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排序方式: 共有82条查询结果,搜索用时 31 毫秒
61.
Thomas H. Henderson K. Ulrich Mayer Beth L. Parker Tom A. Al 《Journal of contaminant hydrology》2009,106(3-4):195-211
A popular method for the treatment of aquifers contaminated with chlorinated solvents is chemical oxidation based on the injection of potassium permanganate (KMnO4). Both the high density (1025 gL− 1) and reactivity of the treatment solution influence the fate of permanganate (MnO4) in the subsurface and affect the degree of contaminant treatment. The MIN3P multicomponent reactive transport code was enhanced to simulate permanganate-based remediation, to evaluate the pathways of MnO4 utilization, and to assess the role of density contrasts for the delivery of the treatment solution. The modified code (MIN3P-D) provides a direct coupling between density-dependent fluid flow, solute transport, contaminant treatment, and geochemical reactions. The model is used to simulate a field trial of TCE oxidation in a sandy aquifer that is underlain by an aquitard. Three-dimensional simulations are conducted for a coupled reactive system comprised of ten aqueous components, two mineral phases, TCE (dissolved, adsorbed, and NAPL), reactive organic matter, and including ion exchange reactions. Model parameters are constrained by literature data and a detailed data set from the field site under investigation. The general spatial and transient evolution in observed concentrations of the oxidant, dissolved TCE, and reaction products are adequately reproduced by the simulations. The model elucidates the important role of density-induced flow and transport on the distribution of the treatment solution into NAPL containing regions located at the aquifer–aquitard interface. Model results further suggest that reactions that do not directly affect the stability of MnO4 have a negligible effect on solution density and MnO4 delivery. 相似文献
62.
Biochar, as a soil amendment, can increase concentrations of soil organic matter, especially water-extractable organic carbon (WEOC). This can affect the adsorption-desorption equilibrium between the dissolved solid phases in soil organic matter. Dissolved organic carbon (DOC) represents a small proportion of soil organic matter, but is of significant importance in the soil ecosystem due to its mobility and reactivity. Here, water extracts obtained from twelve non-herbaceous biochars (before, and after, chemical treatment with either H(3)PO(4) or KOH), were tested by Liquid Chromatography - Organic Carbon Detection (LC-OCD) to identify the effects of both pyrolysis conditions and chemical treatments on WEOC content. LC-OCD has the capacity to provide a fingerprint of WEOC, which allows analysis of the various fractions present. WEOC content was affected by both the pyrolysis temperature and the feedstock used. High mineral ash contents deriving from the feedstock can prompt thermochemical reactions of lignocelluloses to produce a relatively high WEOC content, which includes low molecular weight neutrals and humic acids as dominant components. A significant change in WEOC occurred during pyrolysis due to secondary reactions which resulted in a much lower WEOC in the high temperature biochars where fractions of low molecular weight acids and neutrals are dominant. Chemical treatments with H(3)PO(4) or KOH increased WEOC concentration, possibly by promoting hydrolysis reactions on biochar surfaces. These observations assist in assessing the contribution of biochar additions to the soil ecosystem and demonstrate the utility of LC-OCD in providing an understanding of how biochar additions to soil can alter DOC. 相似文献
63.
James K. Henderson Ronald W. Falta David L. Freedman 《Journal of contaminant hydrology》2009,108(1-2):29-45
An analytical model is used to simulate the effects of partial source removal and plume remediation on ethylene dibromide (EDB) and 1,2-dichloroethane (1,2-DCA) plumes at contaminated underground storage tank (UST) sites. The risk posed by EDB, 1,2-DCA, and commingled gasoline hydrocarbons varies throughout the plume over time. Dissolution from the light nonaqueous phase liquid (LNAPL) determines the concentration of each contaminant near the source, but biological decay in the plume has a greater influence as distance downgradient from the source increases. For this reason, compounds that exceed regulatory standards near the source may not in downgradient plume zones. At UST sites, partial removal of a residual LNAPL source mass may serve as a stand alone remedial technique if dissolved concentrations in the source zone are within several orders of magnitude of the applicable government or remedial standards. This may be the case with 1,2-DCA; however, EDB is likely to be found at concentrations that are orders of magnitude higher than its low Maximum Contaminant Level (MCL) of 0.05 μg/L (micrograms per liter). For sites with significant EDB contamination, even when plume remediation is combined with source depletion, significant timeframes may be required to mitigate the impact of this compound. Benzene and MTBE are commonly the focus of remedial efforts at UST sites, but simulations presented here suggest that EDB, and to a lesser extent 1,2-DCA, could be the critical contaminants to consider in the remediation design process at many sites. 相似文献
64.
Johnston FH Hanigan IC Henderson SB Morgan GG Portner T Williamson GJ Bowman DM 《Journal of the Air & Waste Management Association (1995)》2011,61(4):390-398
Epidemiological studies of exposure to vegetation fire smoke are often limited by the availability of accurate exposure data. This paper describes a systematic framework for retrospectively identifying the cause of air pollution events to facilitate a long, multicenter analysis of the public health effects of vegetation fire smoke pollution in Australia. Pollution events were statistically defined as any day at or above the 95th percentile of the 24-hr average concentration of particulate matter (PM). These were identified for six cities from three distinct ecoclimatic regions of Australia. The dates of each event were then crosschecked against a range of information sources, including online newspaper archives, government and research agency records, satellite imagery, and aerosol optical thickness measures to identify the cause for the excess particulate pollution. Pollution events occurred most frequently during summer for cities in subtropical and arid regions and during winter for cities in temperate regions. A cause for high PM on 67% of days examined in the city of Sydney was found, and 94% of these could be attributed to landscape fire smoke. Results were similar for cities in other subtropical and arid locations. Identification of the cause of pollution events was much lower in colder temperate regions where fire activity is less frequent. Bushfires were the most frequent cause of extreme pollution events in cities located in subtropical and arid regions of Australia. Although identification of pollution episodes was greatly improved by the use of multiple sources of information, satellite imagery was the most useful tool for identifying bushfire smoke pollution events. 相似文献
65.
Kirsten A. Henderson Mateus Reis Carolina C. Blanco Valério D. Pillar Rodrigo C. Printes Chris T. Bauch Madhur Anand 《Sustainability Science》2016,11(2):321-330
The forest–grassland mosaics of southern Brazil have been subject to many land use and policy changes over the decades. Like many grasslands around the world, the Campos grasslands are declining with few conservation efforts underway. In contrast, forests receive much attention and many incentives. It is hypothesized that perception of land cover has the potential to shape ecosystems. Here we conduct a questionnaire to further our understanding of decision-making practices that alter landscapes (Campos grassland, Araucaria forest, agriculture and plantation) and direct land policies in the region. Our analysis reveals that plantations are significantly less desirable than the other landscape types. However, plantation land use has increased by 87 % over the past few decades, as a result of industry and government incentives. The proportions of other landscape types have remained consistent over the past two decades. Restoration of native vegetation is not a priority of landowners and restoration would require a financial incentive. 相似文献
66.
Boris Poff Karen A. Koestner Daniel G. Neary Victoria Henderson 《Journal of the American Water Resources Association》2011,47(6):1241-1254
Poff, Boris, Karen A. Koestner, Daniel G. Neary, and Victoria Henderson, 2011. Threats to Riparian Ecosystems in Western North America: An Analysis of Existing Literature. Journal of the American Water Resources Association (JAWRA) 47(6):1241–1254. DOI: 10.1111/j.1752‐1688.2011.00571.x Abstract: A total of 453 journal articles, reports, books, and book chapters addressing threats to riparian ecosystems in western North America were analyzed to identify, quantify, and qualify the major threats to these ecosystems as represented in the existing literature. Publications were identified either as research, policy, literature review, historical comparison, or management papers. All papers were evaluated based on year of publication, area of interest, and type(s) of threats addressed. Research papers, however, were assessed in more depth. The publications ranged from the 1930s to 2010 and addressed the following threats: dams, pollution (point and nonpoint), grazing, land use change, timber harvesting, water diversion, road construction, recreation, mining, groundwater pumping, invasive species, climate change, salinity, fire, insect and diseases, woody encroachment, watershed degradation, elimination of native vegetation, beavers, fire suppression, and fuel management. While the types of threats vary on spatial and temporal scales, some persist through decades in western North America. This analysis shows that grazing has been perceived as a dominant threat since the 1980s, but has been diminishing in the past decade, while invasive species, dams and, in recent years, climate change are increasingly represented in the literature as threats to riparian ecosystems in western North America. 相似文献
67.
Elmira Kujundzic David A. Zander Largus T. Angenent David E. Henderson Shelly L. Miller 《Journal of the Air & Waste Management Association (1995)》2013,63(2):210-218
Abstract The purpose of this study was to assess the effectiveness of a new generation of high-volume, ceiling-mounted high-efficiency particulate air (HEPA)-ultraviolet (UV) air filters (HUVAFs) for their ability to remove or inactivate bacterial aerosol. In an environmentally controlled full-scale laboratory chamber (87 m3), and an indoor therapy pool building, the mitigation ability of air filters was assessed by comparing concentrations of total bacteria, culturable bacteria, and airborne endotoxin with and without the air filters operating under otherwise similar conditions. Controlled chamber tests with pure cultures of aerosolized Mycobacterium parafortuitum cells showed that the HUVAF unit tested provided an equivalent air-exchange rate of 11 hr?1. Using this equivalent air-exchange rate as a design basis, three HUVAFs were installed in an indoor therapy pool building for bioaerosol mitigation, and their effectiveness was studied over a 2-year period. The HUVAFs reduced concentrations of culturable bacteria by 69 and 80% during monitoring periods executed in respective years. The HUVAFs reduced concentrations of total bacteria by 12 and 76% during the same monitoring period, respectively. Airborne endotoxin concentrations were not affected by the HUVAF operation. 相似文献
68.
69.
70.
Jeffrey Trieu Jiayun Yao Kathleen E. McLean Dave M. Stieb Sarah B. Henderson 《Journal of the Air & Waste Management Association (1995)》2020,70(10):1009-1021
ABSTRACT Smoke from burning biomass is an important source of fine particulate matter (PM2.5), but the health risks may not be fully captured by the Canadian Air Quality Health Index (AQHI). In May 2018, the province of British Columbia launched an evidence-based amendment (AQHI-Plus) to improve AQHI performance for wildfire smoke, but the AQHI-Plus was not developed or tested on data from the residential woodsmoke season. This study assesses how the AQHI and AQHI-Plus are associated with acute health outcomes during the cooler seasons of 2010–2017 in British Columbia, Canada. Monthly and daily patterns of temperature and PM2.5 concentrations were used to identify Local Health Areas (LHAs) that were impacted by residential woodsmoke. The effects of the AQHI and AQHI-Plus on five acute health outcomes (including non-accidental mortality, outpatient physician visits, and medical dispensations for cardiopulmonary conditions) were estimated using generalized linear mixed effect models with Poisson distributions adjusted for long- and short-term temperature trends. Values of the Akaike information criterion (AIC) were compared to evaluate whether the AQHI or AQHI-Plus was better fitted to each health outcome. Eleven LHAs were categorized as woodsmoke-impacted. In these LHAs, the AQHI and AQHI-Plus associations with acute health outcomes were sensitive to temperature adjustments. After temperature adjustments, the most consistent associations were observed for the two asthma-specific outcomes where the AQHI-Plus was better fitted than the AQHI. The improved performance of the AQHI-Plus for susceptible populations with asthma is consistent between communities impacted by residential woodsmoke and wildfire smoke. Implications: Canada’s Air Quality Health Index (AQHI) is a three pollutant index used to communicate the short term health impact of degraded air quality. As fine particulate matter (PM2.5) is the lowest weighted pollutant in the AQHI, the index is poorly reflective of woodsmoke impacts. The present analysis found that an AQHI amendment developed for improved sensitivity to PM2.5 during wildfire seasons (AQHI-Plus) is also more predictive of acute asthma-related health outcomes in communities impacted by residential woodsmoke. The BC Ministry of Environment and Climate Change Strategy has piloted the AQHI-Plus year-round. Other jurisdictions should consider whether their air quality indices are reflective of the risks posed by woodsmoke. 相似文献