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911.
M.?Antonia?Lopez-AntonEmail author Nuria?Fernández-Miranda M.?Rosa?Martínez-Tarazona 《Environmental science and pollution research international》2016,23(24):24495-24503
Mercury is a well-known toxic element, and flue gas streams emitted from coal-fired utilities are one of the largest anthropogenic sources of this element. This study briefly reviews the proposed technologies for reducing mercury emissions from coal combustion, focusing on an emerging process which involves the use of regenerable sorbents and especially those loaded with noble metals. Among the mercury species formed during coal combustion, elemental mercury is the most difficult to remove from the flue gases due to its low reactivity and insolubility in water. The widespread interest in using regenerable sorbents with metals is due to their ability to retain elemental mercury. With this technology, not only can efficiencies of 100 % be reached in the retention of elemental mercury but also a way to avoid the generation of new wastes loaded with mercury. This study considers the main aspects that must be taken into account when developing effective regenerable sorbents for mercury capture, with special attention to sorbents containing noble metals. The characteristics of this process are compared with those of other processes in a more advanced state of development. 相似文献
912.
Marco Martínez-Cinco Jesús Santos-Guzmán 《Journal of the Air & Waste Management Association (1995)》2016,66(6):631-642
The Monterrey Metropolitan Area (MMA) in Northeast Mexico has shown high PM2.5 concentrations since 2003. The data shows that the annual average concentration exceeds from 2 to 3 times the Mexican PM2.5 annual air quality standard of 12 µg/m3. In a previous work we studied the chemical characterization of PM2.5 in two sites of the MMA during the winter season. Among the most important components we found ammonium sulfate and nitrate, elemental and organic carbon, and crustal matter. In this work we present the results of a second chemical characterization study performed during the summer time and the application of the chemical mass balance (CMB) model to determine the source apportionment of air pollutants in the region. The chemical analysis results show that the chemical composition of PM2.5 is similar in both sites and periods of the year. The results of the chemical analysis and the CMB model show that industrial, traffic, and combustion activities in the area are the major sources of primary PM2.5 and precursor gases of secondary inorganic and organic aerosol (SO2, NOx, NH3, and volatile organic compounds [VOCs]). We also found that black carbon and organic carbon are important components of PM2.5 in the MMA. These results are consistent with the MMA emission inventory that reports as major sources of particles and SO2 a refinery and fuel combustion, as well as nitrogen oxides and ammonium from transportation and industrial activities in the MMA and ammonium form agricultural activities in the state. The results of this work are important to identify and support effective actions to reduce direct emissions of PM2.5 and its precursor gases to improve air quality in the MMA. Implications: The Monterrey Metropolitan Area (MMA) has been classified as the most air-polluted area in Mexico by the World Health Organization (WHO). Effective actions need to be taken to control primary sources of PM2.5 and its precursors, reducing health risks on the population exposed and their associated costs. The results of this study identify the main sources and their estimated contribution to PM2.5 mass concentration, providing valuable information to the local environmental authorities to take decisions on PM2.5 control strategies in the MMA. 相似文献
913.
This study deals with the question of how winegrowing in Spain may be altered by anthropogenic climate change. The present state and expected future development of three bioclimatic indices relevant for winegrowing were assessed by observation, and four regional climate models from the EU-ENSEMBLES project were investigated. When comparing the 2061–2090 scenario period to the 1961–1990 reference period, the models unanimously indicate a significant increase in the mean of the two considered thermal indices over the entire study region. However, for the index based on temperature and precipitation, the models are heavily biased when verified against observations and generally disagree on the size of the projected future change. For this index, unanimous model agreement was only found for northwestern Spain where all models indicated a significant decrease in the mean. From these results, regional climate change is expected to negatively affect the quality of wine in the growing regions of central and southern Spain, and the Ebro valley, whereas positive effects should be expected in the northwest. No significant changes in the risk of mildew infestation are to be expected except for the northwest, where this risk is projected to decrease. 相似文献
914.
Aleksi Räsänen Sirkku Juhola Anja Nygren Mira Käkönen Maarit Kallio Adrián Monge Monge Markku Kanninen 《Regional Environmental Change》2016,16(8):2291-2302
We systematically reviewed current climate change literature in order to examine how multiple processes that affect human vulnerability have been studied. Of the 125 reviewed articles, 79 % were published after 2009. There are numerous concepts that point out to stressors other than climate change that were used in reviewed studies. These different concepts were used interchangeably, and they illustrate processes that act on different scales. Most widely used concepts included non-climatic (40 % of the articles), multiple stressors (38 %) and other factors (37 %). About 75 % of the studies either acknowledged or carefully analyzed the social and environmental context in which vulnerability is experienced. One-third of the studies recognized climate change-related stressors as the most important, one-third argued that stressors other than climate are more important, and the rest of the studies did not analyze the relative importance of the different processes. Interactions between different stressors were mentioned in 76 % and analyzed explicitly in 28 % of the articles. Our review shows that there are studies that analyze the social context of vulnerability within climate change-related literature and this literature is rapidly expanding. Reviewed studies point out that there are multiple interacting stressors, whose interlinkages need to be carefully analyzed and targeted by policies, which integrate adaptation to climate change and other stressors. In conclusion, we suggest that future studies should include analytical frameworks that reflect dissimilarities between different types of stressors, methodological triangulation to identify key stressors and analysis of interactions between multiple stressors across different scales. 相似文献
915.
Antoine Sambou Ida Theilade Rasmus Fensholt Anders Ræbild 《Regional Environmental Change》2016,16(6):1765-1777
Several studies have documented that vegetation in the Sahel is highly dynamic and is affected by the prevailing climatic conditions, as well as by human use of the areas. However, little is known about vegetation dynamics in the large saline areas bordering the rivers of West Africa. Combining satellite imagery, the perception of local people and botanical information, this study investigated the vegetation dynamics and the drivers of vegetation changes in Fatick Province, Senegal. Satellite images showed a change in vegetation composition, i.e., a loss of tree cover and an increase in shrub cover, herbaceous cover and tans (highly saline areas with sparse vegetation). Although the trend was the same, the three villages had different vegetation histories. A survey of the woody vegetation showed that shrubs and young trees were dominating with relatively few large trees. Local people perceived a general decline of woody plants from 1993 to 2013. Among 60 species mentioned by local people, 90 % were declining and 10 % increasing. Together the three methods documented a decrease in density and diversity of the woody vegetation, mainly influenced by salinity and land use. The large numbers of young trees indicate a potential for regeneration of some, but not all, tree species. As many tree species appreciated by local people were reported to be declining, local communities have experienced a reduction of their natural resources. Based on villagers’ recommendations for improved vegetation management, we discuss possible contributions including reforestation, desalinization and environmental protection for restoration of the vegetation. 相似文献
916.
Ferreira Felipe Silva Brito Samuel Vieira de Oliveira Almeida Waltécio Alves Rômulo Romeu Nóbrega 《Regional Environmental Change》2016,16(2):543-551
Regional Environmental Change - The use and trade of animals in traditional medicine involves many different species, some of which are threatened with extinction. Thus, evaluating biological and... 相似文献
917.
Sánchez-Arcilla Agustín Sierra Joan Pau Brown Sally Casas-Prat Mercè Nicholls Robert James Lionello Piero Conte Dario 《Regional Environmental Change》2016,16(8):2471-2484
Regional Environmental Change - The potential impact of climate change on port operations and infrastructures has received much less attention than the corresponding impact for beach systems.... 相似文献
918.
Brominated flame retardants and organochlorines in the European environment using great tit eggs as a biomonitoring tool 总被引:1,自引:0,他引:1
Van den Steen E Pinxten R Jaspers VL Covaci A Barba E Carere C Cichoń M Dubiec A Eeva T Heeb P Kempenaers B Lifjeld JT Lubjuhn T Mänd R Massa B Nilsson JA Norte AC Orell M Podzemny P Sanz JJ Senar JC Soler JJ Sorace A Török J Visser ME Winkel W Eens M 《Environment international》2009,35(2):310-317
Large-scale studies are essential to assess the emission patterns and spatial distribution of organohalogenated pollutants (OHPs) in the environment. Bird eggs have several advantages compared to other environmental media which have previously been used to map the distribution of OHPs. In this study, large-scale geographical variation in the occurrence of OHPs, such as polychlorinated biphenyls (PCBs), polybrominated diphenyl ethers (PBDEs) and organochlorine pesticides (OCPs), was investigated throughout Europe using eggs of a terrestrial residential passerine species, the great tit (Parus major). Great tit eggs from 22 sampling sites, involving urban, rural and remote areas, in 14 European countries were collected and analysed (5-8 eggs per sampling site). The environmentally most important congeners/compounds of the analysed pollutants were detectable in all sampling locations. For PCBs, PBDEs and OCPs, no clear geographical contamination pattern was found. Sum PCB levels ranged from 143 ng/g lipid weight (lw) to 3660 ng/g lw. As expected, PCB concentrations were significantly higher in the sampled urban compared to the remote locations. However, the urban locations did not show significantly higher concentrations compared to the rural locations. Sum PBDEs ranged from 4.0 ng/g lw to 136 ng/g lw. PBDEs were significantly higher in the urbanized sampling locations compared to the other locations. The significant, positive correlation between PCB and PBDE concentrations suggests similar spatial exposure and/or mechanisms of accumulation. Significantly higher levels of OCPs (sum OCPs ranging from 191 ng/g lw to 7830 ng/g lw) were detected in rural sampling locations. Contamination profiles of PCBs, PBDEs and OCPs differed also among the sampling locations, which may be due to local usage and contamination sources. The higher variance among sampling locations for the PCBs and OCPs, suggests that local contamination sources are more important for the PCBs and OCPs compared to the PBDEs. To our knowledge, this is the first study in which bird eggs were used as a monitoring tool for OHPs on such a large geographical scale. 相似文献
919.
J. R. Park M. J. Stabler P. J. Jones S. R. Mortimer J. R. Tiffin R. B. Tranter 《Environment, Development and Sustainability》2009,11(4):735-750
The issue of the sustainable development of rural economies in England has recently received considerable attention. This
is because many of the poorest areas in the country are rural, often of high environmental quality, but suffering from high
unemployment and a lack of services and facilities. The rapid decline in agricultural incomes and in-migration of affluent
urban workers since 1990 has exacerbated economic inequality in such areas. A number of factors have the potential to drive
rural development and this paper applies, and considers, the feasibility of a method from the USA for combining economic and
environmental variables in a regional growth model to examine the hypothesis that environmental quality is an important determinant
of sustainable rural development in England. The model output suggests that, although environmental quality does play a role
in sustainable rural development in England there are other, more important, factors driving development. These include business
and communications infra-structure, the degree and opportunities for commuting and underlying employment prospects. The robustness
and limitations of the method for combining economic and environmental variables is discussed in relation to the spatial interrelatedness
of Local Authority Districts in England, and conclusions are drawn about areas for refinement and improvement of the method.
相似文献
J. R. ParkEmail: |
920.
April L. Pulvirenti Karen M. Needham Mohamad A. Adel-Hadadi Charles R. Marks Jeffrey A. Gorman Donald L. Shettel Aaron Barkatt 《Journal of contaminant hydrology》2009,109(1-4):62-81
Thermal evaporation of a variety of simulated pore waters from the region of Yucca Mountain, Nevada, produced acidic liquids and gases during the final stages of evaporation. Several simulated pore waters were prepared and then thermally distilled in order to collect and analyze fractions of the evolved vapor. In some cases, distillates collected towards the end of the distillation were highly acidic; in other cases the pH of the distillate remained comparatively unchanged during the course of the distillation. The results suggest that the pH values of the later fractions are determined by the initial composition of the water. Acid production stems from the hydrolysis of magnesium ions, especially at near dryness. Near the end of the distillation, magnesium nitrate and magnesium chloride begin to lose water of hydration, greatly accelerating their thermal decomposition to form acid. Acid formation is promoted further when precipitated calcium carbonate is removed. Specifically, calcium chloride-rich pore waters containing moderate (10–20 ppm) levels of magnesium and nitrate and low levels of bicarbonate produced mixtures of nitric and hydrochloric acid, resulting in a precipitous drop in pH to values of 1 or lower after about 95% of the original volume was distilled. Waters with either low or moderate magnesium content coupled with high levels of bicarbonate produced slightly basic fractions (pH 7–9). If calcium was present in excess of bicarbonate, waters containing moderate levels of magnesium produced acid even in the presence of bicarbonate, due to the precipitation of calcium carbonate. Other salts such as halite and anhydrite promote the segregation of acidic vapors from residual basic solids. The concomitant release of wet acid gas has implications for the integrity of the alloys under consideration for containers at the Yucca Mountain nuclear waste repository. Condensed acid gases at very low pH, especially mixtures of nitric and hydrochloric acid, are capable of corroding even alloys, such as nickel-based Alloy 22, which are considered to be corrosion-resistant under milder conditions. 相似文献