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911.
912.
煤矸石风化物不同粒级中重金属镉含量及其形态变化 总被引:1,自引:0,他引:1
对抚顺西露天矿煤矸石山表层煤矸石风化母岩进行多点取样,风化物筛分成>2 mm、2~0.25 mm和<0.25 mm等3个粒级,分析测定了矸石山表层母岩及其风化物不同粒级中Cd含量及其形态变化特征.结果表明:煤矸石母岩及其风化物中cd含量超过土壤环境质量2级标准,页岩、泥岩及其风化物pH值7.2~8.6,但燃后泥岩pH值4.9.碳质页岩2~0.25 mm粒级风化物中Cd损失最多,为73.6%;<0.25 mm细粒级Cd损失较少,为17.0%,这与细颗粒的表面吸附作用有关;泥岩及其各粒级风化物Cd元素不易损失,其Cd含量变化也相对较小;但燃后泥岩风化物中的Cd较容易损失.煤矸石风化物各样品类型中的Cd均以残渣态为主,可还原态和弱酸可提取态所占比例次之,可氧化态所占比例最小.弱酸可提取态Cd在细颗粒风化物中所占比例较高. 相似文献
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916.
Hwang IH Aoyama H Matsuto T Nakagishi T Matsuo T 《Waste management (New York, N.Y.)》2012,32(3):410-416
Hydrothermal treatments using subcritical water (HTSW) such as that at 234 °C and 3 MPa (LT condition) and 295 °C and 8 MPa (HT condition) were investigated to recover solid fuel from municipal solid waste (MSW). Printing paper, dog food (DF), wooden chopsticks, and mixed plastic film and sheets of polyethylene, polypropylene, and polystyrene were prepared as model MSW components, in which polyvinylchloride (PVC) powder and sodium chloride were used to simulate Cl sources.While more than 75% of carbon in paper, DF, and wood was recovered as char under both LT and HT conditions, plastics did not degrade under either LT or HT conditions. The heating value (HV) of obtained char was 13,886-27,544 kJ/kg and was comparable to that of brown coal and lignite. Higher formation of fixed carbon and greater oxygen dissociation during HTSW were thought to improve the HV of char.Cl atoms added as PVC powder and sodium chloride to raw material remained in char after HTSW. However, most Cl originating from PVC was found to converse into soluble Cl compounds during HTSW under the HT condition and could be removed by washing.From these results, the merit of HTSW as a method of recovering solid fuel from MSW is considered to produce char with minimal carbon loss without a drying process prior to HTSW. In addition, Cl originating from PVC decomposes into soluble Cl compound under the HT condition. The combination of HTSW under the HT condition and char washing might improve the quality of char as alternative fuel. 相似文献
917.
Comparing the greenhouse gas emissions from three alternative waste combustion concepts 总被引:1,自引:0,他引:1
Three alternative condensing mode power and combined heat and power (CHP) waste-to-energy concepts were compared in terms of their impacts on the greenhouse gas (GHG) emissions from a heat and power generation system. The concepts included (i) grate, (ii) bubbling fluidised bed (BFB) and (iii) circulating fluidised bed (CFB) combustion of waste. The BFB and CFB take advantage of advanced combustion technology which enabled them to reach electric efficiency up to 35% and 41% in condensing mode, respectively, whereas 28% (based on the lower heating value) was applied for the grate fired unit. A simple energy system model was applied in calculating the GHG emissions in different scenarios where coal or natural gas was substituted in power generation and mix of fuel oil and natural gas in heat generation by waste combustion. Landfilling and waste transportation were not considered in the model. GHG emissions were reduced significantly in all of the considered scenarios where the waste combustion concepts substituted coal based power generation. With the exception of condensing mode grate incinerator the different waste combustion scenarios resulted approximately in 1 Mton of fossil CO2-eq. emission reduction per 1 Mton of municipal solid waste (MSW) incinerated. When natural gas based power generation was substituted by electricity from the waste combustion significant GHG emission reductions were not achieved. 相似文献
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919.
在自制电化学反应器中,以甲基橙模拟染料废水为处理对象,采用Box-Behnken Design响应面法研究了影响阴阳极同时作用电化学法处理染料废水的因素及其交互作用。实验得出各因素对废水脱色率影响的大小顺序为:电流密度> Fe3+浓度>Cl-浓度。各因素之间的交互作用对废水脱色率影响的大小顺序为:电流密度和Fe3+浓度>电流密度和Cl-浓度>Fe3+浓度和Cl-浓度。优化结果表明:Fe3+浓度为1.02 mmol/L、Cl-浓度为10.96 mmol/L、电流密度为11.52 mA/cm2时,最佳脱色率为94.67%。阴阳极同时作用电化学法对甲基橙去除效果显著。 相似文献
920.
采用溶胶-凝胶法制备了MnOx/TiO2催化剂,考察了n(Mn):n(Ti)、催化剂载体、气体流量对催化燃烧去除废气中正己烷效果的影响.实验结果表明:随着n(Mn):n(Ti)的增加,正己烷去除率先增加后减小,气体流量减小正己烷去除率增大;当n (Mn):n(Ti)为7.85%、气体流量为100 mL/min时,在240℃时正己烷的去除率为90%,MnOx/TiO2催化活性最大;MnOx/TiO2的催化活性优于MnOx/SiO2;SEM和XRD表征结果表明,所制备的MnOx/TiO2是一种活性物种MnOx高度分散的纳米结构催化剂. 相似文献