The spatial and temporal distribution of total ozone over China

In this paper the grid data of total ozone mapping spectrograph (TOMS) installed on Nimbus-7 satellite (1978 to 1994) was used and the spatial and temporal distribution of total ozone over China was analyzed. The research indicates that the Qinghai-Tibet Plateau destroyed the latitudinal distribution of total ozone of China and the low value closed center emerged over Qinghai-Tibet Plateau. Long time change trends of seasonal total ozone of Qinghai-Tibet plateau are provided. It shows that the most obvious decrease of total ozone occurs in winter (Jan.), then in summer (Jul.), the relevant slow change occurs in autumn (Oct.) and spring (Apr.).     

Connecting sources, fractions and algal availability of sediment phosphorus in shallow lakes: An approach to the criteria for sediment phosphorus concentrations

Although point and nonpoint sources contribute roughly equal nutrient loads to lakes, their relative role in supporting algae growth has not been clarified. In this research, we have established a quantitative relationship between algae-available phosphorus (P) and P chemical fractions in sediments; the latter indicates the relative contribution of point versus nonpoint sources. Surface sediments from three large shallow lakes in eastern China, namely, the Chaohu, Taihu and Hongzehu Lakes, were sampled to assess their algae-available P and chemically extracted P fractions. The algae-available P primarily comes from iron/aluminium (hydr)oxide-bound P (Fe/Al-bound P), 45% of which is algae-available P. The ratio of Fe/Al-bound P to calcium compound-bound P (Ca-bound P) indicated the relative contribution of point to nonpoint sources, with the point sources contributing the majority of increased Fe/Al-bound P in sediments. Therefore, the reduction of point sources from urbanized areas, rather than nonpoint sources from agricultural areas that primarily contribute to the Ca-bound P fraction, should be prioritized to alleviate cyanobacterial algal blooms (CyanoHABs) in shallow lakes with sediment P as a potential source to support algae growth. With these important results, we proposed a conceptual model for “P-pumping suction” from sediments to algae to aid in the development of the criteria for sediment P concentrations in shallow lakes.     

国际环境保护公约中技术转让障碍问题的探讨

随着世界各国对全球资源与环境问题认识的逐步提高 ,发展中国家必将签署越来越多的国际环境公约 ,参与到国际环境保护合作中。尽管许多国际环境公约都明确规定了发达国家在资金和技术上支持发展中国家保护环境履行国际公约的义务 ,但是实际履约过程中技术转让的问题并未得到良好的解决。论文将讨论国际环境公约履约中的技术转让障碍问题 ,并以中国履行《关于消耗臭氧层物质的蒙特利尔议定书》 ,实施臭氧层保护行动过程中所存在的实际问题为例 ,对国际环境公约履行中技术转让障碍的原因及其后果进行分析 ,最后对发展中国家所应采取的立场和对策提出建议。     

Spatial and temporal distribution of total ozone over China

In this paper the grid data of total ozone mapping spectrograph (TOMS) installed on Nimbus 7 satellite (1978 to 1994) was used and the spatial and temporal distribution of total ozone over China was analyzed. The research indicates that the Qinghai Tibet Plateau destroyed the latitudinal distribution of total ozone of China and the low value closed center emerged over Qinghai Tibet Plateau. Long time change trends of seasonal total ozone of Qinghai Tibet Plateau are provided. It shows that the most obvious decrease of total ozone occurs in winter (Jan.), then in summer (Jul.), the relevant slow change occurs in autumn (Oct.) and spring (Apr.).     

Catalysts for decomposing ozone tail gas

The preparation of immobilizing-catalysts for decomposing ozone by using dipping method was studied. XRD, XPS and TEM were used to characterize the catalysts. The three kinds of catalysts were selected preferentially, and their catalytic activities were investigated. The results showed that the catalyst with activated carbon dipping acetate( active components are Mn:Cu = 3:2, active component proportion in catalyst is 15%, calcination temperature is 200℃ ) has the best catalytic activity for ozone decomposing. One gram of catalyst can decompose 17.6g ozone at initial ozone concentration of 2.5g/m^3 and the residence time in reactor of 0.1s. The experimental results also indicated that humidity of reaction system had negative effect on catalytic activity.     

臭氧控制膜污染的研究进展

本文对臭氧在控制膜污染方面的研究现状进行了综述,重点放在臭氧用于膜冲洗和臭氧用于过滤液预处理这两个方面;指明了在一定的条件下,臭氧可以有效地减缓、降低膜污染;臭氧控制膜污染的作用主要通过臭氧降解造成膜污染的有机物质来实现.此外,还介绍了一些臭氧与膜联用的开发应用情况.     

碱性环境中臭氧破解污泥的效果研究

实验研究发现,在碱性环境中臭氧破解污泥的效果下降;将污泥pH调至11,24 h后,MLSS减少率=38.3%、MLVSS减少率=45.1%;通入臭氧18 min后,MLSS减少率=18.3%、MLVSS减少率=27.2%;污泥减量过程中pH呈下降趋势.     

臭氧-生物活性炭深度处理黄浦江水源水中试研究

以黄浦江水源水厂的滤后水为试验对象，进行饮用水O3-BAC深度处理工艺影响因素的中试研完。针对进水水质的试验结果表明，最优臭氧投加量为3mg／L左右，空床停留时间为15min左右。试验结果可为工程设计提供有益的参考。     

The GaNE programme in a global perspective

This paper provides the background to this special issue, outlining the extent to which the global atmospheric nitrogen cycle has been modified by human activity and outlining the range of effects. The global total emissions of reduced and oxidized nitrogen, amount to 124 Tg N, and exceed those from natural sources (34 Tg N) by almost a factor of four showing the extent to which anthropogenic activity has taken over the global N cycle. Of the 124 Tg N, 70 Tg N is emitted in the oxidized form, largely as NO and 70% of which results directly from anthropogenic activity. The remaining 54 Tg N is emitted as NH₃, (66% anthropogenic). The enhanced nitrogen emissions are associated with a range of local, regional and global issues including, acidification, eutrophication, climate change, human health and tropospheric O₃. The paper also places the Global Nitrogen Enrichment (GaNE) research programme in the UK in a wider perspective.     

低浓度臭氧在含钴盐硅胶上的吸附研究

常压下对含钴盐硅胶进行低浓度臭氧的吸附实验，吸附达到饱和后用氮气作为载气加热解吸。结果显示，含钴盐的硅胶对臭氧具有较强的吸附能力；臭氧解吸量随着解吸温度的上升而增加；吸附了臭氧的含钴硅胶粒子在常温(313．15K)下可在60min内不问断解吸出臭氧。