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51.
Lutz Ahrens Merle Plassmann Zhiyong Xie Ralf Ebinghaus 《Frontiers of Environmental Science & Engineering》2009,3(2):152-170
The distribution of polyfluoroalkyl compounds (PFCs) in the dissolved and particulate phase and their discharge from the river Elbe into the North Sea were studied. The PFCs quantified included C4-C8 perfluorinated sulfonates (PFSAs), 6:2 fluorotelomer sulfonate (6:2 FTS), C6 and C8 perfluorinated sulfinates (PFSiAs), C4-C12 perfluorinated carboxylic acids (PFCAs), perfluoro-3,7-dimethyl-octanoic acid (3,7m2-PFOA), perfluorooctane sulfonamide (FOSA), and n-ethyl perfluroctane sulfonamidoethanol (EtFOSE). PFCs were mostly distributed in the dissolved phase, where perfluorooctanoic acid (PFOA) dominated with 2.9–12.5 ng/L. In the suspended particulate matter FOSA and perfluorooctane sulfonate (PFOS) showed the highest concentrations (4.0 ng/L and 2.3 ng/L, respectively). The total flux of ΣPFCs from the river Elbe was estimated to be 802 kg/year for the dissolved phase and 152 kg/year for the particulate phase. This indicates that the river Elbe acts as a source of PFCs into the North Sea. However, the concentrations of perfluorobutane sulfonate (PFBS) and perfluorobutanoic acid (PFBA) in the North Sea were higher than that in the river Elbe, thus an alternative source must exist for these compounds. 相似文献
52.
Strutz Tessa J. Hornbruch Götz Dahmke Andreas Köber Ralf 《Environmental science and pollution research international》2016,23(17):17200-17209
Environmental Science and Pollution Research - Nanoscale zero-valent iron (NZVI) particles can be used for in situ groundwater remediation. The spatial particle distribution plays a very important... 相似文献
53.
Martin Volk Sven Lautenbach Hedwig van Delden Lachlan T. H. Newham Ralf Seppelt 《Environmental management》2010,46(6):834-849
This article analyses the benefits and shortcomings of the recently developed decision support systems (DSS) FLUMAGIS, Elbe-DSS,
CatchMODS, and MedAction. The analysis elaborates on the following aspects: (i) application area/decision problem, (ii) stakeholder
interaction/users involved, (iii) structure of DSS/model structure, (iv) usage of the DSS, and finally (v) most important
shortcomings. On the basis of this analysis, we formulate four criteria that we consider essential for the successful use
of DSS in landscape and river basin management. The criteria relate to (i) system quality, (ii) user support and user training,
(iii) perceived usefulness and (iv) user satisfaction. We can show that the availability of tools and technologies for DSS
in landscape and river basin management is good to excellent. However, our investigations indicate that several problems have
to be tackled. First of all, data availability and homogenisation, uncertainty analysis and uncertainty propagation and problems
with model integration require further attention. Furthermore, the appropriate and methodological stakeholder interaction
and the definition of ‘what end-users really need and want’ have been documented as general shortcomings of all four examples
of DSS. Thus, we propose an iterative development process that enables social learning of the different groups involved in
the development process, because it is easier to design a DSS for a group of stakeholders who actively participate in an iterative
process. We also identify two important lines of further development in DSS: the use of interactive visualization tools and
the methodology of optimization to inform scenario elaboration and evaluate trade-offs among environmental measures and management
alternatives. 相似文献
54.
55.
Richard Iannone Ralf Koppmann Jochen Rudolph 《Atmospheric environment (Oxford, England : 1994)》2010,44(34):4135-4141
The stable-carbon kinetic isotope effects (KIEs) associated with the production of methacrolein (MACR) and methyl vinyl ketone (MVK) from the reactions of isoprene with ozone and OH radicals were studied in a 25 L reaction chamber at (298±2) K and ambient pressure. The time dependence of both the stable-carbon isotope ratios and the concentrations was determined using a gas chromatography combustion isotope ratio mass spectrometry (GCC-IRMS) system. The average yields of 13C-containing MACR and MVK generated from the ozone reaction of 13C-containing isoprene differed by ?3.6‰ and ?4.5‰, respectively, from the yields for MACR and MVK containing only 12C. For MACR and MVK generated from the OH-radical oxidation of isoprene the corresponding values were ?3.8‰ and ?2.2‰, respectively. These values indicate a significant depletion in the 13C abundance of MACR and MVK upon their formation relative to isoprene’s pre-reaction 13C/12C ratio, which is supported by theoretical interpretations of the oxidation mechanism of isoprene and its 13C-substituted isotopomers. Numerical model calculations of the isoprene + O3 reaction predicted a similar depletion in 13C for both reaction products upon production. Furthermore, the model predicts mixing ratios and stable carbon delta values for isoprene, MACR, and MVK that were in agreement with the experimental results. The combined knowledge of isotope enrichment values with KIEs will reduce uncertainties in determinations of the photochemical histories of isoprene, MACR, and MVK in the troposphere. The studies presented here were conducted with using isoprene without any artificial isotope enrichment or depletion and it is therefore very likely that these results are directly applicable to the interpretation of studies of isoprene oxidation using stable carbon isotope ratio measurements. 相似文献
56.
57.
Koffi T. Tassou Ralf Schulz 《Environmental science and pollution research international》2013,20(6):3735-3742
A few studies reporting the effects of tebufenozide, a non-steroidal ecdysone agonist that mimics natural moulting hormones in chironomids exist in the literature. However, nothing is known about its chronic or multigenerational effects on the reproduction of aquatic insects, although tebufenozide is present in aquatic ecosystems. Here, we investigated the chronic toxicity of tebufenozide in two successive generations of Chironomus riparius using nominal concentrations that ranged from 4 to 26.2 μg/L. We started the test from the first instar larvae in the parental (P) generation, quantifying life cycle parameters (emergence, sex ratio, development rate, fecundity and fertility) until the emergence in the subsequent F1 generation. Results showed a reduction in reproduction and a significant decrease in male developmental rate of midges for all treatments, in the F1 generation compared with the P generation (paired t?test; p?<?0.001). Two-way analysis of variance revealed a significant exposure?×?generation effect on male fraction with male fraction increasing (P generation) or decreasing (F1 generation) with increasing exposure. These effects on C. riparius underline the importance of conducting long-term studies with environmentally relevant concentrations to investigate population-level endpoints for endocrine disrupting chemicals. 相似文献
58.
59.
Atmospheric concentrations and air-sea exchanges of nonylphenol, tertiary octylphenol and nonylphenol monoethoxylate in the North Sea 总被引:1,自引:0,他引:1
Xie Z Lakaschus S Ebinghaus R Caba A Ruck W 《Environmental pollution (Barking, Essex : 1987)》2006,142(1):170-180
Concentrations of nonylphenol isomers (NP), tertiary octylphenol (t-OP) and nonylphenol monoethoxylate isomers (NP1EO) have been simultaneously determined in the sea water and atmosphere of the North Sea. A decreasing concentration profile appeared following the distance increasing from the coast to the central part of the North Sea. Air-sea exchanges of t-OP and NP were estimated using the two-film resistance model based upon relative air-water concentrations and experimentally derived Henry's law constant. The average of air-sea exchange fluxes was -12+/-6 ng m(-2)day(-1) for t-OP and -39+/-19 ng m(-2)day(-1) for NP, which indicates a net deposition is occurring. These results suggest that the air-sea vapour exchange is an important process that intervenes in the mass balance of alkylphenols in the North Sea. 相似文献
60.
Think globally, act locally'? Climate change and public participation in Manchester and Frankfurt 总被引:1,自引:0,他引:1
'Think Globally, Act Locally' was one of the most famous slogans of the 1970s environmental movement. Discourses about global climate change are now a vivid illustration of this new 'global thinking'. Although there is a substantial amount of research about global environmental issues and policy initiatives, there is still a gap in understanding of how lay publics actually comprehend global climate change. Using qualitative research method, this study is a comparison of how lay publics in Frankfurt (Germany) and Manchester (UK) perceive these issues and the possible solutions. The study found strong similarities in lay public perceptions in both cities including that (1) awareness of global environmental issues is always contextualised in broader perspectives not exclusively 'environmental', (2) there is a shared and strong sense of global equity based on recognition of differences and (3) there is an ambivalence about the role of environmental 'information'. Differences between lay public perceptions in Manchester and Frankfurt can be explained by specific features of national cultures. 相似文献