全文获取类型
收费全文 | 9841篇 |
免费 | 113篇 |
国内免费 | 93篇 |
专业分类
安全科学 | 283篇 |
废物处理 | 459篇 |
环保管理 | 1243篇 |
综合类 | 1193篇 |
基础理论 | 2668篇 |
环境理论 | 2篇 |
污染及防治 | 2774篇 |
评价与监测 | 710篇 |
社会与环境 | 667篇 |
灾害及防治 | 48篇 |
出版年
2022年 | 101篇 |
2021年 | 77篇 |
2020年 | 65篇 |
2019年 | 72篇 |
2018年 | 145篇 |
2017年 | 139篇 |
2016年 | 229篇 |
2015年 | 164篇 |
2014年 | 237篇 |
2013年 | 742篇 |
2012年 | 296篇 |
2011年 | 441篇 |
2010年 | 364篇 |
2009年 | 395篇 |
2008年 | 470篇 |
2007年 | 475篇 |
2006年 | 422篇 |
2005年 | 366篇 |
2004年 | 323篇 |
2003年 | 375篇 |
2002年 | 325篇 |
2001年 | 503篇 |
2000年 | 331篇 |
1999年 | 192篇 |
1998年 | 137篇 |
1997年 | 133篇 |
1996年 | 138篇 |
1995年 | 162篇 |
1994年 | 125篇 |
1993年 | 102篇 |
1992年 | 123篇 |
1991年 | 118篇 |
1990年 | 130篇 |
1989年 | 130篇 |
1988年 | 94篇 |
1987年 | 87篇 |
1986年 | 65篇 |
1985年 | 90篇 |
1984年 | 89篇 |
1983年 | 86篇 |
1982年 | 82篇 |
1981年 | 73篇 |
1980年 | 61篇 |
1979年 | 68篇 |
1977年 | 53篇 |
1976年 | 48篇 |
1975年 | 53篇 |
1974年 | 51篇 |
1973年 | 53篇 |
1970年 | 45篇 |
排序方式: 共有10000条查询结果,搜索用时 10 毫秒
951.
Travis C Obenshain KR Gunter JT Regens JL Whipple C 《Environmental science and pollution research international》2004,11(5):302-306
GOAL, SCOPE AND BACKGROUND: This paper uses two case studies of U.S. Department of Energy nuclear weapons complex installations to illustrate the integration of expedited site characterization (ESC) and multimedia modeling in the remedial action decision making process. CONCEPTUAL SITE MODELS, MULTIMEDIA MODELS, AND EXPEDITED SITE CHARACTERIZATION: Conceptual site models outline assumptions about contaminates and the spatial/temporal distribution of potential receptors. Multimedia models simulate contaminant transport and fate through multiple environmental media, estimate potential human exposure via specific exposure pathways, and estimate the risk of cancer and non-cancer health outcomes. ESC relies on using monitoring data to quantify the key components of an initial conceptual site model that is modified iteratively using the multimedia model. CASE STUDIES: Two case studies are presented that used the ESC approach: Los Alamos National Laboratory (LANL) and Pantex. LANL released radionuclides, metals, and organic compounds, into canyons surrounding the facility. The Pantex Plant has past waste management operations which included burning chemical wastes in unlined pits, burying wastes in unlined landfills, and discharging plant wastewaters into on-site surface waters. CONCLUSIONS: The case studies indicate that using multimedia models with the ESC approach can inform assessors about what, where, and how much site characterization data needs to be collected to reduce the uncertainty associated with risk assessment. Lowering the degree of uncertainty reduces the time and cost associated with assessing potential risk and increases the confidence that decision makers have in the assessments performed. 相似文献
952.
Destruction of Wetlands and Waterbird Populations by Dams and Irrigation on the Murrumbidgee River in Arid Australia 总被引:3,自引:0,他引:3
The Lowbidgee floodplain is the Murrumbidgee Rivers major wetland in southeastern Australia. From more than 300,000 ha in the early 1900s, at least 76.5% was destroyed (58%) or degraded (18%) by dams (26 major storages), subsequent diversions and floodplain development. Diversions of about 2,144,000 ML year–1 from the Murrumbidgee River come from a natural median flow of about 3,380,000 ML year–1 providing water for Australias capital, hydroelectricity, and 273,000 ha of irrigation. Diversions have reduced the amount of water reaching the Lowbidgee floodplain by at least 60%, from 1888 to 1998. About 97,000 ha of Lowbidgee wetland was destroyed by development of the floodplain for an irrigation area (1975–1998), including building of 394 km of channels and 2,145 km of levee banks. Over 19 years (1983–2001), waterbird numbers estimated during annual aerial surveys collapsed by 90%, from an average of 139,939 (1983–1986) to 14,170 (1998–2001). Similar declines occurred across all functional groups: piscivores (82%), herbivores (87%), ducks and small grebe species (90%), large wading birds (91%), and small wading birds (95%), indicating a similar decline in the aquatic biota that formed their food base. Numbers of species also declined significantly by 21%. The Lowbidgee floodplain is an example of the ecological consequences of water resource development. Yanga Nature Reserve, within the Lowbidgee floodplain, conserved for its floodplain vegetation communities, will lose these communities because of insufficient water. Until conservation policies adequately protect river flows to important wetland areas, examples such as the Lowbidgee will continue to occur around the world. 相似文献
953.
954.
R. Goodland M. Ismail F. Strum David Walker Lupton Marc Jay Rogoff William Erich Cline David E. Goldenberg James C. Starbuck Lee S. Tesdell Anthony G. White John F. Schnell Richard S. Krannich Nan C. Burg Frederick Frankena Meredith Kirkpatrick U. G. Yermakov V. L. Mote C. ZumBrunnen T. B. Denisova V. L. Rauner P. P. Micklin G. L. Rutilevskiy 《Environmental management》1978,2(5):473-476
955.
This study investigated the liming effect of water treatment sludge on acid mine spoils. The study was conducted with sludge from a water purification plant along the Vaal River catchments in South Africa. The optimum application rate for liming acid spoils and the speed and depth with which the sludge reacted with the mine waste were investigated. Chemical analysis indicated that the sludge is suitable as a liming agent because of its alkaline pH (8.08), high bicarbonate concentration (183.03 mg L(-1)), and low salinity (electrical conductivity = 76 mS m(-1)). The high cation exchange capacity of 15.47 cmol(c) kg(-1) and elevated nitrate concentration (73.16 mg L(-1)) also increase its value as an ameliorative material. The soluble concentrations for manganese, aluminum, lead, and selenium were high at a pH of 5 although only selenium (0.83 mg L(-1)) warranted some concern. According to experimental results, the application of 10 Mg ha(-1) of sludge to acid gold tailings increased the leach water pH from 4.5 to more than 7.5 and also increased the medium pH from 2.4 to 7.5. The addition of sludge further reduced the solubility of iron, manganese, copper, and zinc in the ameliorated gold tailings, but increased the electrical conductivity. The liming tempo was highest in the coal discard profile that had a coarse particle size distribution and took the longest to move through the gold tailings that had a fine particle size distribution. Results from this study indicate that the water treatment sludge investigated is suitable as a liming agent for rehabilitation of acid mine waste. 相似文献
956.
The levels of copper, zinc, and arsenic in soil surrounding Douglas-fir [Pseudotsuga menziesii (Mirb.) Franco] utility poles treated with ammoniacal copper zinc arsenate (ACZA) were investigated at sites in Florida, Virginia, and New York. Copper levels were elevated near the poles and declined with both horizontal distance away from the pole and depth beneath the soil surface. Zinc levels were also elevated next to the poles, but the levels declined more slowly than did those of copper. Arsenic levels were elevated in soil immediately next to the poles but declined to near background levels farther away. The results indicate that metals can leach from ACZA-treated poles, but do not migrate far in the soil, and thus the levels decline sharply with distance from the poles. 相似文献
957.
Removal of selenium (Se) from agricultural drainage water is important in protecting wetland wildlife. Three flow-through bioreactor channel systems (BCSs), each with three channels filled with rice (Oryza sativa L.) straw, were set in the laboratory to determine removal of selenate [Se(VI)] (1020 microg L(-1)) from drainage water with a salinity of 10.4 dS m(-1), a pH of 8.1, and a nitrate (NO3-) range of 0 to 100 mg L(-1). Results showed that the rice straw effectively reduced Se(VI) during 122 to 165 d of the experiments. Calculation of Se mass in the three BCSs showed that 89.5 to 91.9% of the input Se(VI) was reduced to red elemental Se [Se(0)], where 96.6 to 98.2% was trapped in the BCSs. Losses of each gram of rice straw were almost equal to the removal of 1.66 mg of Se from the drainage water as a form of red Se(0), indicating that rice straw is a very effective organic source for removing Se(VI) from drainage water. 相似文献
958.
Intensive livestock operations can release odorous gases from stored or land-applied manure. We measured concentrations of dust and 14 odor-causing gases at increasing distances from four feedlots near Lethbridge, southern Alberta, Canada. Concentration was determined from the amount of total dust or gas accumulated in the sampIers, and the volume of air sampled. Adjacent the feedlots, the maximum concentration of many volatile fatty acids exceeded reported odor detection thresholds; the maximum ammonia concentration was close to the threshold. Ammonia and butyric acid approached or exceeded their individual odor thresholds as far as 200 m downwind of the feedlots. Highest concentrations were measured adjacent to land where manure was being applied. None of the odorant concentrations exceeded their irritation threshold. There was a positive relationship between ammonia concentration and odor intensity as well as dry deposition. Much of the emitted ammonia was deposited to soil immediately downwind, enough to supply all the nitrogen needed for crop growth. Odorant concentrations declined sharply with distance, though measurable odor occasionally persisted to 1 km from the feedlot, beyond the minimum separation guidelines (Alberta) for a single residential dwelling. The weekly averaged total suspended particulates (> 5 microm) were below the Alberta guideline criterion except for one period. Differences among feedlots in odorant plume concentrations were partly related to the stocking density of feedlots, which presumably affects manure moisture and amount of volatiles within the pens. 相似文献
959.
Rodriguez RR Basta NT Casteel SW Armstrong FP Ward DC 《Journal of environmental quality》2003,32(3):876-884
Soil ingestion by children is an important pathway in assessing public health risks associated with exposure to arsenic-contaminated soils. Soil chemical methods are available to extract various pools of soil arsenic, but their ability to measure bioavailable arsenic from soil ingestion is unknown. Arsenic extracted by five commonly used soil extractants was compared with bioavailable arsenic measured in vivo by immature swine (Sus scrofa) dosing trials. Fifteen contaminated soils that contained 233 to 17 500 mg kg(-1) arsenic were studied. Soil extractants were selected to dissolve surficially adsorbed and/or readily soluble arsenic (water, 1 M sodium acetate, 0.1 M Na2HPO4/0.1 M NaH2PO4) and arsenic in Fe and Mn oxide minerals (hydroxylamine hydrochloride, ammonium oxalate). The mean percent of total arsenic extracted was: ammonium oxalate (53.6%) > or = hydroxylamine hydrochloride (51.7%) > phosphate (10.5%), acetate (7.16%) > water (0.15%). The strongest relationship between arsenic determined by soil chemical extraction and in vivo bioavailable arsenic was found for hydroxylamine hydrochloride extractant (r = 0.88, significant at the 0.01 probability level). Comparison of the amount of arsenic extracted by soil methods with bioavailable arsenic showed the following trend: ammonium oxalate, hydroxylamine hydrochloride > in vivo > phosphate, acetate > water. The amount of arsenic dissolved in the stomach (potentially bioavailable) is between surficially adsorbed (extracted by phosphate or acetate) and surficially adsorbed + nonsurficial forms in Fe and Mn oxides (extracted by hydroxylamine hydrochloride or ammonium oxalate). Soil extraction methods that dissolve some of the amorphous Fe, such as hydroxylamine hydrochloride, can be designed to provide closer estimates of bioavailable arsenic. 相似文献
960.
The lysianassid amphipod Orchomenella aahu was associated with small-scale mass mortality of Ecklonia radiata, the dominant laminarian alga in north-eastern New Zealand. O. aahu burrowed into and hollowed out stipes with severe bleaching, accelerating mortality by 12–14 months. Meristoderm tissue of bleached plants contained approximately one-third of the phlorotannin content (~4% dry mass) present in unbleached, apparently healthier, sporophytes (~12% dry mass). Unbleached stages consistently lacked amphipod damage. O. aahu also colonised plants when non-lethal storm damage afforded entry into the cortical layers of the primary lamina, and ultimately the stipe. O. aahu typically consumed both medullary and cortical tissue of the stipes, forming networked brood-chambers within them, with increasing populations often reducing the plant to the holdfast. There was synchronised mortality across sites and between depths over spatial scales of metres. Following loss of the mature canopy, recruitment of E. radiata was generally within 2 months at most study sites where mortality had occurred.Communicated by G.F. Humphrey, Sydney 相似文献