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141.
Jinbo Xiong Chaohua Wang Zhiyuan Yao Pingping Zhan Xianghua Yi Jiong Chen 《环境科学学报(英文版)》2023,35(2):429-439
Antibiotic pollution imposes urgent threats to public health and microbial-mediated ecological processes. Existing studies have primarily focused on bacterial responses to antibiotic pollution, but they ignored the microeukaryotic counterpart, though microeukaryotes are functionally important (e.g., predators and saprophytes) in microbial ecology. Herein, we explored how the assembly of sediment microeukaryotes was affected by increasing antibiotic pollution at the inlet (control) and across the outlet sites along a shrimp wastewater discharge channel. The structures of sediment microeukaryotic community were substantially altered by the increasing nutrient and antibiotic pollutions, which were primarily controlled by the direct effects of phosphate and ammonium (−0.645 and 0.507, respectively). In addition, tetracyclines exerted a large effect (0.209), including direct effect (0.326) and indirect effect (−0.117), on the microeukaryotic assembly. On the contrary, the fungal subcommunity was relatively resistant to antibiotic pollution. Segmented analysis depicted nonlinear responses of microeukaryotic genera to the antibiotic pollution gradient, as supported by the significant tipping points. We screened 30 antibiotic concentration-discriminatory taxa of microeukaryotes, which can quantitatively and accurately predict (98.7% accuracy) the in-situ antibiotic concentration. Sediment microeukaryotic (except fungal) community is sensitive to antibiotic pollution, and the identified bioindicators could be used for antibiotic pollution diagnosis. 相似文献
142.
143.
Tu C Ma LQ Zhang W Cai Y Harris WG 《Environmental pollution (Barking, Essex : 1987)》2003,124(2):223-230
Arsenic speciation is important not only for understanding the mechanisms of arsenic accumulation and detoxification by hyperaccumulators, but also for designing disposal options of arsenic-rich biomass. The primary objective of this research was to understand the speciation and leachability of arsenic in the fronds of Chinese brake (Pteris vittata L.), an arsenic hyperaccumulator, with an emphasis on the implications for arsenic-rich biomass disposal. Chinese brake was grown for 18 weeks in a soil spiked with 50 mg As kg(-1) as arsenate (AsO4(3-)), arsenite (AsO3(3-)), dimethylarsinic acid (DMA), or methylarsonic acid (MMA). Plant samples were extracted with methanol/water (1:1) and arsenic speciation was performed using high performance liquid chromatography coupled with atomic fluorescence spectrometry. The impacts of air-drying on arsenic species and leachability in the fronds were examined in the laboratory. After 18 weeks, water-soluble arsenic in soil was mainly present as arsenate with little detectable organic species or arsenite regardless of arsenic species added to the soil. However, arsenic in the fronds was primarily present as inorganic arsenite with an average of 94%. Arsenite re-oxidation occurred in the old fronds and the excised dried tissues. Arsenic species in the fronds were slightly influenced by arsenic forms added to the soil. Air-drying of the fronds resulted in leaching of substantial amounts of arsenic. These findings can be of significance when looking at disposal options of arsenic-rich biomass from the point of view of secondary contamination. 相似文献
144.
Hongjun Chen Chunhu Yu Zeyang Xue Pengxiang Wang Zi Wang Qianmin Cong 《毒物与环境化学》2020,102(7-8):356-385
Abstract Lithium-doped bismuth oxide nanoplates with the thickness of 50–150?nm and tetragonal bismuth oxide, monoclinic lithium bismuthate phases have been synthesized via a simple hydrothermal process using lithium acetate and sodium bismuthate as the raw materials. Cobalt nanoparticles modified lithium-doped bismuth oxide nanoplates hybrids were obtained by an in situ photo-deposition route. The cobalt nanoparticles-modified nanoplates hybrids display significantly enhanced photocatalytic activity toward gentian violet compared with the nanoplates. Gentian violet solution can be totally degraded by the hybrids within 60?min under ultraviolet–visible light irradiation. The superior photocatalytic activity of the cobalt nanoparticles modified nanoplates hybrids originates from the superior charge transfer capacity and the energy band structure of the hybrids. The excellent photocatalytic performance makes the cobalt nanoparticles modified nanoplates hybrids a promising candidate as the photocatalyst for wastewater treatment. 相似文献
145.
利用海南省水文局提供的1960—2000年水文资料,对近40年来海南省三大河下游水体的含沙量特征及影响因素进行了分析。结果表明,南渡江、昌化江和万泉河下游水体4—11月份的含沙量一般都较大,而1、2、3、12月份的含沙量都很小,夏秋两季的含沙量明显高于冬春两季,这也跟三大河下游地区的不同月份和季节性平均降雨量分布规律基本相一致,说明降雨在一定程度上决定着三大河流域的土壤侵蚀状况。从年平均含沙量来看,昌化江的含沙量整体明显高于南渡江和万泉河,这可能是昌化江流域原始森林的破坏引起水土流失等自然灾害向下游输送泥沙的结果。 相似文献
146.
五指山不同海拔高度的土壤化学性质特征 总被引:4,自引:0,他引:4
根据海南省五指山2003年土壤样品的分析结果,对不同海拔高度下五指山土壤的化学性质特征进行了分析。结果表明,在不同海拔高度下水提pH和盐提pH随采样深度的增加基本呈明显的增大趋势,交换性H 、CEC、全N和有机质随采样深度的增加基本呈明显的下降趋势;而交换性Al3 和交换性酸除在720m、894m处剖面外,其它海拔高度下也基本随采样深度的增加而明显降低。从化学过程较为活跃的表层土壤来看,水提pH、盐提pH、交换性H、交换性Al3 和交换性酸随海拔高度的增加并没有明显的同时增大或减小的分布规律,而CEC、全N和有机质有明显的增加趋势。 相似文献
147.
陵水普通野生稻(Oryza rufipogon)内生菌的固氮及溶磷特行 总被引:10,自引:0,他引:10
从陵水普通野生稻中分离了36株内生菌,经乙炔还原法确定22株菌为内生固氮菌,并测定了其溶磷特性.在22株内生固氮菌中,除菌株Ls2不具有溶磷能力外,其余21株菌溶磷能力差异较大,为(0.002±0.01)~(12.7±0.04)μgmL-1.将这些内生固氮菌接种籼型水稻华航1号,除菌株Ls23外,其余菌株均能使接种水稻苗的根、茎长度增加(在α=0.05水平上差异显著).以上研究结果表明,这些菌株在水稻菌肥研制方面具有较大的开发潜力.图2表3参21 相似文献
148.
本文分析了目前我国城市生活垃圾处理处置现状及其存在的主要问题.认为合理处置垃圾,是实现城市资源、环境和经济可持续发展的重要途径.根据我国国情,提出采取适合我国城市生活垃圾处置的措施:即向多元化方向发展,选择从源头分类收集、回收利用;综合利用堆肥、焚烧和卫生填埋等技术,实行分类处理处置;建设垃圾产业化结构和加强垃圾管理体制. 相似文献
149.
Anyun Zhang Zunfang Tu Junrui Shui Jinxin Liu Hongmei Tuo Haoyu Zhang Cong Lin Jingyi Feng Yuxuan Feng Wen Su 《环境科学学报(英文版)》2023,35(2):462-471
Plasmids play a critical role in the dissemination of antimicrobial resistance genes (ARGs), however, a systematical understanding of ARGs originated from plasmids in swine production is currently lacking. Herein, quantitative polymerase chain reaction was applied to determine the prevalence of ten ARGs and the class1 integron gene intI1 of plasmid source in swine manure from 44 farms in Sichuan, Hubei and Hebei provinces, China. All assayed ARGs were observed in plasmid DNA samples, and the average absolute abundance of aac(6’)-Ib-cr, blaNDM, blaCTX-M, optrA, ermB, floR, mcr-1, qnrS, tetM, sul1 and intI1 were 7.09, 2.90, 4.67, 6.62, 7.55, 7.14, 4.08, 4.85, 7.16, 7.11 and 8.07 of 10 log copies/gram, respectively. IntI1 showed a high correlation (r > 0.8, P < 0.01) with the abundance of aac(6’)-Ib-cr and sul1 in swine manure. Moreover, the farm scale (i.e., herd population) and geographical location were not found to be critical factors influencing the absolute abundance of ARGs of plasmid DNA in swine farms. However, the concentrations of florfenicol, Cu, Zn, Fe, total phosphorus (TP) and total potassium (TK) demonstrated a significant correlation with the abundance of several ARGs. Particularly, Cu and Zn had high correlations with optrA and blaCTX-M, respectively. Our results demonstrated that antibiotics, heavy metals and environmental nutrients are likely jointly contributing to the long-term persistence of ARGs in swine production. This study provides insights into the abundance and influencing factors of ARGs from swine manure, which is of significance for assessing and reducing the public health risks in livestock production. 相似文献
150.
Wenjuan Liao Hao-Jie Cui Yaqi Ning Cong Wu Wei Peng Dong Cheng Lichu Yin Weijun Zhou 《环境科学学报(英文版)》2023,35(2):688-698
It has been documented that organic contaminants can be degraded by hydroxyl radicals ( • OH) produced by the activation of H2 O2 by Fe(II)-bearing clay. However, the interfacial electron transfer reactions between structural Fe(II) and H 2 O 2 for • OH generation and its effects on contaminant remediation are unclear. In this study, we first investigated the relation between • OH generation sites and sulfamethoxazole (SMX) degradation by activating H2O2 using nontronite with different reduction extents. SMX (5.2–16.9 μmol/L) degradation first increased and then decreased with an increase in the reduction extent of nontronite from 22% to 62%, while the • OH production increased continually. Passivization treatment of edge sites and structural variation results revealed that interfacial electron transfer reactions between Fe(II) and H 2 O 2 occur at both the edge and basal plane. The enhancement on basal plane interfacial electron transfer reactions in a high reduction extent rNAu-2 leads to the enhancement on utilization efficiencies of structural Fe(II) and H 2 O 2 for • OH generation.However, the • OH produced at the basal planes is less efficient in oxidizing SMX than that of at edge sites. Oxidation of SMX could be sustainable in the H 2 O 2 /rNAu-2 system through chemically reduction. The results of this study show the importance role of • OH generation sites on antibiotic degradation and provide guidance and potential strategies for antibiotic degradation by Fe(II)-bearing clay minerals in H 2 O 2 -based treatments. 相似文献