全文获取类型
收费全文 | 1008篇 |
免费 | 17篇 |
国内免费 | 8篇 |
专业分类
安全科学 | 49篇 |
废物处理 | 42篇 |
环保管理 | 268篇 |
综合类 | 97篇 |
基础理论 | 229篇 |
环境理论 | 2篇 |
污染及防治 | 215篇 |
评价与监测 | 83篇 |
社会与环境 | 40篇 |
灾害及防治 | 8篇 |
出版年
2023年 | 5篇 |
2022年 | 13篇 |
2021年 | 14篇 |
2020年 | 10篇 |
2019年 | 19篇 |
2018年 | 27篇 |
2017年 | 28篇 |
2016年 | 33篇 |
2015年 | 33篇 |
2014年 | 24篇 |
2013年 | 74篇 |
2012年 | 37篇 |
2011年 | 57篇 |
2010年 | 40篇 |
2009年 | 42篇 |
2008年 | 64篇 |
2007年 | 46篇 |
2006年 | 53篇 |
2005年 | 41篇 |
2004年 | 38篇 |
2003年 | 37篇 |
2002年 | 21篇 |
2001年 | 22篇 |
2000年 | 29篇 |
1999年 | 13篇 |
1998年 | 6篇 |
1997年 | 12篇 |
1996年 | 10篇 |
1995年 | 10篇 |
1994年 | 11篇 |
1993年 | 14篇 |
1992年 | 12篇 |
1991年 | 9篇 |
1990年 | 7篇 |
1989年 | 6篇 |
1988年 | 5篇 |
1987年 | 9篇 |
1986年 | 8篇 |
1985年 | 10篇 |
1984年 | 10篇 |
1983年 | 9篇 |
1982年 | 11篇 |
1981年 | 10篇 |
1980年 | 6篇 |
1978年 | 7篇 |
1977年 | 9篇 |
1976年 | 3篇 |
1975年 | 4篇 |
1972年 | 3篇 |
1971年 | 5篇 |
排序方式: 共有1033条查询结果,搜索用时 15 毫秒
61.
L.-W. Antony Chen Judith C. Chow Bruce G. Doddridge Russell R. Dickerson William F. Ryan Peter K. Mueller 《Journal of the Air & Waste Management Association (1995)》2013,63(8):946-956
Abstract Observations of the mass and chemical composition of particles less than 2.5 μm in aerodynamic diameter (PM2.5), light extinction, and meteorology in the urban Baltimore-Washington corridor during July 1999 and July 2000 are presented and analyzed to study summertime haze formation in the mid-Atlantic region. The mass fraction of ammoniated sulfate (SO4 2-) and carbonaceous material in PM2.5 were each ~50% for cleaner air (PM2.5 < 10 μg/m3) but changed to ~60% and ~20%, respectively, for more polluted air (PM2.5 > 30 μg/m3). This signifies the role of SO4 2- in haze formation. Comparisons of data from this study with the Interagency Monitoring of Protected Visual Environments network suggest that SO4 2? is more regional than carbonaceous material and originates in part from upwind source regions. The light extinction coefficient is well correlated to PM2.5 mass plus water associated with inorganic salt, leading to a mass extinction efficiency of 7.6 ± 1.7 m2/g for hydrated aerosol. The most serious haze episode occurring between July 15 and 19, 1999, was characterized by westerly transport and recirculation slowing removal of pollutants. At the peak of this episode, 1-hr PM2.5 concentration reached ~45 μg/m3, visual range dropped to ~5 km, and aerosol water likely contributed to ~40% of the light extinction coefficient. 相似文献
62.
D. Bruce Henschel Roy C. Fortmann Nancy F. Roache Xiaoyu Liu 《Journal of the Air & Waste Management Association (1995)》2013,63(5):708-717
ABSTRACT A laboratory thermal desorption apparatus was used to measure emissions from a number of nominally identical photocopier toners—manufactured to meet the specifications of one specific model copier—when these toners were heated to fuser temperature (180-200 °C). The objective was to assess how potential volatile organic compound (VOC) emissions from the toner for a given copier can vary, depending upon the production run and the supplier. Tests were performed on a series of toner (and associated raw polymer feedstock) samples obtained directly from a toner manufacturer, representing two production runs using a nonvented extrusion process, and on toner cartridges purchased from two local retailers, representing three different production lots (histories unknown). The results showed that the retailer toners consistently had up to 350% higher emissions of some major compounds (expressed as |ig of compound emit-ted/g of toner), and up to 100% lower emissions of others, relative to the manufacturer toners (p ≤ 0.01). The manufacturer toners from one production run had emissions of certain compounds, and of total VOCs, that were modestly higher (13-18%) than those from the other run (p ≤ 0.01). The emission differences between the retailer and manufacturer toners are probably due to differences 相似文献
63.
Catherine A. Yanca Douglas C. Barth Krag A. Petterson Michael P. Nakanishi Bruce E. Johnsen 《Journal of the Air & Waste Management Association (1995)》2013,63(12):1733-1742
Abstract Three new methods applicable to the determination of hazardous metal concentrations in stationary source emissions were developed and evaluated for use in U.S. Environmental Protection Agency (EPA) compliance applications. Two of the three independent methods, a continuous emissions monitor-based method (Xact) and an X-ray-based filter method (XFM), are used to measure metal emissions. The third method involves a quantitative aerosol generator (QAG), which produces a reference aerosol used to evaluate the measurement methods. A modification of EPA Method 301 was used to validate the three methods for As, Cd, Cr, Pb, and Hg, representing three hazardous waste combustor Maximum Achievable Control Technology (MACT) metal categories (low volatile, semivolatile, and volatile). The modified procedure tested the methods using more stringent criteria than EPA Method 301; these criteria included accuracy, precision, and linearity. The aerosol generation method was evaluated in the laboratory by comparing actual with theoretical aerosol concentrations. The measurement methods were evaluated at a hazardous waste combustor (HWC) by comparing measured with reference aerosol concentrations. The QAG, Xact, and XFM met the modified Method 301 validation criteria. All three of the methods demonstrated precisions and accuracies on the order of 5%. In addition, correlation coefficients for each method were on the order of 0.99, confirming the methods’ linear response and high precision over a wide range of concentrations. The measurement methods should be applicable to emissions from a wide range of sources, and the reference aerosol generator should be applicable to additional analytes. EPA recently approved an alternative monitoring petition for an HWC at Eli Lilly’s Tippecanoe site in Lafayette, IN, in which the Xact is used for demonstrating compliance with the HWC MACT metal emissions (low volatile, semivolatile, and volatile). The QAG reference aerosol generator was approved as a method for providing a quantitative reference aerosol, which is required for certification and continuing quality assurance of the Xact. 相似文献
64.
65.
The aim of this work is to assess the potential ecotoxicological effects of contaminated sediments treated with mineral additives. The Microtox solid phase test was used to evaluate the effect of mineral additives on the toxicity of sediment suspensions. Four Mediterranean port sediments were studied after dredging and bioremediation: Sample A from navy harbor, sample B from commercial port and samples C and D from pleasure ports. Sediment samples were stabilized with three mineral additives: hematite, zero-valent iron and zeolite. Results show that all studied mineral additives can act as stabilizer agent in highly contaminated sediments (A and C) by decreasing dissolved metal concentrations and sediment toxicity level. On the contrary, for the less contaminated samples (B and D) hematite and zeolite can provoke toxic effect towards Vibrio fischeri since additive particles can favor bacteria retention and decrease bioluminescence emission. 相似文献
66.
Regular fuel reduction burning is an important management strategy for reducing the scale and intensity of wildfires in south-west
Australian native forests, but the long term effects of this on tree and stand growth are not well understood. Five fire treatments,
including application of frequent and infrequent low intensity burns, and 25 years of fire exclusion, were applied to small
(4 ha) experimental plots in a low rainfall mixed jarrah (Eucalyptus marginata) and marri (Corymbia calophylla) forest to investigate the effects of these treatments on tree stem diameter growth, stand basal area increment and tree
mortality. Mean tree stem growth measured over 20 years was lowest in the long unburnt treatment compared with the burn treatments,
although surface soil nutrient levels were generally higher in the unburnt treatment, suggesting these sites may be moisture
limited. There was no clear pattern of the effects of the burn treatments, including the number of fires and the interval
between fires, on tree stem growth, stand basal area increment, crown health or mortality. These factors were strongly influenced
by dominance condition, with dominant and co-dominant trees growing most and suppressed trees growing least and experiencing
the highest mortality levels. There was no evidence of deteriorating tree or stand health that could be attributed to either
regular low intensity burning or to a long period (25 years) of fire exclusion. 相似文献
67.
Jeffrey J. Opperman Ryan Luster Bruce A. McKenney Michael Roberts Amanda Wrona Meadows 《Journal of the American Water Resources Association》2010,46(2):211-226
Opperman, Jeffrey J., Ryan Luster, Bruce A. McKenney, Michael Roberts, and Amanda Wrona Meadows, 2010. Ecologically Functional Floodplains: Connectivity, Flow Regime, and Scale. Journal of the American Water Resources Association (JAWRA) 46(2):211-226. DOI: 10.1111/j.1752-1688.2010.00426.x Abstract: This paper proposes a conceptual model that captures key attributes of ecologically functional floodplains, encompassing three basic elements: (1) hydrologic connectivity between the river and the floodplain, (2) a variable hydrograph that reflects seasonal precipitation patterns and retains a range of both high and low flow events, and (3) sufficient spatial scale to encompass dynamic processes and for floodplain benefits to accrue to a meaningful level. Although floodplains support high levels of biodiversity and some of the most productive ecosystems on Earth, they are also among the most converted and threatened ecosystems and therefore have recently become the focus of conservation and restoration programs across the United States and globally. These efforts seek to conserve or restore complex, highly variable ecosystems and often must simultaneously address both land and water management. Thus, such efforts must overcome considerable scientific, technical, and socioeconomic challenges. In addition to proposing a scientific conceptual model, this paper also includes three case studies that illustrate methods for addressing these technical and socioeconomic challenges within projects that seek to promote ecologically functional floodplains through river-floodplain reconnection and/or restoration of key components of hydrological variability. 相似文献
68.
Eric C. Merten Nathaniel A. Hemstad Randall K. Kolka Raymond M. Newman Elon S. Verry Bruce Vondracek 《Journal of the American Water Resources Association》2010,46(4):733-743
Merten, Eric C., Nathaniel A. Hemstad, Randall K. Kolka, Raymond M. Newman, Elon S. Verry, and Bruce Vondracek, 2010. Recovery of Sediment Characteristics in Moraine, Headwater Streams of Northern Minnesota After Forest Harvest. Journal of the American Water Resources Association (JAWRA) 46(4): 733-743. DOI: 10.1111/j.1752-1688.2010.00445.x Abstract: We investigated the recovery of sediment characteristics in four moraine, headwater streams in north-central Minnesota after forest harvest. We examined changes in fine sediment levels from 1997 (preharvest) to 2007 (10 years postharvest) at study plots with upland clear felling and riparian thinning, using canopy cover, proportion of unstable banks, surficial fine substrates, residual pool depth, and streambed depth of refusal as response variables. Basin-scale year effects were significant (p < 0.001) for all responses when evaluated by repeated-measures ANOVAs. Throughout the study area, unstable banks increased for several years postharvest, coinciding with an increase in windthrow and fine sediment. Increased unstable banks may have been caused by forest harvest equipment, increased windthrow and exposure of rootwads, or increased discharge and bank scour. Fine sediment in the channels did not recover by summer 2007, even though canopy cover and unstable banks had returned to 1997 levels. After several storm events in fall 2007, 10 years after the initial sediment input, fine sediment was flushed from the channels and returned to 1997 levels. Although our study design did not discern the source of the initial sediment inputs (e.g., forest harvest, road crossings, other natural causes), we have shown that moraine, headwater streams can require an extended period (up to 10 years) and enabling event (e.g., high storm flows) to recover from large inputs of fine sediment. 相似文献
69.
Nicolas Creusot Nathalie Tapie Benjamin Piccini Patrick Balaguer Jean-Marc Porcher Hélène Budzinski Selim Aït-Aïssa 《Environmental science and pollution research international》2013,20(5):2784-2794
The contamination of aquatic systems by endocrine disrupting chemicals (EDCs) is now a widely established fact. Nevertheless, there is still a scarcity of knowledge concerning the source, transport, fate and bioavailability of such active compounds. In the present study we assessed the distribution of estrogenic, (anti-)androgenic, pregnane X receptor-like (PXR) and dioxin-like activities between sediment and water compartments using a polar organic compound integrative sampler (POCIS) and a semi-permeable membrane device (SPMD) passive sampler in a river where sediment has been previously described as highly and multi-contaminated. We first confirmed the contamination pattern of this river sediment between 2004, 2009 and 2010 samples, suggesting that this river is subject to a constant high contamination level. However, we showed a different distribution pattern of these activities between compartments: estrogenic activity was mainly detected in POCIS extracts and to a lesser extent in sediment and SPMD extracts; anti-androgenic activities were mainly detected in SPMD and sediment extracts while no activity was detected in POCIS extracts; PXR-like activity was detected in all three investigated compartments, with POCIS > SPMD > sediment; dioxin-like activity was mainly found in the sediment and the SPMD extracts. Overall, partitioning of the biological activities was in accordance with physicochemical properties (e.g., log K ow) of typical known active chemicals in each bioassay. Furthermore, in order to establish whether the chemicals involved in these activities were similar between the compartments, we fractionated sediment, POCIS and SPMD extracts using a multi-step fractionation procedure. This highlighted differences in the nature of active chemicals between compartments. Altogether, our results support the need to consider different compartments in order to enhance exposure assessment. 相似文献
70.
A. Manoukian E. Quivet B. Temime-Roussel M. Nicolas F. Maupetit H. Wortham 《Environmental science and pollution research international》2013,20(7):4659-4670
Volatile organic compounds (VOCs) and particles emitted by incense sticks and candles combustion in an experimental room have been monitored on-line and continuously with a high time resolution using a state-of-the-art high sensitivity-proton transfer reaction-mass spectrometer (HS-PTR-MS) and a condensation particle counter (CPC), respectively. The VOC concentration–time profiles, i.e., an increase up to a maximum concentration immediately after the burning period followed by a decrease which returns to the initial concentration levels, were strongly influenced by the ventilation and surface interactions. The obtained kinetic data set allows establishing a qualitative correlation between the elimination rate constants of VOCs and their physicochemical properties such as vapor pressure and molecular weight. The emission of particles increased dramatically during the combustion, up to 9.1(±0.2)?×?104 and 22.0(±0.2)?×?104 part cm?3 for incenses and candles, respectively. The performed kinetic measurements highlight the temporal evolution of the exposure level and reveal the importance of ventilation and deposition to remove the particles in a few hours in indoor environments. 相似文献