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271.
Geological CO2 capture and storage (CCS) is among the main near-term contenders for addressing the problem of global climate change. Even
in a baseline scenario, with no comprehensive international climate policy, a moderate level of CCS technology is expected
to be deployed, given the economic benefits associated with enhanced oil and gas recovery. With stringent climate change control,
CCS technologies will probably be installed on an industrial scale. Geologically stored CO2, however, may leak back to the atmosphere, which could render CCS ineffective as climate change reduction option. This article
presents a long-term energy scenario study for Europe, in which we assess the significance for climate policy making of leakage
of CO2 artificially stored in underground geological formations. A detailed sensitivity analysis is performed for the CO2 leakage rate with the bottom-up energy systems model MARKAL, enriched for this purpose with a large set of CO2 capture technologies (in the power sector, industry, and for the production of hydrogen) and storage options (among which
enhanced oil and gas recovery, enhanced coal bed methane recovery, depleted fossil fuel fields, and aquifers). Through a series
of model runs, we confirm that a leakage rate of 0.1%/year seems acceptable for CCS to constitute a meaningful climate change
mitigation option, whereas one of 1%/year is not. CCS is essentially no option to achieve CO2 emission reductions when the leakage rate is as high as 1%/year, so more reductions need to be achieved through the use of
renewables or nuclear power, or in sectors like industry and transport. We calculate that under strict climate control policy,
the cumulative captured and geologically stored CO2 by 2100 in the electricity sector, when the leakage rate is 0.1%/year, amounts to about 45,000 MtCO2. Only a little over 10,000 MtCO2 cumulative power-generation-related emissions are captured and stored underground by the end of the century when the leakage
rate is 1%/year. Overall marginal CO2 abatement costs increase from a few €/tCO2 today to well over 150 €/tCO2 in 2100, under an atmospheric CO2 concentration constraint of 550 ppmv. Carbon costs in 2100 turn out to be about 40 €/tCO2 higher when the annual leakage rate is 1%/year in comparison to when there is no CO2 leakage. Irrespective of whether CCS deployment is affected by gradual CO2 seepage, the annual welfare loss in Europe induced by the implementation of policies preventing “dangerous anthropogenic
interference with the climate system” (under our assumption, implying a climate stabilisation target of 550 ppmv CO2 concentration) remains below 0.5% of GDP during the entire century.
相似文献
Koen SmekensEmail: |
272.
273.
Charcoal versus LPG grilling: A carbon-footprint comparison 总被引:1,自引:0,他引:1
Undoubtedly, grilling is popular. Britons fire up their barbeques some 60 million times a year, consuming many thousands of tonnes of fuel. In milder climates consumption is even higher, and in the developing world, charcoal continues to be an essential cooking fuel. So it is worth comparing the carbon footprints of the two major grill types, charcoal and LPG, and that was the purpose of the study this paper documents. Charcoal and LPG grill systems were defined, and their carbon footprints were calculated for a base case and for some plausible variations to that base case. In the base case, the charcoal grilling footprint of 998 kg CO2e is almost three times as large as that for LPG grilling, 349 kg CO2e. The relationship is robust under all plausible sensitivities. The overwhelming factors are that as a fuel, LPG is dramatically more efficient than charcoal in its production and considerably more efficient in cooking. Secondary factors are: use of firelighters, which LPG does not need; LPG's use of a heavier, more complicated grill; and LPG's use of cylinders that charcoal does not need. 相似文献
274.
建立了一种利用活性炭管采样,二硫化碳洗脱,DB-624UI气相色谱柱(30 m×0.25 mm×1.4μm)进行分离,FID检测器检测的测定环氧丙烷和环氧氯丙烷的气相色谱方法。结果显示,环氧丙烷和环氧氯丙烷在0.5~50 mg/L范围内线性关系良好,方法检出限达到了0.026 mg/m3和0.048 mg/m3(以采集4.5 L空气样品计);环氧丙烷平均解析效率84.84%(RSD=1.770),环氧氯丙烷平均解析效率92.07%(RSD=2.270),适用于工作场所中环氧丙烷和环氧氯丙烷的同时测定。 相似文献
275.
Russell LM Rasch PJ Mace GM Jackson RB Shepherd J Liss P Leinen M Schimel D Vaughan NE Janetos AC Boyd PW Norby RJ Caldeira K Merikanto J Artaxo P Melillo J Morgan MG 《Ambio》2012,41(4):350-369
Geoengineering methods are intended to reduce climate change, which is already having demonstrable effects on ecosystem structure and functioning in some regions. Two types of geoengineering activities that have been proposed are: carbon dioxide (CO(2)) removal (CDR), which removes CO(2) from the atmosphere, and solar radiation management (SRM, or sunlight reflection methods), which reflects a small percentage of sunlight back into space to offset warming from greenhouse gases (GHGs). Current research suggests that SRM or CDR might diminish the impacts of climate change on ecosystems by reducing changes in temperature and precipitation. However, sudden cessation of SRM would exacerbate the climate effects on ecosystems, and some CDR might interfere with oceanic and terrestrial ecosystem processes. The many risks and uncertainties associated with these new kinds of purposeful perturbations to the Earth system are not well understood and require cautious and comprehensive research. 相似文献
276.
The concept of CO2 chemo-absorption by sodium hydroxide in a wet scrubber followed by microalgae cultivation was used as a means to reduce the major greenhouse gas. A thermophilic and alkaline tolerable cyanobacterium named Thermosynechococcus CL-1 (TCL-1) was cultivated in continuous system, with a carbonate-bicarbonate buffer as carbon source. The effects of dissolved inorganic carbon (DICin) and nutrient levels in influent on cell mass productivity, DIC removal efficiency, and alkaline solution regeneration by TCL-1 were investigated. The results show the highest cell mass productivity reaches 1.7 g L−1 d−1 under the highest DIC and nutrients level. Conversely, the best regeneration of alkaline solution proceeds from pH 9.5 to 11.3 under the lowest level. In addition, the highest ΔDIC (DIC consumption) and DIC removal efficiency are 42 mM and 43% at 113.2 and 57 mM DICin, respectively. 相似文献
277.
This work focuses on the influence of humic acids (HAs) on the fate of carbon nanotubes (CNTs) in aqueous media. This influence was demonstrated by mixing CNT powder with HAs in aqueous solution in varying concentrations. The aqueous media containing HAs and CNTs were size-characterized by asymmetrical flow field-flow fractionation (AsFlFFF) coupled with multi-angle light scattering (MALS). This coupling yielded information concerning the size distribution of single- and multi-walled CNTs (SWCNTs and MWCNTs) and HAs under different physico-chemical conditions that can occur in environmental water. HAs can disperse individual CNTs in aqueous media. However, the difference in the physical structure between SWCNTs and MWCNTs leads to significant differences in the quantity of HA that can adsorb onto the nanotube surface and in the stability of the CNT/HA complex. Compared with MWCNTs, SWCNTs suspended in HAs are less affected by changing ionic strength with respect to stability and the amount suspended. 相似文献
278.
The volume of industrial and domestic wastewater is increasing significantly year by year with the change in the lifestyle based on mass consumption and mass disposal brought about by the dramatic development of economies and industries. Therefore, effective advanced wastewater treatment is required because wastewater contains a variety of constituents such as particles, organic materials, and emulsion depending on the resource. However, residual chemicals that remain during the treatment of wastewaters form a variety of known and unknown by-products through reactions between the chemicals and some pollutants. Chronic exposure to these by-products or residual chemicals through the ingestion of drinking water, inhalation and dermal contact during regular indoor activities (e.g., showering, bathing, cooking) may pose cancer and non-cancer risks to human health. For example, residual aluminium salts in treated water may cause Alzheimer's disease (AD). As for carbon nanotubes (CNTs), despite their potential impacts on human health and the environment having been receiving more and more attention in the recent past, existing information on the toxicity of CNTs in drinking water is limited with many open questions. Furthermore, though general topics on the human health impacts of traditional water treatment chemicals have been studied, no comparative analysis has been done. Therefore, a qualitative comparison of the human health effects of both residual CNTs and traditional water treatment chemicals is given in this paper. In addition, it is also important to cover and compare the human health effects of CNTs to those of traditional water treatment chemicals together in one review because they are both used for water treatment and purification. 相似文献
279.
The role of nitrogen (N) in acidification of soil and water has become relatively more important as the deposition of sulphur has decreased. Starting in 1991, we have conducted a whole-catchment experiment with N addition at Gårdsjön, Sweden, to investigate the risk of N saturation. We have added 41 kg N ha−1 yr−1 as NH4NO3 to the ambient 9 kg N ha−1 yr−1 in fortnightly doses by means of sprinkling system. The fraction of input N lost to runoff has increased from 0% to 10%. Increased concentrations of NO3 in runoff partially offset the decreasing concentrations of SO4 and slowed ecosystem recovery from acid deposition. From 1990-2002, about 5% of the total N input went to runoff, 44% to biomass, and the remaining 51% to soil. The soil N pool increased by 5%. N deposition enhanced carbon (C) sequestration at a mean C/N ratio of 42-59 g g−1. 相似文献
280.
Górka M Sauer PE Lewicka-Szczebak D Jędrysek MO 《Environmental pollution (Barking, Essex : 1987)》2011,159(1):294-301
This paper describes results of chemical and isotopic analysis of inorganic carbon species in the atmosphere and precipitation for the calendar year 2008 in Wroc?aw (SW Poland). Atmospheric air samples (collected weekly) and rainwater samples (collected after rain episodes) were analysed for CO2 and dissolved inorganic carbon (DIC) concentrations and for δ13C composition. The values obtained varied in the ranges: atmospheric CO2: 337-448 ppm; δ13CCO2 from −14.4 to −8.4‰; DIC in precipitation: 0.6-5.5 mg dm−3; δ13CDIC from −22.2 to +0.2‰. No statistical correlation was observed between the concentration and δ13C value of atmospheric CO2 and DIC in precipitation. These observations contradict the commonly held assumption that atmospheric CO2 controls the DIC in precipitation. We infer that DIC is generated in ambient air temperatures, but from other sources than the measured atmospheric CO2. The calculated isotopic composition of a hypothetical CO2 source for DIC forming ranges from −31.4 to −11.0‰, showing significant seasonal variations accordingly to changing anthropogenic impact and atmospheric mixing processes. 相似文献