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121.
Noriyuki Momoshima Fumio Inoue Jun Shimada 《Journal of environmental radioactivity》2010,101(8):615-621
Atmospheric 85Kr concentration at Fukuoka, Japan was determined by an improved 85Kr analytical method using liquid scintillation counting (LSC). An average value of 1.54 ± 0.05 Bq m−3 was observed in 2008, which is about two times that measured in 1981 at Fukuoka, indicating a 29 mBq y−1 rate of increase as an average for these 27 years. The analytical method developed involves collecting Kr from air using activated charcoal at liquid N2 temperature and purifying it using He at dry ice temperature, followed by Kr separation by gas chromatography. An overall Kr recovery of 76.4 ± 8.1% was achieved when Kr was analyzed in 500-1000 l of air. The Kr isolated by gas chromatography was collected on silica gel in a quartz glass vial cooled to liquid N2 temperature and the activity of 85Kr was measured with a low-background LS counter. The detection limit of 85Kr activity by the present analytical method is 0.0015 Bq at a 95% confidence level, including all propagation errors, which is equivalent with 85Kr in 1.3 l of the present air under the analytical conditions of 72.1% counting efficiency, 0.1597 cps background count rate, and 76.4% Kr recovery. 相似文献
122.
Adsorption characteristics of carbonaceous adsorbents were examined using 1,2,3,4-tetrachlorobenzene, naphthalene and 2,4,6-tribromophenol as adsorbates. The breakthrough and equilibrium adsorption characteristics were evaluated using laboratory-scale adsorption test equipment. A micropore volume of diameter less than 2 nm is the most important factor governing the adsorption capacity of all adsorbates. A kinetic analysis was performed and the adsorption behavior of the adsorbates was analyzed. Diffusion within porous particles controls the adsorption rate in this system, and the diffusion process is a function of pore diffusion. The operating conditions in working incineration facility adsorbers were reviewed and the breakthrough time of these adsorbents in actual adsorbers was estimated using the mass transfer zone method. Information on the optimal operating conditions of adsorbers was derived from the adsorption breakthrough characteristics. 相似文献
123.
124.
Hajime Masukawa Masaharu Kitashima Kazuhito Inoue Hidehiro Sakurai Robert P. Hausinger 《Ambio》2012,41(2):169-173
To mitigate global warming caused by burning fossil fuels, a renewable energy source available in large quantity is urgently required. We are proposing large-scale photobiological H2 production by mariculture-raised cyanobacteria where the microbes capture part of the huge amount of solar energy received on earth’s surface and use water as the source of electrons to reduce protons. The H2 production system is based on photosynthetic and nitrogenase activities of cyanobacteria, using uptake hydrogenase mutants that can accumulate H2 for extended periods even in the presence of evolved O2. This review summarizes our efforts to improve the rate of photobiological H2 production through genetic engineering. The challenges yet to be overcome to further increase the conversion efficiency of solar energy to H2 also are discussed. 相似文献
125.
Lichtfouse Eric Morin-Crini Nadia Bradu Corina Boussouga Youssef-Amine Aliaskari Mehran Schfer Andrea Iris Das Soumya Wilson Lee D. Ike Michihiko Inoue Daisuke Kuroda Masashi Don Sbastien Fievet Patrick Crini Grgorio 《Environmental Chemistry Letters》2022,20(3):2019-2041
Environmental Chemistry Letters - Worldwide contamination of waters by metals, metalloids, and organometallic pollutants is a major health issue. In particular, the occurrence of the selenium... 相似文献