The spatial distribution of ammonia emitted from seabirds and its contribution to atmospheric nitrogen deposition in the UK

Simple bioenergetics models were used to derive annual nitrogen excretion rates of each seabird species occurring at colonies in the UK. These were combined with population distribution data and an estimated fraction of nitrogen volatilized to estimate the spatial distribution of NH₃ emissions from seabird colonies at a 1 km resolution. The effect of these emissions on atmospheric NH₃ concentrations and nitrogen deposition in the UK was assessed using the FRAME atmospheric chemistry and transport model. The total emission of NH₃ from the UK seabird colonies is estimated at 2.7 kt yr^–1. Emissions from seabirds are largely concentrated in remote parts of Britain, where agricultural and other anthropogenic emissions are minimal. Although seabirds account for less than 1% of total UK NH₃ emissions (370 kt yr^–1), their occurrence in remote areas and frequently large colony sizes results in seabirds providing a major fraction of the atmospheric nitrogen deposition for many remote ecosystems.     

Formation of Reactive Gaseous Mercury in the Arctic: Evidence of Oxidation of Hg° to Gas-Phase Hg-II Compounds after Arctic Sunrise

We have measured total gaseous mercury concentrations(Hg°) at Point Barrow, Alaska since September 1998 in aneffort to determine the geographic extent and reaction mechanismof the so-called mercury depletion events (MDE) previouslyreported in the high Arctic at Alert, Canada. Hg° has beensampled now for nearly 2 years at Barrow. In September, 1999, webegan making the first automated measurements of reactive gaseousmercury (RGM) attempted in the Arctic, along with measurements ofHg accumulation in snowpack to determine the fate of the depleted Hg°. During the fall and early winter, Hg°and RGM exhibit only minor variation, Hg° remaining within10% of global background, near 1.6–1.8 ng m^-3. The MDEperiods are quite different, however; within days of Arcticsunrise in January, Hg° exhibits major variations from themean, rapidly dropping as low as 0.05 ng m^-3 and then cyclingback to typical levels, sometimes exceeding global background. These events continue throughout Arctic spring, then end abruptlyfollowing snowmelt, in early June. Prior to Arctic sunrise, RGMremains near detection (<2 pg m^-3), but after sunriseincreases dramatically (to levels as high as 900 pg/m³) insynchrony with the depletion of Hg°. Both phenomenaexhibit a strong diel cycle, in parallel with UV-B. We concludethat MDE's involve rapid in-air oxidation of Hg° to aspecies of RGM by photochemically-driven reactions, probablyinvolving the same reactive bromine and chlorine compoundsinvolved in ozone destruction. Sharp increases in Hg in thesurface snowpack after sunrise coincident with periods of peakRGM suggest surface accumulation of the RGM by dry deposition.     

On the Size Dependence of Particle Deposition

Measurements of dry deposition ofparticles 0.1 to 1.0 m diameter to forest bythroughfall and eddy correlation methods giveresults of 1.0 cm s^-1 or more, whilemechanistic models do not explain values greaterthan about 1 mm s^-1. Results of othermethods involving radioactive tracers arerecalled. These data indicate values of about 5 mm s^-1. The possibility of additionalmechanisms, omitted from the models, is difficultto exclude, but much of the remaining discrepancymay be due to the wide size distribution of theadventitious radioactive tracers in the atmosphere.     

SEDIMENT DEPOSITION ESTIMATION FROM CESIUM-137 MEASUREMENTS1

ABSTRACT The movement of fallout ¹³⁷Cs carried by soil particles was studied as an indicator of erosion and sedimentation in the Allerton watersheds and 4-H Memorial Lake located near Monticello, Illinois. Sediment deposition was greater in the waterway draining from watershed IB than in the waterway from watershed IA. At the average rate of 2.3 cm/yr of sediment deposition in the lake (from 1954 to 1979), there will be a loss of over 2 meters of water depth in the next century. However, there appears to be a decreasing rate of sediment deposition in the 4-H Memorial Lake as a result of improved conservation practices on the watersheds and the increased effectiveness of vegetated waterways and buffers for retaining sediment.     

格子Boltzmann方法及其在泥石流堆积研究中的应用

以格子Boltzmann方法为平台,结合泥石流流团模型的特点,建立了特殊的格子Boltzmann模型。该模型从平衡态分布函数和非平衡态分布函数两个层次精细刻画了泥石流运动的非线性特征及其复杂的流变关系,成功模拟了泥石流的堆积过程,研究了地面形态与泥石流堆积形态之间的关系。     

Why Critical Loads of Acidity and N for Soils Should be Based on Pollutant Effective Concentrations Rather Than Deposition Fluxes

Numerous assumptions have been made over the past 17 years when calculating critical loads for soils, both for acidity (based upon base cation steady state mass balances (SMB)) and for N (eutrophication, based upon N mass balances), often without all the assumptions being explicitly stated. The tacit assumptions that the author believes to be implicit in the SMB approach are critically reviewed, with particular reference to upland regions where slope processes are highly significant. It is concluded that many of them cannot be justified, especially those that involve ignoring many key processes known to be important to biogeochemical cycling and soil evolution in upland catchments. The evidence presented suggests that critical loads of acidity and of N for soils should be based upon effective pollutant and, for acidity, also effective base cation deposition concentrations, rather than upon pollutant deposition fluxes. This is because of the dominant role of cation exchange equilibria, rather than weathering rate, in regulation of the pH and base status of the more acidification-sensitive soils, and because of the importance of transport down slope of base cations, alkalinity and N species.     

Evaluation of anthropogenic atmospheric inputs on US national park ecosystems

It is estimated that more than half the threats to national park resources originate outside park boundaries, and most threats are attributable to degradation of air and water quality. Atmospheric contaminants are the principal source of external threats to national park ecosystems. This article examines the potential impact to national park resources by anthropic atmospheric inputs and summarizes present research methods and results regarding impacts. Air quality monitoring currently receives much more emphasis and support than effects research. Present research on effects focuses on vegetation impact, biomonitoring, and acid rain. This research and that of other investigators suggest that the most likely impacts will not be direct cause-effect situations, but indirect, incremental, and possibly synergistic effects on the interactions of ecosystem components. Conceptually, such alteration of interactions can be measured through long-term observation of biogeochemical cycles, energy transfer, and community structure and function. But traditional Park Service research has not emphasized the ecosystem and especially ecosystem processes and component interactions. Most research on effects, then, must begin with baseline data acquisition. A research program to mitigate present national data base deficiencies would require a fundamental change in present research priorities, administration, and funding.     

State-of-the-art science and environmental assessments: the case of acid deposition

Scientific quality in a technical policy document is defined in terms of the proportion of contemporary scientific principles on a subject that the document competently discusses. As a case study of the scientific quality of such documents, this articles examines the treatment of acid deposition effects in 126 environmental impact statements on fossil-fuel power plants. On average, the relevant environmental statements cover only a quarter of the eligible scientific principles. Bureaucratic and political factors influence the quality of discussion of acid deposition more than do strictly objective or scientific factors. In particular, public participation and interagency review processes foster relatively thorough consideration of scientific information in environmental impact statements.     

A COMPARISON OF THREE METHODS FOR MEASURING RECENT RATES OF SEDIMENT ACCUMULATION1

ABSTRACT: The determination of sediment accumulation rates is important in understanding how these materials are affecting lakes and reservoirs ecosystems. In this study three methods were used to estimate sediment accumulation rates in the impounded backwater lakes behind Lock and Dam Nos. 8 and 9 on the upper Mississippi River. The three methods were: 1) a “spud” survey, 2) a survey of bottom contours, and 3) the use of fallout cesium-137. The field use of these three methods of determining sediment accumulation and the potential errors and merits involved in each method are discussed. The results from the field study in backwater areas along the upper Mississippi River showed the survey of bottom contour method gave the lowest rate of sediment deposition and the ¹³⁷Cs method gave the highest rates. Sediment accumulation rates from 0 to 7.8 cm per year were measured in the study area. All three methods are useful and have unique characteristics for determining rates and patterns of sediment accumulation. Thus the choice of a method to be used in a sediment survey is dependent on the type of information needed and the time available.     

NUMERICAL TECHNIQUES APPLIED TO PARTICLE DEPOSITION DURING SLOT FLOW1

ABSTRACT A mathematical model is presented of the process of particle sedimentation from a fluid-solid slurry while flowing through a vertical slot. The differential equations describing the process consist of 1st order, non-linear, partial differential equation and a 1st order, ordinary differential equation. These two equations have been solved using a forward difference technique. Results for typical sets of system parameters are presented and discussed. The model finds practical application to solid-waste disposal processes and to petroleum reservoir stimulation processes.