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文章介绍了聚合硫酸铁的制备,并用不同的原料合成了几种聚合硫酸铁产品,讨论了影响产品性能的因素。同时,将它们用于给水处理和污水处理,取得了较为理想的结果。 相似文献
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以硫酸钡、聚异丁烯为线性混合成膜体系的填料和改性剂,经表面改性,制得具有较强防腐能力的复合型石英表面蚀刻保护涂料,通过正交实验设计确定了涂料组分配比和配制工艺.以载玻片为底材模拟蚀刻加工过程,进行了HF和NH4HF2混合酸(4∶1)的浸渍比检测,并考察了涂层的热稳定性.结果表明,线型混合体系中m(PS)(硬组分)和m(SBs)(软组分)质量比、w(改性剂)及w(填料)用量分别为1∶1,1.67%,2%,在60 ℃~80 ℃的浸渍温度下,浸渍比(W)为63.9,涂层可耐热到300℃,且对饱和氟化氢、氟化氢铵溶液等强腐蚀性介质有较好的化学稳定性. 相似文献
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Transport and transformation of sulfur compounds over East Asia during the TRACE-P and ACE-Asia campaigns 总被引:4,自引:0,他引:4
Meigen Zhang Itsushi Uno Yasuhiro Yoshida Yongfu Xu Zifa Wang Hajime Akimoto Timothy Bates Trish Quinn Alan Bandy Byron Blomquist 《Atmospheric environment (Oxford, England : 1994)》2004,38(40):6947
On the basis of the recently estimated emission inventory for East Asia with a resolution of 1×1°, the transport and chemical transformation of sulfur compounds over East Asia during the period of 22 February through 4 May 2001 was investigated by using the Models-3 Community Multi-scale Air Quality (CMAQ) modeling system with meteorological fields calculated by the regional atmospheric modeling system (RAMS). For evaluating the model performance simulated concentrations of sulfur dioxide (SO2) and aerosol sulfate (SO42−) were compared with the observations on the ground level at four remote sites in Japan and on board aircraft and vessel during the transport and chemical evolution over the Pacific and Asian Pacific regional aerosol characterization experiment field campaigns, and it was found that the model reproduces many of the important features in the observations, including horizontal and vertical gradients. The SO2 and SO42− concentrations show pronounced variations in time and space, with SO2 and SO42− behaving differently due to the interplay of chemical conversion, removal and transport processes. Analysis of model results shows that emission was the dominant term in regulating the SO2 spatial distribution, while conversion of SO2 to SO42− in the gas phase and the aqueous phase and wet removal were the primary factors that controlled SO42− amounts. The gas phase and the aqueous phase have the same importance in oxidizing SO2, and about 42% sulfur compounds (25% in SO2) emitted in the model domain was transported out, while about 57% (35% by wet removal processes) was deposited in the domain during the study period. 相似文献
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无机高分子混凝剂的发展与应用 总被引:5,自引:0,他引:5
讨论了不同类型无机高分子混凝剂的混凝机理、生产及应用,并指出了新型混凝剂的研制方向. 相似文献
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聚合氯化铝与聚磷硫酸铁絮凝除藻比较研究 总被引:1,自引:0,他引:1
针对武汉市莲花湖湖水,采用聚合氯化铝(PAC)和聚磷硫酸铁(PPFS)进行絮凝实验,比较了两种无机絮凝剂的絮凝效果及原水处理前后藻类群落变化。主要结论如下:①PPFS与PAC的最佳投加量分别为1.5mg/L、2.0mg/L;②PPFS在去除藻类细胞、浊度和色度方面均优于PAC,当PPFS投加过量时,因水体中Fe3+过量分布,使水样色度去除率下降;③PPFS絮凝处理微囊藻为主体的水华原水时,其效果比PAC更好。本文研究后表明:PPFS是一种新型高效絮凝剂,其絮凝性能明显优于PAC,当水体以微型藻类为主时,可使用PPFS以替代PAC,能提高絮凝效果。 相似文献
58.
《环境科学学报(英文版)》2023,35(2):350-359
Sulfite (SO32−) activation is one of the most potential sulfate-radical-based advanced oxidation processes, and the catalysts with high efficiency and low-cost are greatly desired. In this study, the cobalt nanoparticles embedded in nitrogen-doped graphite layers (Co@NC), were used to activate SO32− for removal of Methyl Orange in aqueous solution. The Co@NC catalysts were synthesized via pyrolysis of Co2+-based metal-organic framework (Co-MOF), where CoO was firstly formed at 400℃ and then partially reduced to Co nanoparticles embedded in carbon layers at 800℃. The Co@NC catalysts were more active than other cobalt-based catalysts such as Co2+, Co3O4 and CoFe2O4, due to the synergistic effect of metallic Co and CoxOy. A series of chain reaction between Co species and dissolved oxygen was established, with the production and transformation of SO3•−, SO52−, and subsequent active radicals SO4•− and HO•. In addition, HCO3− was found to play a key role in the reaction by complexing with Co species on the surface of the catalysts. The results provide a new promising strategy by using the Co@NC catalyst for SO32− oxidation to promote organic pollutants degradation. 相似文献
59.
Sulfate aerosol contributes to particulate matter pollution and plays a key role in aerosol radiative forcing, impacting human health and climate change. Atmospheric models tend to substantially underestimate sulfate concentrations during haze episodes, indicating that there are still missing mechanisms not considered by the models. Despite recent good progress in understanding the missing sulfate sources, knowledge on different sulfate formation pathways during polluted periods still involves large uncertainties and the dominant mechanism is under heated debate, calling for more field, laboratory, and modeling work. Here, we review the traditional sulfate formation mechanisms in cloud water and also discuss the potential factors affecting multiphase S(Ⅳ) oxidation. Then recent progress in multiphase S(Ⅳ) oxidation mechanisms is summarized. Sulfate formation rates by different prevailing oxidation pathways under typical winter-haze conditions are also calculated and compared. Based on the literature reviewed, we put forward control of the atmospheric oxidation capacity as a means to abate sulfate aerosol pollution. Finally, we conclude with a concise set of research priorities for improving our understanding of sulfate formation mechanisms during polluted periods. 相似文献
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Bin Liang Deyong Kong Mengyuan Qi Hui Yun Zhiling Li Ke Shi E Chen Alisa S. Vangnai Aijie Wang 《Frontiers of Environmental Science & Engineering》2019,13(6):84