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161.
Quantifying the importance of diffuse minewater pollution in a historically heavily coal mined catchment 总被引:1,自引:0,他引:1
Mayes WM Gozzard E Potter HA Jarvis AP 《Environmental pollution (Barking, Essex : 1987)》2008,151(1):165-175
There has been considerable progress in developing treatment systems for point sources of minewater pollution in recent years; however, there remains a knowledge gap in the characterisation and remediation of diffuse minewater sources. Data are presented from the River Gaunless catchment, a historically heavily coal mined catchment in the northeast of England. Instream iron (Fe) loadings were monitored alongside loadings arising from point minewater discharges over a 12-month period to assess the dynamic importance of diffuse sources of minewater pollution. In low flow, diffuse sources account for around 50% of instream loading, a proportion which increases to 98% in high flow conditions. The low flow sources appear to be dominated by direct discharge of contaminated groundwater to surface waters in lower reaches of the catchment. In high flow, resuspended Fe-rich sediments, which are both naturally occurring and derived from historic mining, become the dominant diffuse source of Fe in the water column. 相似文献
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163.
A substantial percentage of days with below normal temperatures in central Illinois during May and June (1956-1965) appear to be associated with polar air masses which traverse the Hudson Bay area before entering the Midwest. January departures, in contrast, are related to polar air masses that enter the United States near the Mackenzie River in western Canada. The general influences of the Hudson Bay area on climate are discussed. 相似文献
164.
Naphthenic acids are complex mixtures of alkyl-substituted acyclic and cycloaliphatic carboxylic acids, with the general chemical formula CnH2n+zO2, where n is the carbon number and Z specifies a homologous family. These acids have a variety of commercial uses, including being used as wood preservatives. They are found in conventional and heavy oils, and in the oil sands of northeastern Alberta, Canada. Naphthenic acids are major contributors to the toxicity of tailings waters that result from the oil sands extraction process. Eight naphthenic acids preparations (four from commercial sources and four from the oil sands operations) were derivatized and analyzed by gas chromatography–mass spectrometry. The composition of each mixture was summarized as a three-dimensional plot of the abundance of specific ions (corresponding to naphthenic acids) versus carbon number (ranging from 5 to 33) and Z family (ranging from 0 to −12). The data in these plots were divided into three groups according to carbon number (group 1 contained carbon numbers 5–14, group 2 contained carbon numbers 15–21, and group 3 contained carbon numbers 22–33). A t-test, using arcsine-transformed data, was applied to compare corresponding groups in samples from various sources. Results of the statistical analyses showed differences between various commercial naphthenic acids preparations, and between naphthenic acids from different oil sands ores and tailings ponds. This statistical approach can be applied to data collected by other mass spectrometry methods. 相似文献
165.
Mass fluxes and spatial trends of xenobiotics in the waters of the city of Halle, Germany 总被引:1,自引:1,他引:1
Reinstorf F Strauch G Schirmer K Gläser HR Möder M Wennrich R Osenbrück K Schirmer M 《Environmental pollution (Barking, Essex : 1987)》2008,152(2):452-460
The behaviour and the effects of xenobiotics including pharmaceuticals and fragrances in the environment are widely unknown. In order to improve our knowledge, field investigations and modelling approaches for the entire area of the city of Halle/Saale, Germany, were performed. The distribution of the concentration values and mass fluxes are exemplified using indicators such as Bisphenol A, t-Nonylphenol, Carbamacepine, Galaxolide, Tonalide, Gadolinium and isotopes. Concentrations at a magnitude of ng/L to microg/L were found ubiquitously in the ground and surface waters. Using the concentration values, the impact of the city concerning the indicators was not always evident. Only the assessment of the mass fluxes shows significant urban impacts along the city passage. The calculation of the mass fluxes shows increasing values for all investigated xenobiotics during the city passage; only Bisphenol A stagnates. A balance model of water and indicator mass fluxes was built up for the entire city area. 相似文献
166.
The outcome of a 21-month monitoring study on anionic surfactants (AS) at five (27–70 ML/d) up-flow anaerobic sludge blanket (UASB) based sewage treatment plants (STPs) is described. The average removals of AS were around 8–30%. Appreciable concentrations of AS were being discharged to the watercourse (average 4.30 mg/L; range 3.60–4.91 mg/L). On an average dried sludge contained 1452 mg AS/kg dry weight. Mass balance at three STPs indicated that, AS load of the order of 5–17% and ≈12% is removed by adsorption in UASB reactors and polishing ponds (PP) respectively. Biodegradation of AS under anaerobic conditions in UASB reactors and PP does not seem to take place. In the sludge stream, appreciable biodegradation (≈46%) of adsorbed AS under aerobic conditions on the sludge drying beds takes place. If influent AS mass flux is normalized to 100 units, than average of ≈74 and ≈7 units are discharged with treated effluent and dried sludge respectively, while 12 and 6 units are adsorbed/settled in PP and aerobically biodegrade on sludge drying beds respectively. At two STPs (34 and 56 ML/d), the filterable fluxes in UASBR increased so that the mass balance could not be computed. 相似文献
167.
W.T. Hoo L.K. FifieldS.G. Tims T. FujiokaN. Mueller 《Journal of environmental radioactivity》2011,102(10):937-942
A study has been carried out to assess the potential of using fallout plutonium (Pu), which originated from atmospheric nuclear-weapons tests, as a tool to investigate recent erosional processes within the lower Cotter water-supply catchment in the Australian Capital Territory. This catchment, which was predominantly pine plantation, was severely affected by a major bush fire in 2003. Accelerator mass spectrometry has been used to measure Pu in soil samples collected from a number of sites across the catchment. The results indicate that less than 1 cm of surface soil had been lost since the early 1960s over much of the catchment. Areas of more erodible soil have, however, lost 2-4 cm of topsoil, and a loss of ∼6 cm of soil was identified at one particular site. 相似文献
168.
169.
Peroxy radicals (RO2), which are formed during the oxidation of volatile organic compounds, play an important role in atmospheric oxidation reactions. Therefore, the measurement of RO2, especially distinct species of RO2 radicals, is important and greatly helps the exploration of atmospheric chemistry mechanisms. Although the speciated detection of RO2 radicals remains challenging, various methods have been developed to study them in detail. These methods can be divided into spectroscopy and mass spectrometry technologies. The spectroscopy methods contain laser-induced fluorescence (LIF), UV-absorption spectroscopy, cavity ring-down spectroscopy (CRDS) and matrix isolation and electron spin resonance (MIESR). The mass spectrometry methods contain chemical ionization atmospheric pressure interface time-of-flight mass spectrometry (CI-APi-TOF), chemical ionization mass spectrometry (CIMS), CI-Orbitrap-MS and the third-generation proton transfer reaction–time-of-flight mass spectrometer (PTR3). This article reviews technologies for the speciated detection of RO2 radicals and the applications of these methods. In addition, a comparison of these techniques and the reaction mechanisms of some key species are discussed. Finally, possible gaps are proposed that could be filled by future research into speciated RO2 radicals. 相似文献
170.
石油化工建设项目环境影响评价中应注意的问题 总被引:6,自引:0,他引:6
我国是最早实施环境评价制度的发展中国家之一,建设项目的环境影响评价作为一项法律制度在我国已实施了20多年。根据实际工作经验,总结了在石油化工建设项目的环评工作中应注意的一些问题。 相似文献