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741.
742.
Hong Zhao Yunshan Ge Tiezhu Zhang Jipeng Zhang Jianwei Tan Hongxin Zhang 《环境科学学报(英文版)》2014,26(10):2027-2033
The alteration and formation of toxic compounds and potential changes in the toxicity of emissions when using after-treatment technologies have gained wide attention. Volatile organic compound(VOC), carbonyl compound and particle-phase polycyclic aromatic hydrocarbon(PAH) emissions were tested at European Steady State Cycle(ESC) to study unregulated emissions from a diesel engine with a fuel-borne catalyst and diesel particulate filter(FBC–DPF). An Fe-based fuel-borne catalyst was used for this study. According to the results, brake specific emissions of total VOCs without and with DPF were 4.7 and4.9 mg/kWh, respectively, showing a 4.3% increase. Benzene and n-undecane emissions increased and toluene emission decreased, while other individual VOC emissions basically had no change. When retrofitted with the FBC–DPF, total carbonyl compound emission decreased 15.7%, from 25.8 to 21.8 mg/kWh. The two highest carbonyls, formaldehyde and acetaldehyde, were reduced from 20.0 and 3.7 to 16.5 and 3.3 mg/kWh respectively. The specific reactivity(SR) with DPF was reduced from 6.68 to 6.64 mg/kWh. Total particle-phase PAH emissions decreased 66.4% with DPF compared to that without DPF. However, the Benzo[a]pyrene equivalent(BaPeq) with DPF had increased from 0.016 to 0.030 mg/kWh.Fluoranthene and Pyrene had the greatest decrease, 91.1% and 88.4% respectively. The increase of two- and three-ring PAHs with DPF indicates that the fuel-borne catalyst caused some gas-phase PAHs to adsorb on particles. The results of this study expand the knowledge of the effects of using a particulate filter and a Fe-based fuel-borne catalyst on diesel engine unregulated emissions. 相似文献
743.
Seasonal and diurnal variations of atmospheric peroxyacetyl nitrate, peroxypropionyl nitrate, and carbon tetrachloride in Beijing 总被引:1,自引:0,他引:1
Gen Zhang Yujing Mu Junfeng Liu Chenglong Zhang Yuanyuan Zhang Yujie Zhang Hongxing Zhang 《环境科学学报(英文版)》2014,26(1):65-74
Atmospheric peroxyacetyl nitrate(PAN), peroxypropionyl nitrate(PPN), and carbon tetrachloride(CCl4) were measured from September 2010 to August 2011 in Beijing. PAN exhibited low values from mid-autumn to early spring(October to March) with monthly average concentrations ranging from 0.28 to 0.73 ppbV, and increased from early spring to summer(March to August), ranging from 1.37–3.79 ppbV. The monthly variation of PPN was similar to PAN, with low values(below detection limit to 0.18 ppbV) from mid-autumn to early spring, and a monthly maximum in September(1.14 ppbV). The monthly variation of CCl4was tightly related to the variation of temperature, exhibiting a minimum in winter(69.3 pptV) and a maximum of 180.6 pptV in summer. Due to weak solar intensity and short duration, PAN and O3showed no distinct diurnal patterns from morning to night during winter, whereas for other seasons, they both exhibited maximal values in the late afternoon(ca. 15:00 to 16:00 local time) and minimal values during early morning and midnight. Good linear correlations between PAN and PPN were found in autumn(R = 0.91), spring(R = 0.94), and summer(R = 0.81), with slopes of 0.130, 0.222, and 0.133, respectively, suggesting that anthropogenic hydrocarbons dominated the photochemical formation of PANs in Beijing. Positive correlation between PAN and O3 in summer with the low slopes( O3 / PAN) ranging from 9.92 to 18.0 indicated serious air pollution in Beijing, and strong negative correlation in winter reflected strong O3consumption by NO titration and less thermal decompositin of PAN. 相似文献
744.
本文通过对国外和我国民间直升机的救援现状进行分析,从救援装备、专业人才、基础设施、政策法规、运营模式等方面做了对比研究,发现我国在各方面都存在较大差距,提出了构建我国民间直升机救援体系的具体措施。 相似文献
745.
Ionic composition of submicron particles (PM1.0) during the long-lasting haze period in January 2013 in Wuhan, central China 总被引:1,自引:0,他引:1
Hairong Cheng Wei Gong Zuwu Wang Fan Zhang Xinming Wang Xiaopu Lv Jia Liu Xiaoxin Fu Gan Zhang 《环境科学学报(英文版)》2014,26(4):810-817
In January 2013, a long-lasting severe haze episode occurred in Northern and Central China; at its maximum, it covered a land area of approximately 1.4 million km2. In Wuhan, the largest city in Central China, this event was the most severe haze episode in the 21st century. Aerosol samples of submicron particles (PM1.0) were collected during the long-lasting haze episode at an urban site and a suburban site in Wuhan to investigate the ion characteristics of PM1.0 in this area. The mass concentrations of PM1.0 and its water-soluble inorganic ions (WSIIs) were almost at the same levels at two sites, which indicates that PM1.0 pollution occurs on a regional scale in Wuhan. WSIIs (Na+, NH4+, K+, Mg2+, Ca2+, Cl-, NO3- and SO42-) were the dominant chemical species and constituted up to 48.4% and 47.4% of PM1.0 at WD and TH, respectively. The concentrations of PM1.0 and WSIIs on haze days were approximately two times higher than on normal days. The ion balance calculations indicate that the particles were more acidic on haze days than on normal days. The results of the back trajectory analysis imply that the high concentrations of PM1.0 and its water-soluble inorganic ions may be caused by stagnant weather conditions in Wuhan. 相似文献
746.
张晓华 《安全.健康和环境》2010,10(10):8-10
介绍了中国石化HSE观察的应用背景与目的,重点探讨了对HSE观察问题的处理与分析,及其对管理的促进。 相似文献
747.
Effect of wastewater composition on the calcium carbonate precipitation in upflow anaerobic sludge blanket reactors 总被引:1,自引:0,他引:1
Shucheng Yang Yanling He Yonghong Liu Charles Chou Pengxiang Zhang Dongqi Wang 《Frontiers of Environmental Science & Engineering in China》2010,4(2):142-149
Calcium carbonate often precipitates in anaerobic reactors treating wastewater with high calcium content. The aim of this
paper is to study the effect of wastewater composition on calcium carbonate precipitation in upflow anaerobic sludge blanket
(UASB) reactors. Two laboratory-scale UASB reactors were operated with calcium-containing influents using acetate and carbohydrate
as substrate, respectively. There was an obvious accumulation of inorganic precipitate observed in the biogranules. Observations
via scanning electron microscope (SEM) and energy dispersive spectroscopy (EDS) showed that the acclimated biogranules in
the two reactors differed in microstructure. Calcium carbonate was found to have precipitated on the surface of acetate-degrading
biogranules, but precipitated at the core of the carbohydrate-degrading biogranules. The results indicated that substrates
had significant influence on the location of calcium carbonate precipitation in anaerobic granular sludge, which was expected
due to the different methanogens distribution and pH gradient within the granular sludge degrading various substrates. Moreover,
the location of calcium carbonate precipitation substantially affected the specific methanogenic activity (SMA) of the granular
sludge. The SMA of the acetate-degrading biogranules dropped from $
1.96 gCOD_{CH_4 } \cdot gVSS^{ - 1} \cdot d^{ - 1}
$
1.96 gCOD_{CH_4 } \cdot gVSS^{ - 1} \cdot d^{ - 1}
to $
0.61 gCOD_{CH_4 } \cdot gVSS^{ - 1} \cdot d^{ - 1}
$
0.61 gCOD_{CH_4 } \cdot gVSS^{ - 1} \cdot d^{ - 1}
after 180-d of operation in the reactor. However, the SMA of the carbohydrate-degrading biogranules was not adversely affected
by calcium carbonate precipitation. 相似文献
748.
对海底管线穿孔后如何阻止溢油、减少海上.油污染,提出了采用负压保护的可行性方案. 相似文献
749.
简要介绍了济南分公司油气回收装置、真空泵的工作原理以及安装与调试应注意的问题. 相似文献
750.
通过对大连城市环境系统的考察,设立了完整的评价指标体系,运用模糊优选理论建立模糊评价模型,对大连城市环境进行了定量研究,并结合经济和城市化情况进行了分析。研究结果表明:城市环境质量总体上是在逐年提高的,但从2002年以来发展较为平缓。经济和城市化情况有较大发展,但仍有不足之处。 相似文献