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131.
Passive monitoring of nitrogen dioxide in urban air: a case study of Durban metropolis, South Africa
To devise and implement strategies to manage the quality of urban air, a metropolis needs air pollution data on which an air quality management plan can be formulated. Although air pollutants can come from several sources, many reports suggest that nitrogen dioxide from motor vehicle emissions is the major contributor to air pollution in cities. Since vehicles stop or move slowly through traffic intersections, concentrations of nitrogen dioxide (NO(2)) are expected to be relatively high at these sites. Inexpensive Ogawa passive samplers were placed at selected traffic intersections in the Durban Metropolis to trap the NO(2) which was then analysed by a sensitive laboratory-based method. The data obtained by this method was compared with data from sophisticated system comprising an active sampler cum on-line chemiluminescence detector. The sampling was done over a twelve month period to cover all seasons. Statistical analysis of the data showed that there was no significant difference between the means for the two methods. This study has established that an Ogawa passive sampler may be used as an economical and reliable collector for NO(2) in ambient air under varying climatic conditions. Further, the analysis method using a UV-Visible spectrophotometer was sensitive enough to detect NO(2) at the 10-20 ppb level. The cost of the method should be well within the budgets of most municipalities and it would motivate them to develop policies to alleviate traffic congestion. 相似文献
132.
So far little is known about air-soil exchange under any sealed circumstances (e.g., in plastic and glass sheds), which however has huge implications for the soil-air-plant pathways of persistent organic pollutants including organochlorine pesticides (OCPs). A newly designed passive air sampler was tested in a sealed chamber for measuring the vertical concentration profiles of gaseous phase OCPs (hexachlorocyclohexanes (HCHs) and dichlorodiphenyltrichloroethanes (DDTs)). Air was sampled at 5, 15, and 30 cm above ground level every 10th day during a 60-day period by deploying polyurethane foam cylinders housed in acrylonitrile butadiene styrene-covered cartridges. Concentrations and compositions of OCPs along the vertical sections indicated a clear relationship with proximity to the mixture of HCHs and DDTs which escapes from the soils. In addition, significant positive correlations were found between air temperatures and concentrations of HCHs and DDTs. These results indicated revolatilization and re-deposition being at or close to dynamic pseudo-equilibrium with the overlying air. The sampler used for addressing air-soil exchange of persistent organic pollutants in any sealed conditions is discussed. 相似文献
133.
Gilles Billen Vincent Thieu Josette Garnier Marie Silvestre 《Agriculture, ecosystems & environment》2009,133(3-4):234
The watersheds of the Seine, Somme and Scheldt rivers (France, Belgium, the Netherlands), flowing into the continental coastal zone of the English Channel and Southern North Sea, are among the regions of the world with the highest anthropogenic inputs of reactive nitrogen through fertilizer use, legume fixation and deposition of atmospheric nitrogen. They also represent examples of widely open systems, either exporting a large fraction of their N inputs under the form of agricultural products (case of the Seine basin) or importing high amounts of nitrogen as feed for livestock nutrition (case of the Scheldt basin), and delivering up to 2000 kg N km−2 yr−1 at river outlet into the sea. Taking these three watersheds as a case study, we review the different approaches developed so far for describing and predicting the fate of reactive nitrogen inputs to regional systems and its cascade from soils to sea. These approaches range from simple lumped input–output budget, to detailed process-based, spatially distributed models of nutrient transfers. The merits and the limits of these approaches are discussed. Their combination allows to establish a reasonably consistent budget for the three basins, emphasizing the various ‘retention’ terms linked to both landscape and in-stream processes, including storage in long residence time compartments (soil organic matter, vadose zone, aquifers, etc.), denitrification (in soil, riparian zones or river benthos) or sediment burial. Root-zone and riparian denitrification processes appear as major terms of landscape retention in all three investigated watersheds. Retention of nitrogen associated with collection and treatment of urban wastewater is also a major term in the two most populated watersheds. 相似文献
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L. J. Lane M. H. Diskin D. E. Wallace R. M. Dixon 《Journal of the American Water Resources Association》1978,14(5):1143-1158
ABSTRACT: Significant errors in estimating surface runoff and erosion rates are possible if a watershed is assumed to contribute runoff uniformly over the entire area, when actually only a portion of the entire area may be contributing. Generation of overland flow on portions of small semiarid watersheds was analyzed by three methods: an average loss rate procedure, a lumped-linear model, and a distributed-nonlinear model. These methods suggested that, on the average, 45, 60, and 50% of the drainage area was contributing runoff at the watershed outlet. Infiltrometer data support the partial area concept and indicate that the low infiltration zones are the runoff source areas as simulated with the distributed-nonlinear model. 相似文献
138.
EFFECTS OF SPATIAL ORIENTATION OF MULTIPLE PLATE ARTIFICIAL SUBSTRATES ON INVERTEBRATE COLONIZATION1
K. V. Slack R. F. Ferreira R. C. Averert S. S. Kennelly 《Journal of the American Water Resources Association》1988,24(4):781-789
ABSTRACT: Jumbo multiple plate samplers were suspended in a river at 0.3 and 1 m depth in one of three orientations: interplate spaces closed to downwelling light and open to flow, open to light and flow, or open to light and closed to flow. Mean numbers of colonizing taxa and individuals were not significantly different among orientations after eight weeks of submergence. All variables tested decreased significantly with depth. Mean number of taxa, number of individuals (1 m only), and insect diversity decreased between samplings at four and eight weeks for samplers that were closed to light and open to flow. All orientations, depths, and durations had one-half to two-thirds of the total taxa. Colonization was affected by location in the river and position on sampler suspension equipment. The results indicate lack of orientation effects on colonization or high variability that obscured such effects. The sampler suspension equipment possibly increased among-sampler variability by forming artificial snag habitats, and interplate light and flow conditions at different orientations may not have been sufficiently distinct to elicit different biological responses. Individual samplers provided diverse microhabitats regardless of orientation, but it would be prudent to include orientation among the variables considered in use of multiple plate samplers. 相似文献
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