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41.
《Environmental Forensics》2013,14(3-4):349-355
Assessment of environmental damage following accidental oil spills requires reliable oil identification methods. Results from hydrocarbon analyses of environmental samples are often difficult to interpret, because of the changes in oil composition (or weathering) that follows release into the environment, and because of confounding by hydrocarbons from other sources. To a first-order approximation, weathering proceeds according to simple first-order loss-rate (FOLR) kinetics for polycyclic aromatic hydrocarbons (PAH) based on molecular size. This relationship between relative weathering rate and molecular size can be exploited to infer the initial PAH composition of spilled oils, and this information can be combined with results for weathering-invariant analytes to substantially increase the precision and accuracy of hydrocarbon source recognition methods. The approach presented here evaluates a goodness-of-fit metric between the measured hydrocarbon composition of an environmental sample and a suspected source, after correcting for PAR weathering losses based on FOLR kinetics. Variability from analytical and sampling error may thus be accounted for, and source identifications can be expressed as objective probability statements. This approach is illustrated by application to four independent case studies. 相似文献
42.
《Environmental Forensics》2013,14(3-4):279-291
As part of the ongoing work to develop new guidelines for oil spill identification for the European Committee for Standardization (CEN), a Round Robin test was arranged by SINTEF in co-operation with the Norwegian General Standardizing Body (NAS). Twelve laboratories from ten countries participated in the Round Robin study. They include: Denmark, Finland, France, Germany, the Netherlands, Norway, Scotland, Sweden, Wales, and the U.S.A. The analytical methodology used for the Round Robin testing is a result of the ongoing project "Revision of the Nordtest Methodology for Oil Spill Identification". The analytical methodology is described in the AMOP proceedings 2002. Seven oil samples (two artificially weathered "spill" samples and five possible sources) were analyzed following the recommended analytical protocols. The Round Robin study was a "difficult case", because the two spill samples and three of the suspected sources were highly correlated to one another. These samples were from the same oil field in the North Sea, but from different production wells. The present paper summarizes the Round Robin study, and demonstrates the potential of this methodology as a strong technically defensible tool in oil spill identification due to its ability to distinguish qualitatively similar oils from a spill and any available candidate source. 相似文献
43.
44.
George SJ Sherbone J Hinz C Tibbett M 《Environmental pollution (Barking, Essex : 1987)》2011,159(10):2740-2749
Onshore oil production pipelines are major installations in the petroleum industry, stretching many thousands of kilometres worldwide which also contain flowline additives. The current study focuses on the effect of the flowline additives on soil physico-chemical and biological properties and quantified the impact using resilience and resistance indices. Our findings are the first to highlight deleterious effect of flowline additives by altering some fundamental soil properties, including a complete loss of structural integrity of the impacted soil and a reduced capacity to degrade hydrocarbons mainly due to: (i) phosphonate salts (in scale inhibitor) prevented accumulation of scale in pipelines but also disrupted soil physical structure; (ii) glutaraldehyde (in biocides) which repressed microbial activity in the pipeline and reduced hydrocarbon degradation in soil upon environmental exposure; (iii) the combinatory effects of these two chemicals synergistically caused severe soil structural collapse and disruption of microbial degradation of petroleum hydrocarbons. 相似文献
45.
K. M. S. Sundaram S. Y. Szeto 《Journal of environmental science and health. Part. B》2013,48(5):579-599
Abstract An oil‐based formulation of carbaryl (1‐naphthyl N‐methyl‐carbamate) (Sevin‐2‐Oil) was applied twice by a fixed‐wing aircraft at a dosage rate of 280 g of A.I./ha/application to a coniferous forest near Allardville, New Brunswick. The highest concentrations of the chemical in fir foliage, litter and forest soil 1 h after application were respectively 4.20, 1.21 and 0.59 ppm (fresh weight). The residues dissipated rapidly and the DT50 values obtained from the depletion curves were 2.3 d for foliage and 1.5 d for litter and soil samples. Very low levels (<0.1 ppm) of carbaryl persisted in foliage and litter beyond the 10 d sampling period. The maximum residue level found in stream water was 0.314 ppm and more than 50% of it had dissipated within 1 h. Low but detectable levels (0.001 ppm) of the chemical persisted in water until the end of the 10 d sampling period. Sediment samples contained a maximum level of 0.04 ppm, which dissipated below the detection limit within 5 h. Brook trout and slimy sculpins captured in the stream 1 d after the spray contained on average about 0.04 ppm of carbaryl and none of it was found in 3 d postspray samples. 相似文献
46.
Adriana C. Bejarano Jacqueline Michel 《Environmental pollution (Barking, Essex : 1987)》2010,158(5):1561-1569
A large-scale assessment of polycyclic aromatic hydrocarbons (PAHs) from the 1991 Gulf War oil spill was performed for 2002-2003 sediment samples (n = 1679) collected from habitats along the shoreline of Saudi Arabia. Benthic sediment toxicity was characterized using the Equilibrium Partitioning Sediment Benchmark Toxic Unit approach for 43 PAHs (ESBTUFCV,43). Samples were assigned to risk categories according to ESBTUFCV,43 values: no-risk (≤1), low (>1-≤2), low-medium (>2-≤3), medium (>3-≤5) and high-risk (>5). Sixty seven percent of samples had ESBTUFCV,43 > 1 indicating potential adverse ecological effects. Sediments from the 0-30 cm layer from tidal flats, and the >30-<60 cm layer from heavily oiled halophytes and mangroves had high frequency of high-risk samples. No-risk samples were characterized by chrysene enrichment and depletion of lighter molecular weight PAHs, while high-risk samples showed little oil weathering and PAH patterns similar to 1993 samples. North of Safaniya sediments were not likely to pose adverse ecological effects contrary to sediments south of Tanaqib. Landscape and geomorphology has played a role on the distribution and persistence in sediments of oil from the Gulf War. 相似文献
47.
Hosny Khordagui 《Environmental management》1991,15(4):455-459
This article describes and assesses the impact of oil spillage and oil well fires on Kuwait and its surroundings. The marine
ecology of the Arabian Gulf is shown to be relatively resistant to damage from oil spillage. The risks of the contamination
of thermal desalination plants by oil and oil products are assessed, and remedies are suggested. Air pollution from burning
oil wells is described and its consequences are predicted.
Editor’s note: Professor Hosny Khordagui worked as a research scientist at the Environmental and Earth Science Department of the Kuwait
Institute for Scientific Research. The Iraqi invasion of Kuwait on August 2, 1990, led to the permanent loss of most of his
data, research reports, and laboratory equipment, and Prof. Khordagui was constrained to live under the Iraqi occupation for
a few weeks. His article “A Conceptual Approach to the Selection of a Control Measure for Residual Chlorine Discharge in Kuwait
Bay” will appear in a forthcoming issue ofEnvironmental Management. 相似文献
48.
我国部分油田原油生产出砂严重,经常造成集输处理系统的严重磨损和堵塞,储油罐严重积砂,不能实现密闭。储油罐清砂完全靠人工完成,劳动强度大,而且造成环境污染。在海上平台,若采出砂含油量不达标排入海洋,则会给海洋带来严重的污染,因此,采出砂处理是急待解决的问题。文章根据国内外采出砂处理技术调研,介绍了水力旋流器除砂技术原理及工艺和在国外应用实例以及该技术在我国油田的开发应用情况。 相似文献
49.
石油工业废弃物处置及其生物治理趋势 总被引:4,自引:0,他引:4
鉴于我国石油工作者对石油工业废弃物的普遍关注,现在介绍生物治理的基本概念及SPE石油工程师协会中有关含油污泥生物处置的途径及其突出优越性。生物液/固处理工艺(LST)是目前含油污泥处置现场最经济可行的处置方案。这种好氧的LST工艺过程,能够比较充分地代谢和降解石油污泥中的油和脂并大量除去多环芳烃类(PAH)化合物及其它有机化合物,明显地降低了石油废弃物对人、畜的毒害程度。其工艺较简单,操作也简易,凡经此工艺处理后的废弃物不留残毒和后患,因此早已被世界上先进国家的炼油业视为处理含油污泥的有效选择了。石油工业废弃物的生物防治和生物降解工艺较大程度地领先于目前我国现场正在执行的各种处理含油废弃物的处理工艺。 相似文献
50.