Flame Ionization Detector) method. 相似文献
118.
Schaldach Rüdiger Meurer Katharina H. E. Jungkunst Hermann F. Nendel Claas Lakes Tobia Gollnow Florian Göpel Jan Boy Jens Guggenberger Georg Strey Robert Strey Simone Berger Thomas Gerold Gerhard Schönenberg Regine Böhner Jürgen Schindewolf Marcus Latynskiy Evgeny Hampf Anna Parker Phillip S. Sentelhas Paulo César 《Regional Environmental Change》2018,18(1):161-173
Regional Environmental Change - This article describes the design of a new model-based assessment framework to identify and analyse possible future trajectories of agricultural development and... 相似文献
119.
Marcus C. Sarofim 《Environmental Modeling and Assessment》2012,17(3):231-239
The Global Temperature Potential (GTP) has recently been proposed as an alternative to the Global Warming Potential (GWP).
Using two different Earth Models of Intermediate Complexity, we show that the solution to the 100-year sustained GTP for methane
is significantly larger than the equivalent GWP due to the inclusion of future changes in greenhouse gas concentrations in
the reference scenario and different atmospheric chemistry assumptions. This result suggests that methane reductions may be
undervalued when using GWPs, but the policy implications depend on how the objectives of greenhouse gas policy are defined. 相似文献
120.
L. F. Jô R. Marcus O. Marcelin 《Environmental science and pollution research international》2014,21(11):6975-6981
The recycling of nitric acid and copper nitrate contained in an industrial effluent was studied. The experiments conducted on such a medium showed that the presence of copper nitrate significantly improves nitric acid-water separation during distillation in an azeotropic medium. At the temperature of the azeotrope, however, this metal salt starts to precipitate, making the medium pasty, thus inhibiting the nitric acid extraction process. The optimisation of parameters such as column efficiency and adding water to the boiler at the azeotrope temperature are recommended in this protocol in order to collect the various components while avoiding the formation of by-products: NOx compounds. Thus, the absence of column, along with the addition of a small volume of water at a temperature of 118 °C, significantly increases the yield, allowing 94 % nitric acid to be recovered at the end of the process, along with the residual copper nitrate. The resulting distillate, however, is sufficiently dilute to not be used as is. Rectification is required to obtain concentrated nitric acid at 15 mol·l?1, along with a weakly acidic distillate from the distillation front. This latter is quenched using potassium hydroxide and is used as a fertiliser solution for horticulture or sheltered market gardening. This process thus allows complete recycling of all the medium’s components, including that of the distillate resulting from the nitric acid rectification operation. 相似文献