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91.
Sulphate, Nitrogen and Base Cation Budgets at 21 Forested Catchments in Canada, the United States and Europe 总被引:1,自引:0,他引:1
Watmough SA Aherne J Alewell C Arp P Bailey S Clair T Dillon P Duchesne L Eimers C Fernandez I Foster N Larssen T Miller E Mitchell M Page S 《Environmental monitoring and assessment》2005,109(1-3):1-36
To assess the concern over declining base cation levels in forest soils caused by acid deposition, input-output budgets (1990s
average) for sulphate (SO4), inorganic nitrogen (NO3-N; NH4-N), calcium (Ca), magnesium (Mg) and potassium (K) were synthesised for 21 forested catchments from 17 regions in Canada,
the United States and Europe. Trend analysis was conducted on monthly ion concentrations in deposition and runoff when more
than 9 years of data were available (14 regions, 17 sites). Annual average SO4 deposition during the 1990s ranged between 7.3 and 28.4 kg ha−1 per year, and inorganic nitrogen (N) deposition was between 2.8 and 13.8 kg ha−1 per year, of which 41–67% was nitrate (NO3-N). Over the period of record, SO4 concentration in deposition decreased in 13/14 (13 out of 14 total) regions and SO4 in runoff decreased at 14/17 catchments. In contrast, NO3-N concentrations in deposition decreased in only 1/14 regions, while NH4-N concentration patterns varied; increasing at 3/14 regions and decreasing at 2/14 regions. Nitrate concentrations in runoff
decreased at 4/17 catchments and increased at only 1 site, whereas runoff levels of NH4-N increased at 5/17 catchments. Decreasing trends in deposition were also recorded for Ca, Mg, and K at many of the catchments
and on an equivalent basis, accounted for up to 131% (median 22%) of the decrease in acid anion deposition. Base cation concentrations
in streams generally declined over time, with significant decreases in Ca, Mg and K occurring at 8, 9 and 7 of 17 sites respectively,
which accounted for up to 133% (median 48%) of the decrease in acid anion concentration. Sulphate export exceeded input at
18/21 catchments, likely due to dry deposition and/or internal sources. The majority of N in deposition (31–100%; median 94%)
was retained in the catchments, although there was a tendency for greater NO3-N leaching at sites receiving higher (<7 kg ha-1 per year) bulk inorganic N deposition. Mass balance calculations show that export of Ca and Mg in runoff exceeds input at
all 21 catchments, but K export only exceeds input at 16/21 sites. Estimates of base cation weathering were available for
18 sites. When included in the mass balance calculation, Ca, Mg and K exports exceeded inputs at 14, 10 and 2 sites respectively.
Annual Ca and Mg losses represent appreciable proportions of the current exchangeable soil Ca and Mg pools, although losses
at some of the sites likely occur from weathering reactions beneath the rooting zone and there is considerable uncertainty
associated with mineral weathering estimates. Critical loads for sulphur (S) and N, using a critical base cation to aluminium
ratio of 10 in soil solution, are currently exceeded at 7 of the 18 sites with base cation weathering estimates. Despite reductions
in SO4 and H+ deposition, mass balance estimates indicate that acid deposition continues to acidify soils in many regions with losses of
Ca and Mg of primary concern.
The U.S. Government's right to retain a non-exclusive, royalty free licence in and to any copyright is acknowledged.
The Canadian Crown reserves the right to retain a non-exclusive, royalty free licence in and to any copyright. 相似文献
92.
93.
The present work attempts statistical analysis of groundwater quality near a Landfill site in Nagpur, India. The objective
of the present work is to figure out the impact of different factors on the quality of groundwater in the study area. Statistical
analysis of the data has been attempted by applying Factor Analysis concept. The analysis brings out the effect of five different
factors governing the groundwater quality in the study area. Based on the contribution of the different parameters present
in the extracted factors, the latter are linked to the geological setting, the leaching from the host rock, leachate of heavy
metals from the landfill as well as the bacterial contamination from landfill site and other anthropogenic activities. The
analysis brings out the vulnerability of the unconfined aquifer to contamination. 相似文献
94.
汉江水质评价的化学计量学研究 总被引:4,自引:1,他引:4
运用因子分析法对汉江各主要水质断面进行水质因子分析及综合评价,通过各主因子的方差贡献及因子得分得出各水质因子的赋权值,从而对所取断面进行水质污染程度的综合评价、分析与排序。同时运用聚类分析法对汉江17个断面的水质污染相似性进行分析,给出分类处理结果。 相似文献
95.
大气颗粒物中元素碳的直接测定 总被引:4,自引:1,他引:4
对原来用元素分析仪测定大气颗粒物样品中有机碳、元素碳的方法[1 ] 进行改进 ,将差减法间接测定元素碳改为一步直接测定元素碳。有机碳、元素碳的测量标准偏差的平均值分别为 0 35 %、0 34% ,提高了元素碳的测量精度 ,同时避免了误差传递 ,解决了差减法测定元素碳时出现负值的情况。 相似文献
96.
97.
苯胺类化合物含量对还原--偶氮光度法测定硝基苯的影响 总被引:1,自引:0,他引:1
通过将硝基苯和苯胺以不同比例混合制作标准曲线,讨论苯胺类化合物含量对还原-偶氮光度法测定硝基苯的影响。 相似文献
98.
亚铵法制浆造纸厂中段废水处理技术分析研究 总被引:1,自引:0,他引:1
通过对采用两级气浮做预处理 ,生物硫化床串联接触氧化做深度处理的治理技术的分析研究 ,结合废水处理工程实例 ,说明了用两级串联气浮 +硫化床 +接触氧化工艺处理造纸中段水技术切实可靠 ,该治理工艺对处理亚铵法麦草制浆造纸中段废水有较强的针对性和可行性。 相似文献
99.
固相萃取-气相色谱法测定水中硝基苯类有机污染物的方法研究 总被引:3,自引:0,他引:3
建立了固相萃取、毛细柱气相色谱-电子捕获检测器定量分析水中硝基苯类化合物的分析方法。通过对固相萃取柱的选择、固相萃取条件(样品溶液的pH值、上样速度、上样体积、洗脱液选择及配比)的优化,得出了最佳实验条件。穿透体积可达1.5L,回收率在80%~105%,最小检出浓度在0.00037~0.072μg/L之间,均大大低于GB13194-91的规定。相对标准偏差在0.7%~5.3%之间。该方法准确、简单,重现性好、回收率高,污染小。 相似文献
100.
《中国环境监测》于2006年8月第22卷第4期发表了一篇名为“碱性高锰酸钾指数标准分析方法的错误”的文章,该文作者通过配制不同浓度的葡萄糖标准溶液,分别用酸性法与碱性法来测定其高锰酸盐指数值,对相应的结果与计算公式进行讨论,指出碱性高锰酸钾操作方法与计算公式均存在错误,并提出了碱性高锰酸钾测定的修正方法与公式。文章对上述观点和结论有不同的看法,从碱性高锰酸钾指数标准分析方法的试验操作步骤及方法原理的理解入手,进行相关的阐述和讨论。 相似文献