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911.
Material Disposal Area G is the primary low-levelradioactive waste disposal site at Los Alamos NationalLaboratory, New Mexico, and is adjacent to Pueblo of SanIldefonso lands. Pueblo residents and Los Alamos scientists areconcerned about radiological doses resulting from uptake of AreaG radionuclides by mule deer (Odocoileus hemionus) andRocky Mountain elk (Cervus elaphus), then consumption ofdeer and elk meat by humans. Tissue samples were collected fromdeer and elk accidentally killed near Area G and were analyzedfor 3H, 90Sr, total U, 238Pu, 239, 240Pu,241Am, and 137Cs. These data were used to estimatehuman doses based on meat consumption of 23 kg y-1. Humandoses were also modeled using RESRAD, and dose rates to deer andelk were estimated with a screening model. Dose estimates tohumans from tissue consumption were 2.9 × 10-3 mSv y-1and 1.6 × 10-3 mSv y-1 from deer and elk, respectively,and RESRAD dose estimates were of the same order of magnitude. Estimated dose rates to deer and elk were 2.1 × 10-4 mGyd-1 and 4.7 × 10-4 mGy d-1, respectively. Allestimated doses were significantly less than established exposurelimits or guidelines. 相似文献
912.
Hong S Boutron CF Barbante C Do Hur S Lee K Gabrielli P Capodaglio G Ferrari CP Turetta C Petit JR Lipenkov VY 《Journal of environmental monitoring : JEM》2005,7(12):1326-1331
Lead (Pb), cadmium (Cd), copper (Cu) and zinc (Zn) have been measured by electrothermal atomic absorption spectrometry in various sections of the 3623 m deep ice core drilled at Vostok, in central East Antarctica. The sections were dated from 240 to 410 kyear BP (Marine Isotopic Stages (MIS) 7.5 to 11.3), which corresponds to the 3rd and 4th glacial-interglacial cycles before present. Concentrations are found to have varied greatly during this 170 kyear time period, with high concentration values during the coldest climatic stages such as MIS 8.4 and 10.2 and much lower concentration values during warmer periods, such as the interglacials MIS 7.5, 9.3 and 11.3. Rock and soil dust were the dominant sources for Pb, whatever the period, and for Zn and Cu and possibly Cd during cold climatic stages. The contribution from volcanic emissions was important for Cd during all periods and might have been significant for Cu and Zn during warm periods. 相似文献
913.
Sutton MA Asman WA Ellermann T Van Jaarsveld JA Acker K Aneja V Duyzer J Horvath L Paramonov S Mitosinkova M Tang YS Achermann B Gauger T Bartniki J Neftel A Erisman JW 《Environmental monitoring and assessment》2003,82(2):149-185
In the context of international efforts to reduce the impactsof atmospheric NH3 and NH4
+ (collectively, NHx), it is important to establish the link between NH3emissions and monitoring of NHx concentrations and deposition. This is equally relevant to situations where NH3emissions changes are certain (e.g. due to changed source sectoractivity), as to cases where NH3 abatement technologies havebeen implemented. Correct interpretation of adequate atmosphericmeasurements is essential, since monitoring data provide the onlymeans to evaluate trends in regional NH3 emissions.These issues have been reviewed using available measurements and modelling from nine countries. In addition to historic datasets,the analysis here considers countries where NH3 source sector activity changed (both increases and decreases) and countries where NH3 abatement policies have been implemented.In The Netherlands an `ammonia gap' was identified between the expected reduction and results of monitoring, and was attributedinitially to ineffectiveness of the abatement measures. The analysis here for a range of countries shows that atmospheric interactions complicate the expected changes, particularly sinceSO2 emissions have decreased at the same time, while at manysites the few years of available data show substantial inter-annual variation. It is concluded that networks need to beestablished that speciate between NH3 and aerosol NH4
+, in addition to providing wet deposition, and sample at sufficient sites for robust regional estimates to be established. Such measurements will be essential to monitor compliance of the international agreements on NH3 emission abatement. 相似文献
914.
F. A. Y. Gailey G. H. Smith L. J. Rintoul O. Ll. Lloyd 《Environmental monitoring and assessment》1985,5(3):291-309
Lichen transplants of Hypogymnia physodes were used in a high-density network of sites for collecting airborne metals from the atmosphere in Armadale, a small industrial town in central Scotland. The mapping of the concentrations of various metals revealed a gradient of metal values which decreased outwards from the town's steel foundry. The findings were discussed in the context of a previous epidemiological investigation of lung disease in the town. 相似文献
915.
The content of lead and cadmium in surface dust within a 4 km radius of a sewage sludge incinerator has been investigated. Particular attention was given to Pb and Cd in different size fractions of dust, an aspect not explored in previous studies, and the differences between expressions of contamination as concentration or loading were examined. Despite suggestions from reports that sludge incinerators may have difficulty in complying with emission standards, the present investigation found little evidence for a major contribution to local pollution by the incinerator. Certainly, the highest Cd level was found some 2.2 km downwind of the prevailing wind direction from the incinerator, suggesting some resultant contamination, although the levels do not appear to be excessive. Similar observations apply to Pb contamination of the area. While data of the type produced in this study contribute to an understanding of environmental quality, both loadings and levels need to be considered, as the implications of only consideration one of these may be limited and even misleading. 相似文献
916.
Han JS Moon KJ Kong BJ Lee SJ Kim JE Kim YJ 《Environmental monitoring and assessment》2005,107(1-3):221-237
PM2.5 aerosol samples were collected at Gosan in Jeju Island during six intensive measurement periods between November 2001 and
August 2003. In order to investigate the chemical composition of fine particles, major ion components, trace elements, and
elemental and organic carbon were analyzed. Quite different seasonal characteristic in the chemical composition of fine particles
was observed. The concentration of most secondary aerosol components showed a summer minimum and a winter maximum with higher
correlation between them at Gosan. This fact clearly reveals the possibility of long-range transport of such pollutants in
winter. On the other hand, OC and EC had the highest concentration and good correlation with ion components, such as K+, Ca2+ in fall. It means that biomass burning could significantly influence the ambient fine carbonaceous particulate in fall, which
was primarily long-range transported. 相似文献
917.
918.
919.
Samples of the hermatypic coralGalaxea fascicularis were collected between April 1987 and April 1990 from coral reefs off Singapore (103 °45E; 1 °13N). Ca2+-activated adenosine triphosphatase (ATPase) activity was detected in the plasma-membrane-enriched heavy microsomal fraction ofG. fascicularis. The high affinity component hadKm andVmax values of 0.0021 mM and 0.050 µmol Pi mg–1 protein min–1, respectively; corresponding values for the low affinity component were 0.15 mM and 0.85 µmol mg–1 protein min–1. The activity of the high affinity component was inhibited 80 and 50%, respectively, by the anticalmodulin drugs calmidazolium and chlorpromazine. The low affinity component of the Ca2+-ATPase may represent activities of alkaline phosphatase, Ca2+-ATPase from membranes of mitochondria and endoplasmic reticulum, or calmodulin-dissociated plasma membrane Ca2+-ATPase resulting from the removal of Ca2+ by EDTA during the isolation process. The high affinity Ca2+-ATPase is probably the enzyme responsible for Ca2+ extrusion from the cells ofG. fascicularis. The high and low affinity components of this Ca2+-ATPase could use ATP and ADP as substrates. Maximum activities of both components were registered at pH 7 and at 45°C. Ruthenium red, a specific inhibitor of Ca2+-ATPase, inhibited the activities of the high and low affinity Ca2+-ATPase by 100 and 60%, respectively. Inhibition of the activities of both components was also observed with sulphydryl reagents (PCMB and mersalyl). However, DCMU, diamox, dinitrophenol, iodoacetate, fluoride, cyanide, ouabain, oligomycin B and L-phenylalanine had no effect on the enzyme activities. 相似文献
920.
We simulated the long range transport of dust emitted from dust storms that occurred in China by using a global three-dimensional chemical transport model. A modified dust emission flux scheme and a nonlocal diffusion scheme for determining the atmospheric eddy diffusivity in the atmospheric boundary layer were implemented to improve the chemical transport model. We examined the dust transport by comparing the model results with TOMS satellite images. The model calculated monthly total deposition of dust masses were used for comparison with the measurements collected at sampling stations in Japan, and good agreement was found. The model generally reproduced the temporal and spatial variations of dust reasonably well. 相似文献