全文获取类型
收费全文 | 424篇 |
免费 | 16篇 |
国内免费 | 188篇 |
专业分类
安全科学 | 21篇 |
废物处理 | 21篇 |
环保管理 | 40篇 |
综合类 | 239篇 |
基础理论 | 82篇 |
污染及防治 | 175篇 |
评价与监测 | 25篇 |
社会与环境 | 8篇 |
灾害及防治 | 17篇 |
出版年
2023年 | 6篇 |
2022年 | 21篇 |
2021年 | 16篇 |
2020年 | 14篇 |
2019年 | 12篇 |
2018年 | 16篇 |
2017年 | 19篇 |
2016年 | 20篇 |
2015年 | 30篇 |
2014年 | 30篇 |
2013年 | 51篇 |
2012年 | 36篇 |
2011年 | 45篇 |
2010年 | 33篇 |
2009年 | 22篇 |
2008年 | 35篇 |
2007年 | 32篇 |
2006年 | 23篇 |
2005年 | 13篇 |
2004年 | 13篇 |
2003年 | 12篇 |
2002年 | 21篇 |
2001年 | 11篇 |
2000年 | 13篇 |
1999年 | 13篇 |
1998年 | 12篇 |
1997年 | 20篇 |
1996年 | 17篇 |
1995年 | 6篇 |
1994年 | 2篇 |
1993年 | 1篇 |
1992年 | 4篇 |
1991年 | 4篇 |
1988年 | 1篇 |
1987年 | 1篇 |
1986年 | 2篇 |
1984年 | 1篇 |
排序方式: 共有628条查询结果,搜索用时 281 毫秒
431.
在连续运行条件下,采用水平潜流人工湿地净化低浓度的生活污水,考察了其净化效果。结果表明,该系统能够有效的降低生活污水中的COD、TN、TP,适合于城镇生活污水的处理。在0.1、0.2 m3/(m2.d)的水力负荷条件下,系统较容易出现死水区;当0.3 m3/(m2·d)的水力负荷条件下,水流呈推流状态,有效容积和水力效率得到提高,去除率分别为90.3%、86.6%和96.7%。试验表明,适当增加水力负荷,有利于污染物的去除。 相似文献
432.
Li Chen Yuming Wang Peiwu Li Yaqin Ji Shaofei Kong Zhiyong Li Zhipeng Bai 《环境科学学报(英文版)》2012,24(7):1251-1258
Advancing the understanding of the spatial aspects of air pollution in the city regional environment is an area where improved methods can be of great benefit to exposure assessment and policy support. We created land use regression (LUR) models for SO2, NO2 and PM10 for Tianjin, China. Traffic volumes, road networks, land use data, population density, meteorological conditions, physical conditions and satellite-derived greenness, brightness and wetness were used for predicting SO2, NO2 and PM10 concentrations. We incorporated data on industrial point sources to improve LUR model performance. In order to consider the impact of different sources, we calculated the PSIndex, LSIndex and area of different land use types (agricultural land, industrial land, commercial land, residential land, green space and water area) within different buffer radii (1 to 20 km). This method makes up for the lack of consideration of source impact based on the LUR model. Remote sensing-derived variables were significantly correlated with gaseous pollutant concentrations such as SO2 and NO2. R2 values of the multiple linear regression equations for SO2, NO2 and PM10 were 0.78, 0.89 and 0.84, respectively, and the RMSE values were 0.32, 0.18 and 0.21, respectively. Model predictions at validation monitoring sites went well with predictions generally within 15% of measured values. Compared to the relationship between dependent variables and simple variables (such as traffic variables or meteorological condition variables), the relationship between dependent variables and integrated variables was more consistent with a linear relationship. Such integration has a discernable influence on both the overall model prediction and health effects assessment on the spatial distribution of air pollution in the city region. 相似文献
433.
Mingqiang Huang Weijun Zhang Liqing Hao Zhenya Wang Li Fang Ruihong Kong Xiaobin Shan Fuyi Liu Liusi Sheng 《环境科学学报(英文版)》2010,22(10):1570-1575
Smog chamber experiments were performed to investigate the composition of products formed from photooxidation of aromatic
hydrocarbon ethylbenzene. Vacuum ultraviolet photoionization mass spectrometer and aerosol time-of-flight mass spectrometer were
used to measure the products in the gas and particle phases in real-time. Experimental results demonstrated that ethylphenol,
methylglyoxal, phenol, benzaldehyde, and 2-ethylfurane were the predominant photooxidation products in both the gas and particle
phases. However, there were some di erences between detected gas phase products and those of particle phase, for example,
2-ethylfurane, ethylglyoxylic acid, nitroethylbenzene, 3,4-dioxopentanal and ethyl-nitrophenol were only existing in the particle-phase.
The possible reaction mechanisms leading to these products were also discussed and proposed. 相似文献
434.
Li Chen Zhipeng Bai Shaofei Kong Bin Han Yan You Xiao Ding Shiyong Du Aixia Liu 《环境科学学报(英文版)》2010,22(9):1364-1373
Land use regression (LUR) model was employed to predict the spatial concentration distribution of NO2 and PM10 in the Tianjin
region based on the environmental air quality monitoring data. Four multiple linear regression (MLR) equations were established based
on the most significant variables for NO2 in heating season (R2 = 0.74), and non-heating season (R2 = 0.61) in the whole study area;
and PM10 in heating season (R2 = 0.72), and non-heating season (R2 = 0.49). Maps of spatial concentration distribution for NO2 and
PM10 were obtained based on the MLR equations (resolution is 10 km). Intercepts of MLR equations were 0.050 (NO2, heating season),
0.035 (NO2, non-heating season), 0.068 (PM10, heating season), and 0.092 (PM10, non-heating season) in the whole study area. In the
central area of Tianjin region, the intercepts were 0.042 (NO2, heating season), 0.043 (NO2, non-heating season), 0.087 (PM10, heating
season), and 0.096 (PM10, non-heating season). These intercept values might imply an area’s background concentrations. Predicted
result derived from LUR model in the central area was better than that in the whole study area. R2 values increased 0.09 (heating
season) and 0.18 (non-heating season) for NO2, and 0.08 (heating season) and 0.04 (non-heating season) for PM10. In terms of R2,
LUR model performed more e ectively in heating season than non-heating season in the study area and gave a better result for NO2
compared with PM10. 相似文献
435.
In China, the health risk from overexposure to particles is becoming an important public health concern. To investigate daily exposure characteristics to PM 2.5 with high ambient concentration in urban area, a personal exposure study was conducted for school children, and office workers in Beijing, China. For all participants (N = 114), the mean personal 24-hr exposure concentration was 102.5, 14.7, 0.093, 0.528, 0.934, 0.174 and 0.703 μg/m 3 for PM 2.5 , black carbon, Mn, Al, Ca, Pb, and Fe. Children's exposure concentrations of PM 2.5 were 4-5 times higher than those in related studies. The ambient concentration of PM 2.5 (128.5 μg/m 3 ) was significantly higher than the personal exposure concentration (P 0.05), and exceed the reference concentration (25 μg/m 3 ) of WHO air quality guideline. Good correlation relationships and significant differences were identified between ambient concentration and personal exposure concentration. The relationships indicate that the ambient concentration is the main factor influencing personal exposure concentration, but is not a good indicator of personal exposure concentration. Outdoor activities (commute mode, exposure to heating, workday or weekend travel) influenced personal exposure concentrations significantly, but the magnitude of the influence from indoor activities (exposure to cooking) was masked by the high ambient concentrations. 相似文献
436.
437.
Distribution of polycyclic aromatic hydrocarbons in Datuo karst Tiankeng of South China 总被引:2,自引:0,他引:2
Theodore OI Qi S Kong X Liu H Li J Li J Wang X Wang Y 《Environmental geochemistry and health》2008,30(5):423-429
Levels of polycyclic aromatic hydrocarbons (PAHs) were measured in surface soils of Datuo karst Tiankeng (large sinkholes) in South China with the use of a gas chromatography-mass spectroscopy (GC-MS) system. This paper provides data on the levels and distribution of PAHs from the top to the bottom of the Datuo karst Tiankeng. The results showed that the sum of the 16 EPA priority PAHs from the sampled locations from top to bottom had a relative increment in PAHs concentration. summation operatorPAHs ranged from 16.93 ng/g to 68.07 ng/g with a mean concentration of 42.15 ng/g. The correlated results showed the bottom of the large sinkhole, which accounts for the higher concentrations, probably acts like a trap for the PAHs. Thus, the low evaporation rate at the bottom may play a key role in controlling the high concentration of PAHs at the bottom. 相似文献
438.
Joo-Ae Kim Mihye Kong Ji-Ho Kim Kang-Sup Chung Chi-Yong Eom Hye-On Yoon 《Environmental geochemistry and health》2013,35(3):311-315
Lithium manganese oxide–based adsorbents have been developed for the recovery of lithium from seawater. To maximize the recovery efficiency, it is important to prevent microfouling of lithium adsorbents by marine bacteria. To identify the marine bacteria that cause biofouling against the lithium adsorbents, lithium adsorbents were installed into a non-coated frame or a frame coated with an antifouling agent soaked in seawater. Microorganisms from the surface of lithium adsorbents were collected for 30 days at 10-day intervals, cultured in marine broth, isolated, and identified by 16S rDNA sequencing. Pseudoalteromonas and Vibrio were constituted to 35.6 and 28.8 % of total isolates, respectively, and were predominant in the non-coated frame, whereas Vibrio was poorly isolated (2.3 %) from the antifouling agent–coated frame. In this study, antifouling strategy for maximum lithium recovery efficiency in the marine area takes account of Pseudoalteromonas and Vibrio. 相似文献
439.
440.