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Lidia Pino Cristina ItalianoAntonio Vit Concetto FabianoVincenzo Recupero 《环境科学学报(英文版)》2016,28(10):138-150
Sorbents for CO_2 capture have been prepared by wet impregnation of a commercial active carbon(Ketjen-black, Akzo Nobel) with two CO_2-philic compounds, polyethylenimine(PEI)and tetraethylenepentamine(TEPA), respectively. The effects of amine amount(from 10 to70 wt.%), CO_2 concentration in the feed, sorption temperature and gas hourly space velocity on the CO_2 capture performance have been investigated. The sorption capacity has been evaluated using the breakthrough method, with a fixed bed reactor equipped with on line gas chromatograph. The samples have been characterized by N_2 adsorption–desorption,scanning electron microscopy and energy dispersive X-ray(SEM/EDX). A promising CO_2 sorption capacity of 6.90 mmol/gsorbenthas been obtained with 70 wt.% of supported TEPA at 70℃ under a stream containing 80 vol% of CO_2. Sorption tests, carried out with simulated biogas compositions(CH_4/CO_2mixtures), have revealed an appreciable CO_2 separation selectivity; stable performance was maintained for 20 adsorption–desorption cycles. 相似文献
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Kazuhiro Okabe Hiroshi Mano Yuichi Fujioka 《International Journal of Greenhouse Gas Control》2008,2(4):485
A novel process for carbon dioxide (CO2) separation, which was named a membrane flash process, was developed to realize an energy-saving technology and to substitute it for a conventional regenerator. The electric energy for CO2 recovery in a membrane flash process using aluminum oxide and diethanolamine was lower than the thermal energy of the conventional chemical absorption process. Flashing at elevated temperature by the low temperature energy significantly reduced the electric energy and required much less membrane area. This process has potentiality of low cost capture of CO2 when the low temperature energy, which is not available for other purposes, can be utilized to elevate flashing temperature. 相似文献
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废弃半导体存储介质一方面载有隐私信息,需要被安全销毁,另一方面富含金属导体、半导体、绝缘体材料,极具回收价值。提出用破碎-风力-高压静电分选系统对其进行安全销毁和物料分选,其中多级破碎部分使信息半导体硅存储材料破碎至0.80 mm以下,而风力-高压静电分选部分能实现半导体、导体、绝缘体的分选。为确定系统工艺参数,实验对风机蝶阀角度(α),风机频率(f),电选电压(U),电选机转辊转速(n)等因素对半导体收集量(M)的影响进行研究,通过因子设计建立了非线性数学模型:M=1.943 8-0.418 7α*+0.306 2f*-0.193 7 f*U*n*+0.181 3α*f*U。进而通过响应优化得出最优工艺参数设置为:α=30°,f=45 Hz,U=30 kV,n=40 r·min-1。在此参数下,金属导体收集率达90.3%,半导体硅收集率达61.0%,实现了半导体存储介质破碎销毁和物料分选。 相似文献
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Jennifer J. Harrison Atun ZawadzkiRobert Chisari Henri K.Y. Wong 《Journal of environmental radioactivity》2011,102(10):896-900
A technique for the isolation of thorium (Th), plutonium (Pu), americium (Am), uranium (U) and strontium (Sr) isotopes from various environmental matrices has been adapted from a previously published method specific to water samples (Maxwell, 2006). Separation and isolation of the various elemental fractions from a single sub-sample is possible, thereby eliminating the need for multiple analyses.The technique involves sample dissolution, concentration via calcium phosphate co-precipitation, rapid column extraction using TEVA™, TRU™ and Sr-Spec™ resin cartridges, alpha spectrometry for Th, Pu, U and Am and Cerenkov counting for Sr.Various standard reference materials were analysed and chemical yields are in the range of 70-80% for Th, Am, U and Sr and 50-60% for Pu. Sample sizes of up to 10 L for water, 5 g for dry soil and sediment and 10 g for dry vegetation and seaweed can be processed using this technique. 相似文献
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This paper is the second installment of a paper published on Process Safety and Environment Protection in 2013, which evaluates the Air-Fin-Cooler (AFC) forced ventilation effect over natural ventilation inside congested LNG process train, i.e., modularized LNG, considering the Air Change per Hour (ACH) using Computational Fluid Dynamics (CFD) analysis. This second paper evaluates the effect of forced ventilation on gas cloud dispersion using CFD in order to evaluate possible design measures, such as safety distance in trains and whether to shut down the AFC in case of releases. The results of this evaluation show that gas cloud accumulation is reduced by AFC induced air flow in the case of shorter separation distances between modules. Based on the results, two design measures are proposed, i.e., keep AFC running during emergency and train orientation against prevailing wind direction. 相似文献
39.
石油开采、炼制及储存过程中含油污泥的综合处理 总被引:1,自引:0,他引:1
张显安 《石油化工环境保护》2006,29(4):38-40
主要介绍石油开采、炼制、储存过程中产生的石油油泥的处理和回收利用。油泥经化学水洗调质处理后,通过特殊的分离沉降罐与卧式离心机和碟式离心机分别配合使用达到降低分离难度,提高工艺适应性和获得良好的油、水、泥分离效果。 相似文献
40.
Determination of respiration, gross nitrification and denitrification in soil profile using BaPS system 总被引:6,自引:0,他引:6
A facility of BaPS (Barometric Process Separation) was used to determine soil respiration, gross nitrification and denitrification in a winter wheat field with depths of 0-7, 7--14 and 14-21 cm. N2O production was determined by a gas chromatograph. Crop root mass and relevant soil parameters were measured. Results showed that soil respiration and gross nitrification decreased with the increase of soil depth, while denitrification did not change significantly. In comparison with no-plowing plot, soil respiration increased significantly in plowing plot, especially in the surface soil of 0-7 cm, while gross nitrification and denitrification rates were not affected by plowing. Cropping practice in previous season was found to affect soil gross nitrification in the following wheat-growing season. Higher gross nitrification rate occurred in the filed plot with preceding crop of rice compared with that of maize for all the three depths of 0-7, 7-14 and 14-21 cm. A further investigation indicated that the nitrification for all the cases accounted for about 76% of the total nitrogen transformation processes of nitrification and denitrification and the N2O production correlated with nitrification significantly, suggesting that nitrification is a key process of soil N2O production in the wheat field. In addition, the variations of soil respiration and gross nitrification were exponentially dependent on root mass (p〈0.00l). 相似文献