全文获取类型
收费全文 | 3372篇 |
免费 | 167篇 |
国内免费 | 1013篇 |
专业分类
安全科学 | 249篇 |
废物处理 | 197篇 |
环保管理 | 287篇 |
综合类 | 1733篇 |
基础理论 | 557篇 |
环境理论 | 1篇 |
污染及防治 | 1103篇 |
评价与监测 | 185篇 |
社会与环境 | 104篇 |
灾害及防治 | 136篇 |
出版年
2024年 | 8篇 |
2023年 | 52篇 |
2022年 | 158篇 |
2021年 | 165篇 |
2020年 | 123篇 |
2019年 | 124篇 |
2018年 | 116篇 |
2017年 | 157篇 |
2016年 | 179篇 |
2015年 | 185篇 |
2014年 | 259篇 |
2013年 | 316篇 |
2012年 | 295篇 |
2011年 | 313篇 |
2010年 | 253篇 |
2009年 | 223篇 |
2008年 | 226篇 |
2007年 | 207篇 |
2006年 | 193篇 |
2005年 | 141篇 |
2004年 | 104篇 |
2003年 | 102篇 |
2002年 | 102篇 |
2001年 | 71篇 |
2000年 | 67篇 |
1999年 | 65篇 |
1998年 | 56篇 |
1997年 | 62篇 |
1996年 | 39篇 |
1995年 | 39篇 |
1994年 | 29篇 |
1993年 | 24篇 |
1992年 | 29篇 |
1991年 | 12篇 |
1990年 | 21篇 |
1989年 | 13篇 |
1988年 | 5篇 |
1987年 | 5篇 |
1986年 | 3篇 |
1985年 | 2篇 |
1984年 | 1篇 |
1983年 | 1篇 |
1982年 | 2篇 |
1981年 | 3篇 |
1958年 | 2篇 |
排序方式: 共有4552条查询结果,搜索用时 281 毫秒
101.
Guanglong Pang Donghui Wang Yunhong Zhang Chunyan Ma Zhengping Hao 《Frontiers of Environmental Science & Engineering》2016,10(3):447-457
MnO2 microspheres with various surface structures were prepared using the hydrothermal method, and Au/MnO2 catalysts were synthesized using the sol-gel method. We obtained three MnO2 microspheres and Au/MnO2 samples: coherent solid spheres covered with wire-like nanostructures, solid spheres with nanosheets, and hierarchical hollow microspheres with nanoplatelets and nanorods. We investigated the properties and catalytic activities of formaldehyde oxidation at room temperature. Crystalline structures of MnO2 are the main factor affecting the catalytic activities of these samples, and γ-MnO2 shows high catalytic performance. The excellent redox properties are responsible for the catalytic ability of γ-MnO2. The gold-supported interaction can change the redox properties of catalysts and accelerate surface oxygen species transition, which can account for the catalytic activity enhancement of Au/MnO2. We also studied intermediate species. The dioxymethylene (DOM) and formate species formed on the catalyst surface were considered intermediates, and were ultimately transformed into hydrocarbonate and carbonate and then decomposed into CO2. A proposed mechanism of formaldehyde oxidation over Au/MnO2 catalysts was also obtained. 相似文献
102.
高层建筑竖井火灾中影响因素众多,并且各因素对高层楼梯井火灾中重要现象、关键数值等的影响大小不一,使得此类火灾中的实验或理论研究成本较高。通过建立全局敏感性分析平台,定量考察了高层楼梯井结构所涉及因素的影响大小,并能够方便地筛选掉对所考察量影响较小的因素,以降低实验或计算成本。使用数值模拟方法,通过CFD软件对包含阶梯几何框架的高层楼梯井结构火灾进行了共计60次工况计算。并且根据计算结果,使用全局参数敏感性分析方法,得出建筑尺寸、热释放速率、环境参数对高层楼梯井内烟气湍流特性及输运特性的敏感性排序。结果表明,火源热释放速率对各输出参数的影响均占38%以上。 相似文献
103.
Li-Ming Shao Zhong-He Ma Hua Zhang Dong-Qing Zhang Pin-Jing He 《Waste management (New York, N.Y.)》2010,30(7):1165-1170
Bio-drying can enhance the sortability and heating value of municipal solid waste (MSW), consequently improving energy recovery. Bio-drying followed by size sorting was adopted for MSW with high water content to improve its combustibility and reduce potential environmental pollution during the follow-up incineration. The effects of bio-drying and waste particle size on heating values, acid gas and heavy metal emission potential were investigated. The results show that, the water content of MSW decreased from 73.0% to 48.3% after bio-drying, whereas its lower heating value (LHV) increased by 157%. The heavy metal concentrations increased by around 60% due to the loss of dry materials mainly resulting from biodegradation of food residues. The bio-dried waste fractions with particle size higher than 45 mm were mainly composed of plastics and papers, and were preferable for the production of refuse derived fuel (RDF) in view of higher LHV as well as lower heavy metal concentration and emission. However, due to the higher chlorine content and HCl emission potential, attention should be paid to acid gas and dioxin pollution control. Although LHVs of the waste fractions with size <45 mm increased by around 2× after bio-drying, they were still below the quality standards for RDF and much higher heavy metal pollution potential was observed. Different incineration strategies could be adopted for different particle size fractions of MSW, regarding to their combustibility and pollution property. 相似文献
104.
Małgorzata Mędyk Bommanna Loganathan Leszek Bielawski 《Journal of environmental science and health. Part. B》2013,48(12):831-839
AbstractAnalysis of inorganic and organic contaminants in foodstuffs aids in understanding the human exposure to these compounds via consumption. In this study, an edible mushroom species (Leccinum scabrum) and top soil samples were analysed for essential and toxic substances including phosphorus and inorganic elements over a period of three fruiting seasons. Analysis of silver (Ag), aluminium (Al), barium (Ba), calcium (Ca), cadmium (Cd), cobalt (Co), copper (Cu), iron (Fe), mercury (Hg), potassium (K), magnesium (Mg), manganese (Mn), sodium (Na), nickel (Ni), phosphorus (P), lead (Pb), rubidium (Rb), strontium (Sr) and zinc (Zn) in mushrooms and topsoil were performed using inductively coupled plasma optical emission spectroscopy (ICP-OES) with ultrasonic cross flow nebulizer. Total mercury was determined by cold-vapour atomic absorption spectroscopy (CV-AAS). The results exhibited wide variation in concentrations of metals between soil and mushroom (cap and stipes) during three fruiting seasons. Positive bioconcentration factors (BFCs) indicate on bioaccumulation of several metals including, Cd, Cu, Hg, K, Mg, Na, P, Rb and Zn in caps and stipes of fruitbodies of this mushroom, while other metals such as Al, Ba, Ca, Co, Fe, Mn, Ni, Pb and Sr were not exhibiting significant positive BFCs. Over a period studied, the caps were characterised by different (p?<?0.05) concentrations of Al, Co, Cu, Hg, Mn, Ni, P, Pb and Sr. Contamination profiles, temporal fluctuations, BCFs should be taken into consideration when assessing the nutritional value of this mushroom. 相似文献
105.
106.
Luo Yang Wu Yinghong Ma Shuhua Zheng Shili Zhang Yi Chu Paul K. 《Environmental science and pollution research international》2021,28(15):18727-18740
Environmental Science and Pollution Research - The rapid economic development in China places a large demand for energy, and as a result, thermal power plants in China are producing an enormous... 相似文献
107.
Rehman Abdul Ma Hengyun Chishti Muhammad Zubair Ozturk Ilhan Irfan Muhammad Ahmad Munir 《Environmental science and pollution research international》2021,28(14):17319-17330
Environmental Science and Pollution Research - The accelerated urbanization in China was already coupled with a steadily increasing demand for energy usage. The present study major aim was to... 相似文献
108.
Yan Xingcheng Ma Jie Li Zhichun Ji Ming Xu Jie Xu Xiaoguang Wang Guoxiang Li Yunmei 《Environmental science and pollution research international》2021,28(9):10967-10976
Environmental Science and Pollution Research - Inland freshwater lakes have been widely considered as significant sources of CO2 to the atmosphere. However, long-term measurements of CO2 dynamics... 相似文献
109.
Chen Guifang Sun Xiaofei Feng Yunqi Song Zhanlong Cui Lin Mao Yanpeng Ma Chunyuan Chen Shouyan 《Environmental science and pollution research international》2021,28(6):6664-6674
Environmental Science and Pollution Research - Mechanical vapor compression and multi-effect evaporation have been widely used in achieving zero discharge of desulfurization wastewater as they are... 相似文献
110.
Determination of phthalates in particulate matter and gaseous phase emitted in indoor air of offices
Szewczyńska Małgorzata Dobrzyńska Elżbieta Pośniak Małgorzata 《Environmental science and pollution research international》2021,28(42):59319-59327
Environmental Science and Pollution Research - Phthalate esters (PAEs) are endocrine disrupters and can disrupt the functioning of different hormones, causing adverse effects on human health. Due... 相似文献