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11.
Mojgan Bassandeh Alice Antony Pierre Le-Clech Desmond Richardson Greg Leslie 《Chemosphere》2013,90(4):1461-1469
In this study, the efficiency of six ion exchange resins to reduce the dissolved organic matter (DOM) from a biologically treated newsprint mill effluent was evaluated and the dominant removal mechanism of residual organics was established using advanced organic characterisations techniques. Among the resins screened, TAN1 possessed favourable Freundlich parameters, high resin capacity and solute affinity, closely followed by Marathon MSA and Marathon WBA. The removal efficiency of colour and lignin residuals was generally good for the anion exchange resins, greater than 50% and 75% respectively. In terms of the DOM fractions removal measured through liquid chromatography–organic carbon and nitrogen detector (LC–OCND), the resins mainly targeted the removal of humic and fulvic acids of molecular weight ranging between 500 and 1000 g mol?1, the portion expected to contribute the most to the aromaticity of the effluent. For the anion exchange resins, physical adsorption operated along with ion exchange mechanism assisting to remove neutral and transphilic acid fractions of DOM. The column studies confirmed TAN1 being the best of those screened, exhibited the longest mass transfer zone and maximum treatable volume of effluent. The treatable effluent volume with 50% reduction in dissolved organic carbon (DOC) was 4.8 L for TAN1 followed by Marathon MSA – 3.6 L, Marathon 11 – 2.0 L, 21K-XLT – 1.5 L and Marathon WBA – 1.2 L. The cation exchange resin G26 was not effective in DOM removal as the maximum DOC removal obtained was only 27%. The resin capacity could not be completely restored for any of the resins; however, a maximum restoration up to 74% and 93% was achieved for TAN1 and Marathon WBA resins. While this feasibility study indicates the potential option of using ion exchange resins for the reclamation of paper mill effluent, the need for improving the regeneration protocols to restore the resin efficiency is also identified. Similarly, care should be taken while employing LC–OCND for characterising resin-treated effluents, as the resin degradation is expected to contribute some organic carbon moieties misleading the actual performance of resin. 相似文献
12.
Charles E. Billings Leslie Silverman Richard Dennis Lester H. Levenbaum 《Journal of the Air & Waste Management Association (1995)》2013,63(4):318-330
The trends in and relationships between ambient air concentrations of sulfur dioxide and sulfate aerosols at 48 urban sites and 27 nonurban sites throughout the U.S. between 1963 and 1972 have been analyzed. The substantial decreases in ambient SO2 concentrations measured at urban sites in the eastern and midwestern U.S. are consistent with the corresponding reductions in local SO2 emissions, but these decreases have been accompanied by only modest decreases in ambient sulfate concentrations. Large differences in the amounts of SO2 emitted within individual air quality control regions are associated with much smaller differences in the corresponding ambient sulfate concentrations. Substantial changes in the patterns of SO2 emissions between air quality regions result in essentially no differences between ambient sulfate concentrations in those air quality regions. Comparisons of several air quality regions in the eastern and western U.S. with similar SO2 emission levels and patterns of emissions clearly demonstrates the higher ambient sulfate concentration levels in eastern air quality control regions. Relationships between SO2, sulfates, and vanadium concentrations at eastern nonurban U.S. sites cannot be explained by local emission sources. These various observed results can be best explained by long distance sulfur oxide transport with chemical conversion of SO2 to sulfates occurring over ranges of hundreds of kilometers. This conclusion has been suggested earlier and the present analysis strongly supports previous discussions. An impact of long range transport of sulfates is to emphasize the need for Consistent strategies for reduction of sulfur oxides throughout large geographical regions. Additions of large capacities involving elevated sources in mid-continental or western regions could result in significant increases in sulfate concentrations well downwind of such sources. Some of the types of research activities required to quantitate crucial experimental parameters are discussed. 相似文献
13.
Membrane based treatment processes are very effective in removing salt from wastewater, but are hindered by calcium scale deposit formation. This study investigates the feasibility of removing calcium from treated sewage wastewater using accelerated seeded precipitation. The rate of calcium removal was measured during bench scale batch mode seeded precipitation experiments at pH 9.5 using various quantities of calcium carbonate as seed material. The results indicate that accelerated seeded precipitation may be a feasible option for the decrease of calcium in reverse osmosis concentrate streams during the desalination of treated sewage wastewater for irrigation purposes, promising decreased incidence of scaling and the option to control the sodium adsorption ratio and nutritional properties of the desalted water. It was found that accelerated seeded precipitation of calcium from treated sewage wastewater was largely ineffective if carried out without pre-treatment of the wastewater. Evidence was presented that suggests that phosphate may be a major interfering substance for the seeded precipitation of calcium from this type of wastewater. A pH adjustment to 9.5 followed by a 1-h equilibration period was found to be an effective pre-treatment for the removal of interferences. Calcium carbonate seed addition at 10 g l−1 to wastewater that had been pre-treated in this way was found to result in calcium precipitation from supersaturated level at 60 mg l−1 to saturated level at 5 mg l−1. Approximately 90% reduction of the calcium level occurred 5 min after seed addition. A further 10% reduction was achieved 30 min after seed addition. 相似文献
14.
Zhang Xianbing Ding Zhaoxia Yang Juan Cizmas Leslie Lichtfouse Eric Sharma Virender K. 《Environmental Chemistry Letters》2018,16(3):1069-1075
Environmental Chemistry Letters - Humic acids are complex mixtures of organic molecules of different sizes, molecular weights and functional groups such as phenols, carboxyls, quinones and amino... 相似文献
15.
Disturbance by military maneuvers over short and long time scales may have differential effects on grassland communities.
We assessed small mammals as indicators of disturbance by military maneuvers in a mixed prairie in southern Oklahoma USA.
We examined sites on two soil series, Foard and Lawton, across a gradient of disturbance intensity. A MANOVA showed that abundance
of small mammals was associated (p = 0.03) with short-term (cover of vehicle tracks) disturbance but was not associated (p = 0.12) with long-term (loss of soil organic carbon, SOC) disturbance intensity. At the individual species level, Sigmodon hispidus (cotton rat) and Peromyscus maniculatus (deer mouse) occurred across all levels of disturbance and in both soil types. Only P. maniculatus abundance changed (p < 0.01) with short-term disturbance and increased by about one individual per 5% of additional track-cover. Abundance of
P. maniculatus also increased (p = 0.04) by about three individuals per 1% increase in soil carbon. Chaetodipus hispidus (hispid pocket mouse) and Reithrodontomys fulvescens (fulvous harvest mouse) only occurred in single soil types limiting their potential as more general indicators. Abundance
of P. maniculatus was positively related to shifts in plant species composition and likely reflected changes in vegetation structure (i.e.
litter depth) and forage availability resulting from disturbance. Peromyscus maniculatus may be a useful biological indicator of ecosystem change because it responded predictably to both long-term and short-term
disturbance and, when coupled with soil, plant, and disturbance history variables, can reveal land condition trends. 相似文献
16.
17.
Saud A. Amer Timothy O. Keefer Mark A. Weltz David C. Goodrich Leslie B. Bach 《Journal of the American Water Resources Association》1994,30(1):69-83
ABSTRACT: Certain physical and chemical properties of soil vary with soil water content. The relationship between these properties and water content is complex and involves both the pore structure and constituents of the soil solution. One of the most economical techniques to quantify soil water content involves the measurement of electrical resistance of a dielectric medium that is in equilibrium with the soil water content. The objective of this research was to test the reliability and accuracy of fiberglass soil-moisture electrical resistance sensors (ERS) as compared to gravimetric sampling and Time Domain Reflectometry (TDR). The response of the ERS was compared to gravimetric measurements at eight locations on the USDA-ABS Walnut Gulch Experimental Watershed. The comparisons with TDR sensors were made at three additional locations on the same watershed. The high soil rock content (≥45 percent) at seven locations resulted in consistent overestimation of soil water content by the ERS method. Where rock content was less than 10 percent, estimation of soil water was within 5 percent of the gravimetric soil water content. New methodology to calibrate the ERS sensors for rocky soils will need to be developed before soil water content values can be determined with these sensors. 相似文献
18.
The objective of this research was to analyze the retention of acid precipitation as a viable policy issue on the Congressional
agenda during the 1980s. Issue maintenance (a term borrowed from Barbara Nelson's discussion of the four stages associated
with agenda decision making) was examined in relation to a set of issue characteristics originally developed by Roger Cobb
and Charles Elder, i.e., concreteness, social significance, temporal relevance, complexity, and categorical precedence. Each
issue attribute was found to be somewhat useful in explaining the longevity of acid rain as an agenda item although the direction
of influence for two factors, complexity and temporal relevance, was contrary to expectations. It was suggested that a conceptual
merger of this sort could contribute to the comparative analysis of agenda policy decisions by providing a clearer and more
restricted set of decision points to be explained. 相似文献
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