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The elemental mercury removal abilities of three different zeolites (NaA, NaX, HZSM-5) impregnated with iron (III) chloride were studied on alab-scale fixed-bed reactor. X-ray diffraction, nitrogen adsorption porosimetry, Fourier transform infrared spectroscopy, X-ray photoelectron spectroscopy, and temperature programmed desorption (TPD) analy-ses were used to investigate the physicochemical properties. Results indicated that the pore structure and active chloride species on the surface of the samples are the key factors for physisorption and oxidation of Hg0, respectively. Relatively high surface area and micropore volume are beneficial to efficient mercury adsorption. The active Cl species generated on the surface of the samples were effective oxidants able to convert elemental mercury (Hg0) into oxidized mercury (Hg2+). The crystallization of NaCl due to the ion exchange effect during the impregnation of NaA and NaX reduced the number of active Cl species on the surface, and restricted the physisorption of Hg0. Therefore, the Hg0 removal efficiencies of the samples were inhibited. The TPD analysis revealed that the species of mercury on the surface of FeCl3-HZSM-5 was mainly in the form of mercuric chloride(HgCl2), while on FeCl3-NaX and FeCl3-NaA it was mainly mercuri coxide(HgO). 相似文献
253.
Pin Xie Xiuli Hao Martin Herzberg Yantao Luo Dietrich H.Nies Gehong Wei 《环境科学学报(英文版)》2015,(1):179-187
To better understand the diversity of metal resistance genetic determinant from microbes that survived at metal tailings in northwest of China, a highly elevated level of heavy metal containing region, genomic analyses was conducted using genome sequence of three native metal-resistant plant growth promoting bacteria(PGPB). It shows that: Mesorhizobium amorphae CCNWGS0123 contains metal transporters from P-type ATPase, CDF(Cation Diffusion Facilitator), Hup E/Ure J and CHR(chromate ion transporter) family involved in copper, zinc, nickel as well as chromate resistance and homeostasis. Meanwhile, the putative Cop A/Cue O system is expected to mediate copper resistance in Sinorhizobium meliloti CCNWSX0020 while Znt A transporter, assisted with putative Czc D, determines zinc tolerance in Agrobacterium tumefaciens CCNWGS0286. The greenhouse experiment provides the consistent evidence of the plant growth promoting effects of these microbes on their hosts by nitrogen fixation and/or indoleacetic acid(IAA) secretion,indicating a potential in-site phytoremediation usage in the mining tailing regions of China. 相似文献
254.
裂隙对雾龙洞岩溶发育及地下径流的影响分析 总被引:3,自引:0,他引:3
尝试利用裂隙测量结果探究区域岩溶发育规律。采用统计窗口法对湖北鄂西地区雾龙洞岩溶流域的碳酸盐岩地层进行了大量的裂隙测量,分析了流域内裂隙发育的情况,研究了裂隙的几何参数——倾向、倾角、隙宽、线密度、面裂隙率等在不同层位、不同裂隙分组内的变化情况;结合构造、岩溶洼地发育方向、洞穴野外探测结果,综合分析了裂隙发育对本区岩溶发育的影响;运用渗透张量理论对岩溶流域裂隙的各向异性和非均质性进行了研究,并分析了雾龙洞岩溶流域地下水的主要渗流方向形成的原因,对查明雾龙洞岩溶流域岩溶发育规律以及地下水的运移、赋存规律具有一定的指导作用。 相似文献
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Immediate behavioural responses to earthquakes in Christchurch,New Zealand,and Hitachi,Japan 总被引:1,自引:0,他引:1
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Michael K. Lindell Carla S. Prater Hao Che Wu Shih‐Kai Huang David M. Johnston Julia S. Becker Hideyuki Shiroshita 《Disasters》2016,40(1):85-111
This study examines people's immediate responses to earthquakes in Christchurch, New Zealand, and Hitachi, Japan. Data collected from 257 respondents in Christchurch and 332 respondents in Hitachi revealed notable similarities between the two cities in people's emotional reactions, risk perceptions, and immediate protective actions during the events. Respondents' physical, household, and social contexts were quite similar, but Hitachi residents reported somewhat higher levels of emotional reaction and risk perception than did Christchurch residents. Contrary to the recommendations of emergency officials, the most frequent response of residents in both cities was to freeze. Christchurch residents were more likely than Hitachi residents to drop to the ground and take cover, whereas Hitachi residents were more likely than Christchurch residents to evacuate immediately the building in which they were situated. There were relatively small correlations between immediate behavioural responses and demographic characteristics, earthquake experience, and physical, social, or household context. 相似文献
258.
统计了2008-2015年宁沪高速公路上由雾造成的交通事故92起,分析了雾事故与雾发生频率之间的关系,研究发现,雾事故易发生于秋冬季,而冬季由于路面摩擦系数较低更易出现事故;经过比较,能见度低于100 m的条件下雾事故发生概率较大;早晨6-8时为雾事故发生的高峰期,这与此时段雾发生频率较高及车流量加大有关;宁沪高速的西段为雾事故及雾发生频率较高的路段;分析了雾事故发生时的能见度与湿度、温度和风速的关系;利用能见度区间,雾日变化特征,摩擦系数及雾站点覆盖率制定了宁沪高速雾危险指数NHFI,并利用Spearman秩相关系数法分别比较了NHFI,雾日数与雾事故数的相关性,结果显示NHFI评价路段危险性要比单纯用雾日数更合理和精确。通过利用数值模式计算每段路的NHFI可以预测宁沪高速危险指数及危险路段分布。 相似文献
259.
Xu S Hao X Stanford K McAllister TA Larney FJ Wang J 《Journal of environmental quality》2007,36(6):1914-1919
Composting may be a viable on-farm option for disposal of cattle carcasses. This study investigated greenhouse gas emissions during co-composting of calf mortalities with manure. Windrows were constructed that contained manure + straw (control compost [CK]) or manure + straw + calf mortalities (CM) using two technologies: a tractor-mounted front-end loader or a shredder bucket. Composting lasted 289 d. The windrows were turned twice (on Days 72 and 190), using the same technology used in their creation. Turning technology had no effect on greenhouse gas emissions or the properties of the final compost. The CO2 (75.2 g d(-1) m(-2)), CH4 (2.503 g d(-1) m(-2)), and N2O (0.370 g d(-1) m(-2)) emissions were higher (p < 0.05) in CM than in CK (25.7, 0.094, and 0.076 g d(-1) m(-2) for CO2, CH4, and N2O, respectively), which reflected differences in materials used to construct the compost windrows and therefore their total C and total N contents. The final CM compost had higher (p < 0.05) total N, total C, and mineral N content (NO3*+ NO2* + NH4+) than did CK compost and therefore has greater agronomic value as a fertilizer. 相似文献
260.
气候变化和人类活动对黄河三角洲植被动态变化的影响 总被引:3,自引:0,他引:3
黄河三角洲是我国暖温带最完整、面积最大的湿地生态系统,其植被变化对于黄河三角洲生态功能和生态安全具有重要意义.本研究基于植被覆盖度(fractional vegetation cover,FVC)、叶面积指数(leaf area index,LAI)、净初级生产力(net primary productivity,NPP)3个生态参数,分析了2000-2017年黄河三角洲地区植被的动态变化,并以NPP为指标量化分析了气候变化和人类活动对植被生产力的贡献.研究发现,2000-2017年黄河三角洲FVC(Slope=0.004,p<0.05)、LAI(Slope=0.011,p<0.05)、NPP(Slope=3.54 g·m-2·a-1,p<0.01)呈显著增加趋势,说明2000-2017年黄河三角洲植被生长状况趋好、植被生产力提高.气温、降水和太阳总辐射对植被NPP变化的贡献分别为0.006、0.81、-0.03g·m-2·a-1,即降水对植被NPP变化的贡献最大,这主要是因为黄河三角洲的主要土地利用类型为耕地,受降水影响大,当地土壤具有盐碱化风险,降水可以补充淡水资... 相似文献