东南亚生物质燃烧输送影响我国西南气溶胶辐射特性研究

利用2013年地基CE-318太阳光度计观测数据,结合中分辨率成像光谱仪（MODIS）遥感产品和HYSPLIT后向轨迹分析,研究了一次东南亚生物质燃烧污染长距离输送至中国西南昆明站点过程（2013年4月5~8日）中,气溶胶光学特性和辐射特性的变化及其可能来源.结果表明,此次污染过程期间,我国西南地区生物质燃烧活动较少,而中南半岛地区生物质燃烧活动显著.4月5~7日,昆明站点气溶胶光学厚度（AOD）升高,消光波长指数（EAE）和吸收波长指数（AAE）均增大.此外,依据EAE和AAE分类方法,5~6日昆明站点以城市工业气溶胶为主,7~8日以生物质燃烧气溶胶为主,其细模态峰值半径（0.11μm）小于5~6日（0.15μm）,7日细模态粒子体积浓度峰值（约为0.16μm³/μm²）是5日的2倍.气溶胶直接辐射强迫（ARF）日变化结果表明4月7日气溶胶对地表的降温效应达到最大,对大气的加热作用最强.气溶胶直接辐射强迫效率值（ARFE）的变化表明生物质燃烧气溶胶对大气顶的降温作用减弱.MODIS遥感以及HYSPLIT模式后向轨迹表明,此次昆明站点生物质燃烧气溶胶主要来源于东南亚地区（主要是印度北部、印缅北部和不丹地区）.     

基于神经网络的东北地区秸秆焚烧预测

选取农作物秸秆露天燃烧严重的东北地区,采用人工神经网络的方法,结合卫星火点和气象数据,开展秸秆露天燃烧预测研究.结果表明：人工神经网络预测模型成功验证了松嫩平原地区2015年10月25日~11月15日的秸秆露天燃烧情况,其准确度为67.1%,经过多次试验,在神经网络建模与验证数据配比为80：20时,预测准确度最高,可达69.7%,同时该模型的稳定性较好.而对不同区域,不同时间段的预测研究表明,人工神经网络较适用于长时间序列的预测.就影响因素而言,相对湿度是影响秸秆露天燃烧的最重要因素.本研究结果可为空气质量模式提供火点预测数据,提高其预报预警能力,为区域联防联控政策的制定提供科技支持.     

Large-scale mercury variations in Lake Vänern (Sweden) 1974-98

Lake V?nern, the largest lake in Sweden, has been seriously contaminated with mercury during the 20th century. In the 1970's and 80's the direct load, mainly from a chlor-alkali industry in the area, of mercury was drastically reduced as a response to new legislation, from three to five tons down to between five and ten kg yr(-1). Large amounts of the disposed pollutant have accumulated in the sediments. The question posed in this work is now, is the effect of the drastic load reduction after more than two decades visible in the sediments? The question is relevant as large areas still are blacklisted for fishing, but also as a follow-up of a major remedy action. The lake also serves as a freshwater reservoir for even Sweden's second largest city. This work synthesises and compares data of mercury in the sediments from three major field programs, in 1974, 1984 and 1998. The interest is focused on both spatial heterogeneity and temporal trends. In 1974, the surface concentrations are significantly higher than in subsequent surveys. Significant differences are also found between 1984 and 1998. Significant spatial differences within the lake are found for respective year. The most contaminated area is located in the north, close to the major point source (a former chlor-alkali industry). This is also the area with the largest improvement, as a direct response to the reduction in load. Further from the outlet, the recovery is more affected by burial and transport processes out into the deeper basins.     

Exposure Assessment to Mercury Vapor in Chloralkali Industry

The aim of the study was to develop a sampling method aimed at individual sampling of mercury vapor and subsequent individualexposure assessment of the worker. Hopcalite available fromInowrocawskie Zakady Chemiczne (in Poland) was founduseful for mercury vapor sampling in active and passive individual samplers. However the sampling rate determined forpassive sampler in steady-state laboratory chamber cannot be usedunder fluctuating conditions of mercury vapor concentration andair movement typical for field measurement. In order to check comparativeness of passive and active sampling methods, sampleswere taken in the same time and individual samplers fixed toworker's clothes were used. Mercury vapor concentration wasmeasured at two chloralkali industries in Poland and the resultswere presented. Excessive exposure in both industries wasconfirmed by finding elevated mercury concentration in urinesamples from the workers.     

MERCURY EMISSION INVENTORY IN ONTARIO

Mercury is released to the environment from various anthropogenic and natural sources. This work is a compilation of mercury emissions from anthropogenic sources in Ontario, Canada. The goal of our study was to identify all sources of mercury, and develop an emission inventory of anthropogenic mercury in Ontario. The result of our investigation revealed that combustion of fossil fuels and emissions from landfill sites are two primary sources of mercury to the atmosphere. Other sources of significance are emissions from waste incinerators, various industrial activities, and cement production. Total mercury emission in Ontario is estimated as 4100 kg per year.     

Potential for carbon sequestration in Canadian forests and agroecosystems

The potential for carbon (C) sequestration was examined in selectedCanadian forest settings and prairie agroecosystems under severalmanagement scenarios. A simple C budget model was developed toquantitatively examine C sequestration potential in living biomass of forestecosystems, in associated forest-product C pools, and in displaced fossil-fuelC. A review of previous studies was conducted to examine C sequestrationpotential in prairie agroecosystems. In the forest settings examined, ourwork suggests that substantial C sequestration opportunities can be realizedin the short term through the establishment of protected forest-C reserves.Where stands can be effectively protected from natural disturbance, peaklevels of biomass C storage can exceed that under alternative managementstrategies for 200 years or more. In settings where it is not feasible tomaintain protected forest-C reserves, C sequestration opportunities can berealized through maximum sustained yield management with harvestedbiomass put towards the displacement of fossil fuels. Because there is afinite capacity for C storage in protected forest-C reserves, harvesting forestbiomass and using it to displace the use of fossil fuels, either directlythrough the production of biofuels or indirectly through the production oflong-lived forest products that displace the use of energy-intensive materialssuch as steel or concrete, can provide the greatest opportunity to mitigategreenhouse gas emissions in the long term. In Canadian prairieagroecosystems, modest C sequestration can be realized while enhancingsoil fertility and improving the efficiency of crop production. This can bedone in situations where soil organic C can be enhanced without relianceupon ongoing inputs of nitrogen fertilizer, or where the use of fossil fuelsin agriculture can be reduced. More substantial C offsets can be generatedthrough the production of dedicated energy crops to displace the use offossil fuels. Where afforestation or reconstruction of native prairieecosystems on previously cultivated land is possible, this represents thegreatest opportunity to sequester C on a per unit-area basis. However,these last two strategies involve the removal of land from crop production,and so they are not applicable on as wide a scale as some other Csequestration options which only involve modifications to currentagricultural practices.     

On the determination of nitrous oxide emission factor during biomass burning

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Status of mercury pollution during resources development in Guizhou Province, China

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生物质气化洗焦废水的预处理和微生物降解

为了对生物质气化洗焦废水进行深度处理,达到废水排放标准,采用物理过滤和微生物降解相结合的方法,对洗焦废水的原液进行处理。实验结果表明,用木屑、颗粒活性碳、微生物降解的连续步骤处理生物质气化洗焦废水,可达到理想的生物质气化洗焦废水COD的去除效果。     

镉、汞、铅在体内对氨基酸掺入微粒体的特异性抑制作用

本实验采用DL-(~3H)-亮氨酸作为蛋白质合成的原料,从亚细胞水平观察镉、汞、铅在动物体内对肝脏各亚细胞组分蛋白合成的影响。实验结果表明,给雄性大鼠腹腔一次注入2.4mg/kg醋酸镉后72h和一次注给2.0mg/kg氯化汞或100mg/kg醋酸铅后24h,均可不同程度地抑制DL-(~3H)-亮氨酸掺入微粒体蛋白,而对其它组分包括细胞核、线粒体、去微粒体后上清液蛋白中DL-(~3H)-亮氨酸的掺入无明显影响。