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431.
Scott C. Kronholm Paul D. Capel Silvia Terziotti 《Environmental Modeling and Assessment》2016,21(6):681-690
Accurate estimation of total nitrogen loads is essential for evaluating conditions in the aquatic environment. Extrapolation of estimates beyond measured streams will greatly expand our understanding of total nitrogen loading to streams. Recursive partitioning and random forest regression were used to assess 85 geospatial, environmental, and watershed variables across 636 small (<585 km2) watersheds to determine which variables are fundamentally important to the estimation of annual loads of total nitrogen. Initial analysis led to the splitting of watersheds into three groups based on predominant land use (agricultural, developed, and undeveloped). Nitrogen application, agricultural and developed land area, and impervious or developed land in the 100-m stream buffer were commonly extracted variables by both recursive partitioning and random forest regression. A series of multiple linear regression equations utilizing the extracted variables were created and applied to the watersheds. As few as three variables explained as much as 76 % of the variability in total nitrogen loads for watersheds with predominantly agricultural land use. Catchment-scale national maps were generated to visualize the total nitrogen loads and yields across the USA. The estimates provided by these models can inform water managers and help identify areas where more in-depth monitoring may be beneficial. 相似文献
432.
The significance of metal hyperaccumulation for biotic interactions 总被引:13,自引:0,他引:13
Metal hyperaccumulating plants contain very high metal contents. Because of the general toxicity of metals, chemically-mediated
biotic interactions involving hyperaccumulating plants may differ greatly from those of non-hyperaccumulators. Recent research
has demonstrated a defensive function for hyperaccumulated metals against herbivores and pathogens. We predict that some herbivore/pathogen
species have evolved metal tolerance, and suggest that resulting high metal levels in herbivores/pathogens may defend them
against their own predators. Little is known regarding interference and commensal interactions involving hyperaccumulating
plants. Decreased competition may occur through an interference interaction similar to allelopathy, in which enrichment of
metal in the soil under a hyperaccumulator plant's canopy may inhibit another plant species, thus resulting in “elemental
allelopathy”. Metal enrichment of soil under hyperaccumulators also may result in commensalism if another plant species (possibly
another hyperaccumulator) derives a benefit from growing in the metal-enriched soil under the canopy of a hyperaccumulating
overstory plant. It seems likely that high-metal plant litter will host a specialized microflora of decomposers and may affect
nutrient cycling rates. Mutualist biotic interactions also may be affected by the elevated metal contents of hyperaccumulating
species. Mycorrhizal fungi may form mutualisms with hyperaccumulators, but the phenomenon is poorly-explored. The few cases
investigated to date have not detected mycorrhizae. Pollination and seed dispersal mechanisms may require biotic vectors that
might be affected by plant metal content. Hyperaccumulating plants may have solved this dilemma in three ways. First, some
may rely on abiotic vectors for pollen or seed dispersal. Second, biotic vectors used by these species may have varied diets
and thus dilute metal intake to non-toxic levels. Finally, biotic vectors may have evolved tolerance of elevated dietary levels
of metals, and perhaps have become specialists on hyperaccumulator species.
Received 7 November 1997; accepted 28 December 1997. 相似文献
433.
Laboratory tests of fipronil and its degradation products have revealed acute lethal toxicity at very low concentrations (LC50) of <0.5 microg/L to selected aquatic macroinvertebrates. In streams draining basins with intensive rice cultivation in southwestern Louisiana, USA, concentrations of fipronil compounds were an order of magnitude larger than the LC50. The abundance (rho=-0.64; p=0.015) and taxa richness (r2=0.515, p<0.005) of macroinvertebrate communities declined significantly with increases in concentrations of fipronil compounds and rice-cultivation land-use intensity. Macroinvertebrate community tolerance scores increased linearly (r2=0.442, p<0.005) with increases in the percentage of rice cultivation in the basins, indicating increasingly degraded stream conditions. Similarly, macroinvertebrate community-tolerance scores increased rapidly as fipronil concentrations approached about 1 microg/L. Pesticide toxicity index determinations indicated that aquatic macroinvertebrates respond to a gradient of fipronil compounds in water although stream size and habitat cannot be ruled out as contributing influences. 相似文献
434.
The primary health concern associated with exposures to chromite ore processing residue (COPR)-affected soils is inhalation of hexavalent chromium [Cr(VI)] particulates. Site-specific soil alternative remediation standards (ARSs) are set using soil suspension and dispersion models to be protective of the theoretical excess cancer risk associated with inhalation of soil suspended by vehicle traffic and wind. The purpose of this study was to update a previous model comparison study that identified the 1995 AP-42 particulate emission model for vehicle traffic over unpaved roads and the Fugitive Dust Model (FDM) as the most appropriate model combination for estimating site-specific ARSs. Because the AP-42 model has been revised, we have updated our past evaluation. Specifically, the 2006 AP-42 particulate emissions model; the Industrial Source Complex-Short Term model, version 3 (ISCST3); and the American Meteorological Society/Environmental Protection Agency Regulatory Model (AERMOD) air dispersion models were evaluated, and the results were compared with those from the previously used modeling approaches. Two sites with and two sites without vehicle traffic were evaluated to determine if wind erosion is a significant source of emissions. For the two sites with vehicle traffic, both FDM and ISCST3 produced total suspended particulate (TSP) estimates that were, on average, within a factor of 2 of measured; whereas AERMOD produced estimates that were as much as 5-fold higher than measured. In general, the estimated TSP concentrations for FDM were higher than those for ISCST3. For airborne Cr(VI), the ISCST3 model produced estimates that were only 2- to 8-fold of the measured concentrations, and both FDM and AERMOD estimated airborne Cr(VI) concentrations that were approximately 4- to 14-fold higher than measured. Results using the 1995 AP-42 model were closer to measured than those from the 2006 AP-42 model. Wind erosion was an insignificant contributor to particulate emissions at COPR sites. 相似文献
435.
Geiser LH Ingersoll AR Bytnerowicz A Copeland SA 《Journal of the Air & Waste Management Association (1995)》2008,58(9):1223-1234
Agriculture releases copious fertilizing pollutants to air sheds and waterways of the northwestern United States. To evaluate threats to natural resources and historic rock paintings in remote Hells Canyon, Oregon and Idaho, deposition of ammonia (NH3), nitrogen oxides (NOx), sulfur dioxide (SO2), and hydrogen sulfide (H2S) at five stations along 60 km of the Snake River valley floor were passively sampled from July 2002 through June 2003, and ozone data and particulate chemistry were obtained from the Interagency Monitoring of Protected Visual Environments (IMPROVE) station at Hells Canyon. NH3 concentrations were high; biweekly averages peaked at 5-19 ppb in spring and summer and the nutrient-laden Snake River is a likely source. Fine particulate ammonium nitrate (NH4NO3) averaged 2.6 microg/m3 during the 20% of worst visibility days with winter drainage of air masses from the Snake River Basin and possibly long distance transport from southern California. Other pollutants were within background ranges. NH3 is corrosive to clay-based pictographs; nitrogen deposition can alter natural biotic communities and terrestrial ecosystem processes at levels reported here. 相似文献
436.
地下水铀污染的原位微生物还原与固定:在美国能源部田纳西橡树岭放射物污染现场的试验 总被引:4,自引:0,他引:4
吴唯民 Jack Carley David Watson 顾宝华 Scott Brooks Shelly D. Kelly Kenneth Kemner Joy D. van Nostran 吴力游 许玫英 周集中 罗剑 Erick Cardenas 黃家琪 Matthew W. Fields Terence L. Marsh James M. Tiedje Stefan J. Green Joel E. Kostk Peter K. Kitanidis Philip M. Jardine Craig S. Criddle 《环境科学学报》2011,31(3):449-459
总结了美国斯坦福大学和橡树岭国家实验室等在美国能源部田纳西州橡树岭综合试验基地进行的铀污染原位微生物修复阶段性试验结果.本试验利用微生物以乙醇为电子供体还原地下水和沉积物中的六价铀为不溶解的四价铀,使之原位固定化.随后通过加入溶解氧和硝酸盐来试验微生物还原后的地下水层中还原固定态铀的稳定性.通过预处理和长期间隔注入乙醇... 相似文献
437.
Scott Farrow 《Resources Policy》1987,13(4)
In 1983 Interior Secretary Watt changed the nature of auctions for oil and gas leases on the outer continental shelf by dramatically increasing the acreage offered for lease. The General Accounting Office (GAO) developed the first econometric estimates that this change in policy led to a seven billion nominal dollar loss in the first two years of area-wide leasing. This paper reports regression results from estimating the reduced form of the GAO specification and several alternative specifications. All the specifications indicate no significant effect of the policy change on bonus revenues. 相似文献
438.
Roofing as a source of nonpoint water pollution 总被引:12,自引:0,他引:12
Sixteen wooden structures with two roofs each were installed to study runoff quality for four commonly used roofing materials (wood shingle, composition shingle, painted aluminum, and galvanized iron) at Nacogdoches, Texas. Each roof, either facing NW or SE, was 1.22 m wide x 3.66 m long with a 25.8% roof slope. Thus, there were 32 alternatively arranged roofs, consisting of four roof types x two aspects x four replicates, in the study. Runoff from the roofs was collected through galvanized gutters, downspouts, and splitters. The roof runoff was compared to rainwater collected by a wet/dry acid rain collector for the concentrations of eight water quality variables, i.e. Cu(2+), Mn(2+), Pb(2+), Zn(2+), Mg(2+), Al(3+), EC and pH. Based on 31 storms collected between October 1997 and December 1998, the results showed: (1) concentrations of pH, Cu, and Zn in rainwater already exceed the EPA freshwater quality standards even without pollutant inputs from roofs, (2) Zn and Cu, the two most serious pollutants in roof runoff, exceeded the EPA national freshwater water quality standards in virtually 100% and more than 60% of the samples, respectively, (3) pH, EC, and Zn were the only three variables significantly affected by roofing materials, (4) differences in Zn concentrations were significant among all roof types and between all roof runoff and rainwater samples, (5) although there were no differences in Cu concentrations among all roof types and between roof runoff and rainwater, all means and medians of runoff and rainwater exceeded the national water quality standards, (6) water quality from wood shingles was the worst among the roof types studied, and (7) although SE is the most frequent and NW the least frequent direction for incoming storms, only EC, Mg, Mn, and Zn in wood shingle runoff from the SE were significantly higher than those from the NW; the two aspects affected no other elements in runoff from the other three roof types. Also, Zn concentrations from new wood-shingle roofs were significantly higher than those from aged roofs of a previous study. The study demonstrated that roofs could be a serious source of nonpoint water pollution. Since Zn is the most serious water pollutant and wood shingle is the worst of the four roof types, using less compounds and materials associated with Zn along with good care and maintenance of roofs are critical in reducing Zn pollution in roof runoff. 相似文献
439.
Tetracycline, one of the most widely used antibiotics, is excreted into wastewater after consumption by humans and animals. The focus of this research was to evaluate the fate of tetracycline resistant bacteria in the activated sludge process as a function of tetracycline loading. The studies were conducted with aerobic biological sequencing batch reactors (SBRs). When comparing 250 microgl(-1) tetracycline fed SBRs with parallel SBRs having a background influent wastewater tetracycline concentration of approximately 1 microgl(-1), tetracycline fed reactors were found to have increased concentrations and production rates of tetracycline resistant bacteria, higher net growth rates of resistant bacteria, and higher percentages of tetracycline resistant bacteria, which were amplified by increase in organic loading and growth rates. 相似文献
440.