首页 | 本学科首页   官方微博 | 高级检索  
文章检索
  按 检索   检索词:      
出版年份:   被引次数:   他引次数: 提示:输入*表示无穷大
  收费全文   517篇
  免费   3篇
  国内免费   79篇
安全科学   18篇
废物处理   9篇
环保管理   58篇
综合类   233篇
基础理论   65篇
污染及防治   153篇
评价与监测   55篇
社会与环境   8篇
  2023年   11篇
  2022年   16篇
  2021年   12篇
  2020年   15篇
  2019年   13篇
  2018年   14篇
  2017年   10篇
  2016年   19篇
  2015年   37篇
  2014年   28篇
  2013年   26篇
  2012年   28篇
  2011年   46篇
  2010年   31篇
  2009年   44篇
  2008年   54篇
  2007年   44篇
  2006年   30篇
  2005年   16篇
  2004年   14篇
  2003年   13篇
  2002年   15篇
  2001年   8篇
  2000年   19篇
  1999年   7篇
  1998年   1篇
  1997年   6篇
  1996年   7篇
  1995年   4篇
  1994年   1篇
  1993年   1篇
  1989年   1篇
  1988年   1篇
  1986年   1篇
  1985年   1篇
  1984年   2篇
  1980年   1篇
  1979年   1篇
  1977年   1篇
排序方式: 共有599条查询结果,搜索用时 15 毫秒
141.
Assessment of yield losses in tropical wheat using open top chambers   总被引:2,自引:0,他引:2  
The present study deals with the evaluation of effects of ambient gaseous air pollution on wheat (Triticum aestivum L. var. HUW-234) growing in a suburban area situated in eastern Gangetic plain of India, using open top chambers. Eight hourly air monitoring was conducted for ambient concentrations of SO2, NO2 and O3 in filtered chambers (FCs), non-filtered chambers (NFCs) and open plots (OPs). Various morphological, physiological and biochemical parameters were assessed during different developmental stages and finally yield parameters were quantified at the time of harvest.Mean concentrations of SO2, NO2 and O3 were 8.4, 39.9 and 40.1 ppb, respectively during the experiment in NFCs. Concentrations of SO2, NO2 and O3 reduced by 74.6%, 84.7% and 90.4%, respectively in FCs as compared to NFCs. Plants grown in FCs showed higher photosynthetic rate, stomatal conductance, chlorophyll content and Fv/Fm ratio as compared to the plants in NFCs and OPs. Lipid peroxidation, proline, total phenol and ascorbic acid contents and peroxidase activity were higher in plants grown in NFCs. There were improvements in morphological parameters of plants growing in FCs as compared to those in NFCs and OPs. Yield of plants also increased significantly in FCs as compared to those ventilated with ambient air (NFCs) or grown in OPs. During the vegetative phase, NO2 concentrations were higher than O3, but O3 became dominant pollutant during the time of grain setting and filling. The study concludes that O3 and NO2 are the main air pollutants in the sub-urban areas causing significant yield reductions in tropical wheat plants.  相似文献   
142.
In this paper, a shifted power-law model, based on the wind profile model, had been supposed to simulate concentration gradient of nitrogen dioxide (NO2) with distance from a highway. Field experiments were performed for NO2 gradients from a highway in Shanghai by using passive samplers. The shifted power-law model was fitted well with experimental results of field experiments both in this study and in the literature. The results not only verified the validity of shifted power-law relationship between NO2 concentration and the distance from a highway, but also partially demonstrated that there were some significant similarities between wind profile and air pollutants concentration profile near highway. With known concentration of chosen reference point and appropriate value of the parameter k, the model could be practically applied for predicting the NO2 distributions near a highway. The methods of determining the parameter k were also discussed for further detailed studies.  相似文献   
143.
This research consists of a laboratory study and a field study. The laboratory research reports the formation of NOx from a point to plane corona discharge. Discharge polarity and relative humidity determined the amount of NOx that was produced. The positive point discharge caused more NOx to form than the negative point discharge. For both polarities NOx production showed a nonlinear increase with current. Relative humidity enhanced the NOx formation for both polarities. In each case, the amount of NOx formed was comparable to the quantity of N2O produced from corona discharge. The research also reports the results from a field study that measured the amounts of 03 and NO2 produced by corona discharge during a thunderstorm. The study found that the ambient concentrations of 03 and NO2 increased several fold due to corona discharge and returned to original levels after the thunderstorm.  相似文献   
144.
Walker JT  Geron CD  Vose JM  Swank WT 《Chemosphere》2002,49(10):1389-1398
In this paper, we present two years of seasonal nitric oxide (NO), ammonia (NH3), and nitrous oxide (N2O) trace gas fluxes measured in a recovering riparian zone with cattle excluded and adjacent riparian zone grazed by cattle. In the recovering riparian zone, average NO, NH3, and N2O fluxes were 5.8, 2.0, and 76.7 ng N m−2 s−1 (1.83, 0.63, and 24.19 kg N ha−1 y−1), respectively. Fluxes in the grazed riparian zone were larger, especially for NO and NH3, measuring 9.1, 4.3, and 77.6 ng N m−2 s−1 (2.87, 1.35, and 24.50 kg N ha−1 y−1) for NO, NH3, and N2O, respectively. On average, N2O accounted for greater than 85% of total trace gas flux in both the recovering and grazed riparian zones, though N2O fluxes were highly variable temporally. In the recovering riparian zone, variability in seasonal average fluxes was explained by variability in soil nitrogen (N) concentrations. Nitric oxide flux was positively correlated with soil ammonium (NH4+) concentration, while N2O flux was positively correlated with soil nitrate (NO3) concentration. Ammonia flux was positively correlated with the ratio of NH4+ to NO3. In the grazed riparian zone, average NH3 and N2O fluxes were not correlated with soil temperature, N concentrations, or moisture. This was likely due to high variability in soil microsite conditions related to cattle effects such as compaction and N input. Nitric oxide flux in the grazed riparian zone was positively correlated with soil temperature and NO3 concentration. Restoration appeared to significantly affect NO flux, which increased ≈600% during the first year following restoration and decreased during the second year to levels encountered at the onset of restoration. By comparing the ratio of total trace gas flux to soil N concentration, we show that the restored riparian zone is likely more efficient than the grazed riparian zone at diverting upper-soil N from the receiving stream to the atmosphere. This is likely due to the recovery of microbiological communities following changes in soil physical characteristics.  相似文献   
145.
通过介绍环境空气中二氧化氮的测定方法──自动仪器监测法,对有关问题进行了初步探讨和研究,为正确使用该方法和仪器,确保监测工作的顺利进行提供了依据。  相似文献   
146.
马俊  张永祥  付冰 《环境科技》2005,18(Z1):24-26
通过试验,分别考察了不同HRT、DO、混合液和污泥回流比、温度等条件下,A2/O工艺的脱氮效果和有机物去除效果.结果表明,对于城市生活污水而言,当好氧区水力停留时间为6 h、DO为4 mg/L、混合液回流比为300%、污泥回流比为100%时,A2/O工艺能获得较好的脱氮效果和有机物去除效果.同时,也对如何控制运行中发生的丝状菌型污泥膨胀问题进行了初步的研究,并通过投加次氯酸钠和补充新鲜污泥的方法成功地控制了一次污泥膨胀.  相似文献   
147.
Nitrogen in pond sediments is a major water quality concern and can impact the productivity of aquaculture. Dissolved oxygen is an important factor for improving water quality and boosting fish growth in aquaculture ponds, and plays an important role in the conversion of ammonium-nitrogen (NH4+-N) to nitrite-nitrogen (NO2?-N) and eventually nitrate-nitrogen (NO3?-N). A central goal of the study was to identify the best aeration method and strategy for improving water quality in aquaculture ponds. We conducted an experiment with six tanks, each with a different aeration mode to simulate the behavior of aquaculture ponds. The results show that a 36 hr aeration interval (Tc = 36 hr: 36 hr) and no aeration resulted in high concentrations of NH4+-N in the water column. Using a 12 hr interval time (Tc = 12 hr: 12 hr) resulted in higher NO2?-N and NO3?-N concentrations than any other aeration mode. Results from an 8 hr interval time (Tc = 8 hr: 8 hr) and 24 hr interval time (Tc = 24 hr: 24 hr) were comparable with those of continuous aeration, and had the benefit of being in use for only half of the time, consequently reducing energy consumption.  相似文献   
148.
Dissolved oxygen (DO) concentration is regarded as one of the crucial factors to influence partial nitrification process. However, achieving and keeping stable partial nitrification under different DO concentrations were widely reported. The mechanism of DO concentration influencing partial nitrification is still unclear. Therefore, in this study two same sequencing batch reactors (SBRs) cultivated same seeding sludge were built up with real-time control strategy. Different DO concentrations were controlled in SBRs to explore the effect of DO concentration on the long-term stability of partial nitrification process at room temperature. It was discovered that ammonium oxidation rate (AOR) was inhibited when DO concentration decreased from 2.5 to 0.5 mg/L. The abundance of Nitrospira increased from 1011.5 to 1013.7 copies/g DNA, and its relative percentage increased from 0.056% to 3.2% during 190 operational cycles, causing partial nitrification gradually turning into complete nitrification process. However, when DO was 2.5 mg/L the abundance of Nitrospira was stable and AOB was always kept at 1010.7 copies/g DNA. High AOR was maintained, and stable partial nitrification process was kept. Ammonia oxidizing bacteria (AOB) activity was significantly higher than nitrite oxidizing bacteria (NOB) activity at DO of 2.5 mg/L, which was crucial to maintain excellent nitrite accumulation performance.  相似文献   
149.
Estuarine wetland is the transitional interface linking terrestrial with marine ecosystems, and wetland microbes are crucial to the biogeochemical cycles of nutrients. The soil samples were collected in four seasons (spring, S1; summer, S2; autumn, S3; and winter, S4) from Suaeda wetland of Shuangtaizi River estuary, Northeast China, and the variations of bacterial community were evaluated by high-throughput sequencing. Soil properties presented a significant seasonal change, including pH, carbon (C) and total nitrogen (TN), and the microbial diversity, richness and structure also differed with seasons. Canonical correspondence analysis (CCA) and Mantel tests implied that soil pH, C and TN were the key factors structuring the microbial community. Gillisia (belonging to Bacteroidetes) and Woeseia (affiliating with Gammaproteobacteria) were the two primary components in the rhizosphere soils, displaying opposite variations with seasons. Based on PICRUSt (Phylogenetic Investigation of Communities by Reconstruction of Unobserved States) prediction, the xenobiotics biodegradation related genes exhibited a seasonal decline, while the majority of biomarker genes involved in nitrogen cycle showed an ascending trend. These findings could advance the understanding of rhizosphere microbiota of Suaeda in estuarine wetland.  相似文献   
150.
Reclamation of degraded grasslands as managed grasslands has been increasingly accelerated in recent years in China. Land use change affects soil nitrogen(N) dynamics and nitrous oxide(N_2O) emissions. However, it remains unclear how large-scale grassland reclamation will impact the grassland ecosystem as a whole. Here, we investigated the effects of the conversion from native to managed grasslands on soil N dynamics and N_2O emissions by field experiments in Hulunber in northern China. Soil(0–10 cm), nitrate(NO_3~-),ammonium(NH_4~+), and microbial N were measured in plots in a temperate steppe(Leymus chinensis grassland) and two managed grasslands(Medicago sativa and Bromus inermis grasslands) in 2011 and 2012. The results showed conversion of L. chinensis grassland to M.sativa or B. inermis grasslands decreased concentrations of NO_3~–-N, but did not change NH_4~–N . Soil microbial N was slightly decreased by the conversion of L. chinensis grassland to M.sativa, but increased by the conversion to B. inermis. The conversion of L. chinensis grassland to M. sativa(i.e., a legume grass) increased N_2O emissions by 26.2%, while the conversion to the B. inermis(i.e., a non-legume grass) reduced N_2O emissions by 33.1%. The conversion from native to managed grasslands caused large created variations in soil NO?3~-+–N and NH_4~–N concentrations. Net N mineralization rates did not change significantly in growing season or vegetation type, but to net nitrification rate. These results provide evidence on how reclamation may impact the grassland ecosystem in terms of N dynamics and N_2O emissions.  相似文献   
设为首页 | 免责声明 | 关于勤云 | 加入收藏

Copyright©北京勤云科技发展有限公司  京ICP备09084417号