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Ambient halocarbon mixing ratios in 45 Chinese cities 总被引:4,自引:0,他引:4
Barbara Barletta Simone Meinardi Isobel J. Simpson F. Sherwood Rowland Chuen-Yu Chan Xinming Wang Shichun Zou Lo Yin Chan Donald R. Blake 《Atmospheric environment (Oxford, England : 1994)》2006,40(40):7706-7719
During this study 158 whole air samples were collected in 45 Chinese cities in January and February 2001. The spatial distribution of different classes of halocarbons in the Chinese urban atmosphere, including chlorofluorocarbons (CFCs), hydrochlorofluorocarbons (HCFCs), hydrofluorocarbons (HFCs), Halon-1211, and other chlorinated compounds is presented and discussed. Most of these compounds were enhanced compared to background levels. However, the mean enhancement of CFCs was relatively small, with CFC-12 and CFC-11 increases of 6% (range 1–31%) and 10% (range 2–89%), respectively, with respect to the global background. On the contrary, strongly enhanced levels of CFC replacement compounds and halogenated compounds used as solvents were measured. The average Halon-1211 concentration exceeded the background of 4.3 pptv by 75% and was higher than 10 pptv in several cities. Methyl chloride mixing ratios were also strongly elevated (78% higher than background levels), which is likely related to the widespread use of coal and biofuel in China. 相似文献
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Environmental Chemistry Letters - Microwave irradiation has been intensively studied for environmental remediation, e.g., for wastewater treatment, and for synthesis, to take advantages of the... 相似文献
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“陇中之苦,甲于天下”。这是黄土高原对甘肃定西地区和宁夏的西吉、海原、固原(西海固)的历史性结论。政府和国际援助多年来的努力使这一带的贫困状况有所减轻。但是至今这种状况仍然没有全部改观,特别是在远离城市和道路的深山。“三西”依然是中国最贫困的地区。究其原因,降水少而干旱,是生产效率低下的主因。频繁的旱灾往往使粮食绝收,人畜干渴而死;而夏秋集中的豪雨及多发的冰雹,又往往毁坏农作物和冲毁田地。 相似文献
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High energy gas fracturing (HEGF) technique has been one of central stimulating measures to enhance oil recovery in low permeability reservoirs. But, in recently few years, some serious CO poisoning accidents took place in oilfields here in China. It is very important to reveal the dynamic mechanisms of carbon monoxide flow and diffusion to operating safety during high energy gas fracturing. In this paper, some dynamic mechanisms of carbon monoxide CO flowing inside a oil wellbore and diffusion on the top of the well during high energy gas fracturing were studied with fluid/gas hydrodynamics. The CO flow model within a wellbore and the diffusion model in air were established. The key factors affecting CO flow and diffusion such as wellbore pressure, gas-oil ratio, wind speed, leakage speed, air-permanence were inspected with mathematical simulation. It will be of significance to provide an important guidance for monitoring and preventing CO poisoning accidents during high energy gas fracturing. 相似文献
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Lu Huang Xin Wen Yan Wang Yongde Zou Baohua M Xindi Liao Juanboo Liang Yinbao Wu 《环境科学学报(英文版)》2014,26(10):2001-2006
Effects of antibiotic residues on methane production in anaerobic digestion are commonly studied using the following two antibiotic addition methods:(1) adding manure from animals that consume a diet containing antibiotics, and(2) adding antibiotic-free animal manure spiked with antibiotics. This study used chlortetracycline(CTC) as a model antibiotic to examine the effects of the antibiotic addition method on methane production in anaerobic digestion under two different swine wastewater concentrations(0.55 and 0.22 mg CTC/g dry manure). The results showed that CTC degradation rate in which manure was directly added at 0.55 mg CTC/g(HSPIKE treatment) was lower than the control values and the rest of the treatment groups. Methane production from the HSPIKEtreatment was reduced(p 〈 0.05) by 12% during the whole experimental period and 15% during the first 7 days. The treatments had no significant effect on the pH and chemical oxygen demand value of the digesters, and the total nitrogen of the0.55 mg CTC/kg manure collected from mediated swine was significantly higher than the other values. Therefore, different methane production under different antibiotic addition methods might be explained by the microbial activity and the concentrations of antibiotic intermediate products and metabolites. Because the primary entry route of veterinary antibiotics into an anaerobic digester is by contaminated animal manure, the most appropriate method for studying antibiotic residue effects on methane production may be using manure from animals that are given a particular antibiotic, rather than adding the antibiotic directly to the anaerobic digester. 相似文献
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